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Related papers: Three-body potential energy surface for parahydrog…

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We present an isotropic ab initio (para-H$_2$)$_4$ four-body interaction potential energy surface (PES). The electronic structure calculations are performed at the correlated coupled-cluster theory level, with single, double, and…

Chemical Physics · Physics 2025-06-09 Alexander Ibrahim , Pierre-Nicholas Roy

This paper presents two new adiabatic, global potential energy surfaces (PESs) for the two lowest $^3A'$ and $^3A''$ electronic states of the O($^3P$)+H$_2$ system. For each of these states, ab initio electronic energies were calculated for…

Atomic Physics · Physics 2019-10-02 Alexandre Zanchet , Marta Menéndez , Pablo G. Jambrina , F. Javier Aoiz

The interaction potential energy surface (PES) of He-H2 is of great importance for quantum chemistry, as the simplest test case for interactions between a molecule and a closed-shell atom. It is also required for a detailed understanding of…

Astrophysics · Physics 2009-11-07 Arnold I. Boothroyd , Peter G. Martin , Michael R. Peterson

We present path integral Monte Carlo simulation results for the equation of state of solid parahydrogen between $ 0.024 \, {\r{A}}^{-3} $ and $ 0.1 \, {\r{A}}^{-3} $ at $ T = 4.2 \, $ K. The simulations are performed using non-additive…

Chemical Physics · Physics 2025-06-09 Alexander Ibrahim , Pierre-Nicholas Roy

Reaction probabilities as a function of total angular momentum and the resulting reaction cross-sections for the collision of open shell S($^1$D) atoms with para-hydrogen have been calculated in the kinetic energy range 0.09--10 meV (1--120…

Chemical Physics · Physics 2015-05-28 Manuel Lara , P. G. Jambrina , A. J. C. Varandas , J. -M. Launay , F. J. Aoiz

Accurate potential energy surfaces (PESs) have been determined for the $^3$A$'$ and $^3$A$''$ states of N$_2$O using electronic structure calculations at the multireference configuration interaction level with Davidson correction (MRCI+Q)…

Chemical Physics · Physics 2020-11-06 Debasish Koner , Juan Carlos San Vicente Veliz , Raymond J. Bemish , Markus Meuwly

A detailed characterization of the interaction between the most abundant molecules in air is important for the understanding of a variety of phenomena in atmospherical science. A completely {\em ab initio} global potential energy surface…

We have calculated the three-dimensional potential energy surface (PES) for the fission of compound nucleus $^{236}$U using the covariant density functional theory with constraints on the axial quadrupole and octupole deformations…

Nuclear Theory · Physics 2023-05-30 Ming-Hui Zhou , Ze-Yu Li , Sheng-Yuan Chen , Yong-Jing Chen , Zhi-Pan Li

A new analytical potential energy surface (PES) has been constructed for H$_2^+$-He using a reproducing kernel Hilbert space (RKHS) representation from an extensive number of $ab initio$ energies computed at the multi-reference and full…

Chemical Physics · Physics 2020-07-07 Debasish Koner , Juan Carlos San Vicente Veliz , Ad van der Avoird , Markus Meuwly

Collisional excitation of light hydrides is important to fully understand the complex chemical and physical processes of atmospheric and astrophysical environments. Here, we focus on the NH(X3{\Sigma}-)-Ar van der Waals system. First, we…

Computational Physics · Physics 2019-06-28 D. Prudenzano , F. Lique , R. Ramachandran , L. Bizzocchi , P. Caselli

We present a first principles-quality potential energy surface (PES) describing the inter-atomic forces for hydrogen atoms interacting with free-standing graphene. The PES is a high-dimensional neural network potential that has been…

We present the equation of state (EOS) of solid parahydrogen between $ 0.024 \, {\r{A}}^{-3} $ and $ 0.1 \, {\r{A}}^{-3} $ at $ T = 4.2 $ K, calculated using path-integral Monte Carlo simulations, with ab initio two-body and three-body…

Chemical Physics · Physics 2025-06-05 Alexander Ibrahim , Pierre-Nicholas Roy

Constructing accurate, high dimensional molecular potential energy surfaces (PESs) for polyatomic molecules is challenging. Reproducing Kernel Hilbert space (RKHS) interpolation is an efficient way to construct such PESs. However, the…

Chemical Physics · Physics 2020-11-06 Debasish Koner , Markus Meuwly

Potential Energy Surface for the ($\mathrm{\bar{p}} - \mathrm{He}^{2+} - \mathrm{He}$) system is calculated in the framework of the restricted (singlet spin state) Hartree-Fock method with subsequent account of the electronic correlations…

Nuclear Theory · Physics 2017-06-29 S. N. Yudin , I. V. Bodrenko , G. Ya. Korenman

The reaction dynamics for the H + HeH$^+$ $\rightarrow$ He + H$_2^+$ reaction in its electronic ground state is investigated using two different representations of the potential energy surface (PES). The first uses a combined kernel and…

Chemical Physics · Physics 2025-03-28 Meenu Upadhyay , Silvan Käser , Jayakrushna Sahoo , Yohann Scribano , Markus Meuwly

Non-adiabatic effects play an important role in many chemical processes. In order to study the underlying non-adiabatic potential-energy surfaces (PESs), we present a locally-constrained density-functional theory approach, which enables us…

Materials Science · Physics 2015-06-25 Joerg Behler , Bernard Delley , Karsten Reuter , Matthias Scheffler

A new nine-dimensional potential energy surface (PES) for methane has been generated using state-of-the-art \textit{ab initio} theory. The PES is based on explicitly correlated coupled cluster calculations with extrapolation to the complete…

Chemical Physics · Physics 2016-10-12 Alec Owens , Sergey N. Yurchenko , Andrey Yachmenev , Jonathan Tennyson , Walter Thiel

A detailed interpretation of the detected emission lines of environments in which propyne (or methyl acetylene, CH$_3$CCH) is observed requires a knowledge of its collisional rate coefficients with the most abundant species in the…

Astrophysics of Galaxies · Physics 2024-02-28 M. Ben Khalifa , B. Darna , J. Loreau

A globally correct potential energy surface (PES) for the \hp\ molecular ion is presented. The Born-Oppenheimer (BO) \ai\ grid points of Pavanello et. al. [\textit{J. Chem. Phys.} {\bf 136}, 184303 (2012)] are refitted as BOPES75K, which…

Chemical Physics · Physics 2018-12-17 I. I. Mizus , O. L. Polyansky , Laura K. McKemmish , J. Tennyson , A. Alijah , N. F. Zobov

The Diep and Johnson (DJ) H$_2$-H$_2$ potential energy surface (PES) obtained from the first principles [P. Diep, K. Johnson, J. Chem. Phys. 113, 3480 (2000); 114, 222 (2000)], has been adjusted through appropriate rotation of the…

Chemical Physics · Physics 2015-03-19 Renat A. Sultanov , Dennis Guster , S. K. Adhikari
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