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Pre-trained representation is one of the key elements in the success of modern deep learning. However, existing works on continual learning methods have mostly focused on learning models incrementally from scratch. In this paper, we explore…

Machine Learning · Computer Science 2022-08-18 Hyounguk Shon , Janghyeon Lee , Seung Hwan Kim , Junmo Kim

Machine-learning interatomic potentials (MLIPs) offer a powerful avenue for simulations beyond length and timescales of ab initio methods. Their development for investigation of mechanical properties and fracture, however, is far from…

Universal machine-learned interatomic potentials (U-MLIPs) have demonstrated effectiveness across diverse atomistic systems but often require fine-tuning for task-specific accuracy. We investigate the fine-tuning of two MACE-based…

Computational Physics · Physics 2025-06-10 Xiaoqing Liu , Kehan Zeng , Yangshuai Wang , Teng Zhao

Parameter-efficient fine-tuning (PEFT) of pre-trained language models (PLMs) has emerged as a highly successful approach, with training only a small number of parameters without sacrificing performance and becoming the de-facto learning…

Computation and Language · Computer Science 2023-10-20 Baohao Liao , Shaomu Tan , Christof Monz

Molecular dynamics (MD) employing machine-learned interatomic potentials (MLIPs) serve as an efficient, urgently needed complement to ab initio molecular dynamics (aiMD). By training these potentials on data generated from ab initio…

Materials Science · Physics 2024-09-19 Kisung Kang , Thomas A. R. Purcell , Christian Carbogno , Matthias Scheffler

The use of machine learning interatomic potentials (MLIPs) in simulations of materials is a state-of-the-art approach, which allows achieving nearly \textit{ab initio} accuracy with orders of magnitude less computational cost.…

Materials Science · Physics 2021-10-28 R. E. Ryltsev , N. M. Chtchelkatchev

Pre-trained large multi-modal models (LMMs) exploit fine-tuning to adapt diverse user applications. Nevertheless, fine-tuning may face challenges due to deactivated sensors (e.g., cameras turned off for privacy or technical issues),…

Computer Vision and Pattern Recognition · Computer Science 2024-03-19 Shu Zhao , Xiaohan Zou , Tan Yu , Huijuan Xu

Machine learning interatomic potentials (MLIPs) enables molecular dynamics (MD) simulations with ab initio accuracy and has been applied to various fields of physical science. However, the performance and transferability of MLIPs are…

Chemical Physics · Physics 2024-04-16 Taoyong Cui , Chenyu Tang , Mao Su , Shufei Zhang , Yuqiang Li , Lei Bai , Yuhan Dong , Xingao Gong , Wanli Ouyang

Universal machine learning interatomic potentials (uMLIPs) represent arguably the most successful application of machine learning to materials science, demonstrating remarkable performance across diverse applications. However, critical…

Materials Science · Physics 2025-08-26 Antoine Loew , Jonathan Schmidt , Silvana Botti , Miguel A. L. Marques

The rapid emergence of universal Machine Learning Interatomic Potentials (uMLIPs) has transformed materials modeling. However, a comprehensive understanding of their generalization behavior across configurational space remains an open…

Materials Science · Physics 2025-12-30 Hossein Tahmasbi , Andreas Knüpfer , Thomas D. Kühne , Hossein Mirhosseini

The rapid development of pretrained Machine Learning Interatomic Potentials (MLIPs) that cover a wide range of molecular species has made it challenging to select the best model for a given application. We benchmark 15 pretrained MLIPs,…

Chemical Physics · Physics 2026-04-22 Peter Eastman , Evan Pretti , Thomas E. Markland

Predictive simulation of electrochemical interfaces requires atomistic models that capture reactive bond rearrangements, long-range electrostatics, and charge distributions reflecting the electronic distinctness of electrode and…

Materials Science · Physics 2026-05-01 Akhil Reddy Peeketi , Blas P Uberuaga , Travis E Jones

Replaying past experiences has proven to be a highly effective approach for averting catastrophic forgetting in supervised continual learning. However, some crucial factors are still largely ignored, making it vulnerable to serious failure,…

Machine Learning · Computer Science 2023-11-21 Tiantian Zhang , Kevin Zehua Shen , Zichuan Lin , Bo Yuan , Xueqian Wang , Xiu Li , Deheng Ye

Pretrained language models (PLMs) are today the primary model for natural language processing. Despite their impressive downstream performance, it can be difficult to apply PLMs to new languages, a barrier to making their capabilities…

Computation and Language · Computer Science 2024-01-15 Yihong Chen , Kelly Marchisio , Roberta Raileanu , David Ifeoluwa Adelani , Pontus Stenetorp , Sebastian Riedel , Mikel Artetxe

We propose new methodologies for both unlearning random set of samples and class unlearning and show that they outperform existing methods. The main driver of our unlearning methods is the similarity of predictions to a retrained model on…

Machine Learning · Computer Science 2025-12-09 Ali Ebrahimpour-Boroojeny

Machine-learned interatomic potentials can offer near first-principles accuracy but are computationally expensive, limiting their application to large-scale molecular dynamics simulations. Inspired by quantum mechanics/molecular mechanics…

Materials Science · Physics 2025-11-21 Fraser Birks , Matthew Nutter , Thomas D Swinburne , James R Kermode

Evolution Strategies (ES) has recently emerged as a competitive alternative to reinforcement learning (RL) for large language model (LLM) fine-tuning, offering advantages through simplicity, scalability, and inference-only training.…

Machine Learning · Computer Science 2026-05-29 Kajetan Schweighofer , Conor F. Hayes , Roberto Dailey , Risto Miikkulainen , Xin Qiu

Machine learning interatomic potentials (MLIPs) have become increasingly effective at approximating quantum mechanical calculations at a fraction of the computational cost. However, lower errors on held out test sets do not always translate…

Computational Physics · Physics 2025-04-24 Xiang Fu , Brandon M. Wood , Luis Barroso-Luque , Daniel S. Levine , Meng Gao , Misko Dzamba , C. Lawrence Zitnick

Machine learning interatomic potentials (MLIPs) enable the accurate simulation of materials at larger sizes and time scales, and play increasingly important roles in the computational understanding and design of materials. However, MLIPs…

Materials Science · Physics 2023-07-27 Ji Qi , Tsz Wai Ko , Brandon C. Wood , Tuan Anh Pham , Shyue Ping Ong

Machine Learning Interatomic Potentials (MLIPs) have successfully demonstrated scaling behavior, i.e. the power-law improvement in training performance, however the emergence of novel capabilities at scale remains unexplored. We have…