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We performed high-dimensional quantum dynamical calculations of the dissociative adsorption and associative desorption of hydrogen on Cu(111). The potential energy surface (PES) is obtained from density functional theory calculations. Two…

mtrl-th · Physics 2009-10-28 A. Gross , B. Hammer , M. Scheffler , W. Brenig

A new nine-dimensional potential energy surface (PES) and dipole moment surface (DMS) for silane have been generated using high-level \textit{ab initio} theory. The PES, CBS-F12$^{\,\mathrm{HL}}$, reproduces all four fundamental term values…

Chemical Physics · Physics 2018-08-17 Alec Owens , Sergei N. Yurchenko , Andrey Yachmenev , Walter Thiel

Based on the many-body theory of metals in the third order of the perturbation expansion in electron-ion interaction pseudopotential, the potentials of pair and three-ion interactions are calculated in liquid lead, aluminium and beryllium…

Materials Science · Physics 2007-05-23 E. V. Vasiliu

In order to predict the potential energy surface (PES) from measured structure in equilibrium state, one should typically perform trial-and-error statistical thermodynamic simulation with assumed multibody interactions. Very recently, we…

Disordered Systems and Neural Networks · Physics 2017-07-11 Koretaka Yuge

A very accurate, (HF)$_2$ potential energy surface (PES) is constructed based on \ai\ calculations performed using the MOLPRO package at the CCSD(T) level of theory with an aug-cc-pvQz-F12 basis set at about 161~000 points. a higher…

Atomic and Molecular Clusters · Physics 2021-07-27 Roman I. Ovsyannikov , Vladimir Yu. Makhnev , Nikolai F. Zobov , Jacek Koput , Jonathan Tennyson

Machine-learned potential energy surfaces (PESs) for molecules with more than 10 atoms are typically forced to use lower-level electronic structure methods such as density functional theory and second-order Moller-Plesset perturbation…

Chemical Physics · Physics 2021-05-21 Chen Qu , Paul Houston , Riccardo Conte , Apurba Nandi , Joel M. Bowman

We present the first fully ab initio calculations of collision-induced broadening and shift of spectral lines in antiprotonic helium ($\bar{p}$He$^{+}$) perturbed by atomic helium. To overcome critical limitations of previous studies, we…

The particle exchange model of hadron interactions can be used to describe three-body scattering under the isobar assumption. In this study we start from the 3->3 scattering amplitude for spinless particles, which contains an…

Nuclear Theory · Physics 2017-09-12 M. Mai , B. Hu , M. Doring , A. Pilloni , A. Szczepaniak

We have used the hyperspherical adiabatic representation to describe the system of three identical bosons in an spin stretched state interacting by an attractive 1/r potential. A proposal has been made how such a system might be realized…

Atomic Physics · Physics 2007-05-23 J. P. D'Incao , S. C. Cheng , H. Suno , B. D. Esry

Hydrogen atom transfer (HAT) reactions are essential in many biological processes, such as radical migration in damaged proteins, but their mechanistic pathways remain incompletely understood. Simulating HAT is challenging due to the need…

Machine Learning · Computer Science 2025-11-25 Marlen Neubert , Patrick Reiser , Frauke Gräter , Pascal Friederich

In the interstellar medium (ISM), polycylic aromatic hydrocarbons (PAHs) are believed to be an important carbon reservoir, accounting for up to a quarter of all interstellar carbon in our galaxy. This makes the investigation of their…

Astrophysics of Galaxies · Physics 2025-06-23 Karina Sogomonyan , Malek Ben Khalifa , Phoebe Pierré , Jérôme Loreau

Different models for conserved two- and three-body electromagnetic currents are constructed from two- and three-nucleon interactions, using either meson-exchange mechanisms or minimal substitution in the momentum dependence of these…

Nuclear Theory · Physics 2014-11-18 L. E. Marcucci , M. Viviani , R. Schiavilla , A. Kievsky , S. Rosati

The construction of the potential energy surface (PES) of even a medium-sized molecule employing correlated theory, such as CCSD(T), is an arduous task due to the high computational cost. In this Letter, we report the possibility of…

Chemical Physics · Physics 2022-05-04 Subodh S. Khire , Nalini D. Gurav , Apurba Nandi , Shridhar R. Gadre

For a particular case of three-body scattering in two dimensions, and matching analytical expressions at a transition point, we obtain accurate solutions for the hyperspherical adiabatic basis and potential. We find analytical expressions…

Quantum Physics · Physics 2020-08-05 Monique Lassaut , Alejandro Amaya-Tapia , Anthony D. Klemm , Sigurd Yves Larsen

We study a system of $A$ identical interacting bosons trapped by an external field by solving ab initio the many-body Schroedinger equation. A complete solution by using, for example, the traditional hyperspherical harmonics (HH) basis…

Quantum Physics · Physics 2009-11-10 T. K. Das , B. Chakrabarti

The NH2 + O reaction represents a critical oxidation pathway in ammonia and hydrazine combustion, yet significant discrepancies persist in reported kinetics. Here, we generate a full-dimensional ground-state potential energy surface (PES)…

Chemical Physics · Physics 2026-03-24 Ying Xing , Weijie Hua , Junxiang Zuo

We study the $^6$He Borromean nucleus in coordinate representation within a three-body model with two-body potentials derived from cluster effective field theory (EFT). These potentials are originally developed in momentum space and Fourier…

Nuclear Theory · Physics 2025-06-03 E. C. Pinilla , W. Leidemann , G. Orlandini , P. Descouvemont

We have determined an atom-surface interaction potential for the He$-$Bi$_2$Te$_3$(111) system by analysing ultrahigh resolution measurements of selective adsorption resonances. The experimental measurements were obtained using $^3$He…

State-of-the-art ab initio techniques have been applied to compute the potential energy surface for the lithium atom interacting with the lithium hydride molecule in the Born-Oppenheimer approximation. The interaction potential was obtained…

The non-symmetrized hyperspherical harmonics method for a three-body system, composed by two particles having equal masses, but different from the mass of the third particle, is reviewed and applied to the $^3$H, $^3$He nuclei and…

Nuclear Theory · Physics 2018-10-22 A. Nannini , L. E. Marcucci