Related papers: Circular RABBITT goes under threshold
The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) can become resonant with a discrete atomic level either in the intermediate or the final continuous states. Experimental observations of…
We study theoretically the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) in strongly polar molecules. The time-dependent energy of a polar molecule in the infrared (IR) field gives rise to an…
The scaled-up qubits proposed are molecules which display large amplitude motions at very low temperatures and the matrix that traps them. These comprise ionic solids such as ammonium tetraphenylborate (ATPB) or methane dilute in a xenon…
Quantum mechanically, photoionization can be fully described by the complex photoionization amplitudes that describe the transition between the ground state and the continuum state. Knowledge of the value of the phase of these amplitudes…
Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high…
This perspective introduces attosecond path qubits: measurement-defined two-level subsystems that arise naturally in strong-field physics from the coherent interference of distinguishable quantum pathways. These effective qubits are…
Following up on a recent paper [Bharti et al., Phys. Rev. A 109 (2024) 023110], we compare the predictions from severalR-matrix with time-dependence calculations for a modified three-sideband version of the "reconstruction of attosecond…
Attosecond chronoscopy represents a major breakthrough in the study of ultrafast phenomena and has the potential to revolutionize our understanding of the fundamental physics of matter. We theoretically investigate the…
We present an analytical model that characterizes two-photon transitions in the presence of autoionising states. We applied this model to interpret resonant RABITT spectra, and show that, as a harmonic traverses a resonance, the phase of…
Attosecond photoelectron spectroscopy is often performed with interferometric experimental setups that require outstanding stability. We demonstrate and characterize in detail an actively stabilized, versatile, high spectral resolution…
Quantum sensing is a rapidly growing field of research which is already improving sensitivity in fundamental physics experiments. The ability to control quantum devices to measure physical quantities received a major boost from…
Qudits, the multi-level generalization of qubits, provide a natural extension of the binary paradigm in quantum computation and offer new opportunities to enhance algorithmic performance. Beyond their direct applicability to the simulation…
Resonant transverse driving of a two-level system as viewed in the rotating frame couples two degenerate states at the Rabi frequency, an amazing equivalence that emerges in quantum mechanics. While spectacularly successful at controlling…
We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…
Mid-circuit measurement and reset of subsets of qubits is a crucial ingredient of quantum error correction and many quantum information applications. Measurement of atomic qubits is accomplished through resonant fluorescence, which…
We develop a novel technique for modeling of atomic and molecular ionization in superposition of XUV and IR fields with characteristics typical for attosecond streaking and RABBITT experiments. The method is based on solving the…
Angle-resolved (AR) RABBIT measurements offer a high information content measurement scheme, due to the presence of multiple, interfering, ionization channels combined with a phase-sensitive observable in the form of angle and time-resolved…
Attosecond measurements reveal new physical insights in photo ionization dynamics from atoms, molecules and condensed matter. However, on such time scales even small timing jitter can significantly reduce the time resolution in pump-probe…
An experiment based on a trapped Ytterbium ion validates the inertial theorem for the SU(2) algebra. The qubit is encoded within the hyperfine states of the atom and controlled by RF fields. The inertial theorem generates analytical…
High-harmonic spectroscopy driven by circularly-polarized laser pulses and their counter-rotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the…