Related papers: Line shapes in time- and angle-resolved photoemiss…
Monolayer transition metal dichalcogenides (TMDCs) are direct gap semiconductors with unique potential for ultrathin light emitters. Yet, their photoluminescence (PL) is not completely understood. We compute the radiative recombination rate…
Atomic-scale disorder shapes the potential energy landscape traversed by photoexcited charge carriers, while the carriers themselves also dynamically reshape this landscape. However, resolving ultrafast photocarrier motion at atomic length…
We present a numerical implementation of the time-dependent surface flux (tSURFF) method [New J. Phys. 14, 013021 (2012)], an efficient computational scheme to extract photoelectron energy spectra, to the time-dependent multiconfiguration…
Determining the pulse duration of femtosecond electron bunches is challenging and often experimentally invasive. An effective method for measuring the duration based on the time-dependent variations in electron beam divergence induced by a…
We study light curves and the spectral broadening of the radiation emitted during the finite interval of time by a surface of a collapsing object. We study a simplified model of monochromatic radiations from a spherical surface which is…
A time-resolved spectroscopic protocol exploiting terahertz-assisted photoionization is proposed to reconstruct transient density matrix. Population and coherence elements are effectively mapped onto spectrally separated peaks in…
Time-resolved photoemission orbital tomography (tr-POT) offers unique possibilities for tracing molecular electron dynamics. The recorded pump-induced changes of the angle-resolved photoemission intensities allow to characterize unoccupied…
We perform a first study of time-dependent X-ray reflection in photo-ionized accretion disks. We assume a step-functional change in the X-ray flux and use a simplified prescription to describe the time evolution of the illuminated gas…
Visualizing the electron dynamics in four dimensions of space and time is crucial to the understanding of several ubiquitous processes in nature. Hence, ultrafast X-ray and electron imaging tools have been developed to probe the dynamics of…
Frontier orbitals, i.e., the highest occupied and lowest unoccupied orbitals of a molecule, generally determine molecular properties, such as chemical bonding and reactivities. Consequently, there has been a lot of interest in measuring…
Photonic time-crystals (PTCs) are spatially-homogeneous media whose electromagnetic (EM) susceptibility varies periodically in time, causing temporal reflections and refractions for any wave propagating within the medium. The time-reflected…
The quasi-symmetric shape of the lightcurves, as seen in the X-rays and in the optical, together with the fast variations of the flux observed, suggest that the cooling time for the highest energy electrons may be shorter than the light…
Photo-induced processes are fundamental in nature, but accurate simulations are seriously limited by the cost of the underlying quantum chemical calculations, hampering their application for long time scales. Here we introduce a method…
Time- and angle-resolved photoemission spectroscopy accesses the ultrafast evolution of quasiparticles and many-body interactions in solid-state systems. However, the momentum- and energy-resolved transient photoemission intensity may not…
Mass spectrometry is a widespread approach to work out what are the constituents of a material. Atoms and molecules are removed from the material and collected, and subsequently, a critical step is to infer their correct identities based…
Time-frequency (TF) analysis is a powerful tool for exploring ultrafast dynamics in atoms and molecules. While some TF methods have demonstrated their usefulness and potential in several of quantum systems, a systematic comparison among…
The electron dynamics in the unoccupied states of the Weyl semimetal PtBi$_2$ is studied by time- and angle-resolved photoemission spectroscopy (TR-ARPES). The measurement's result is the photoemission intensity $I$ as a function of at…
Optical Emission Spectroscopy is a widely used technique for plasma diagnosis, with particular interest in hydrogen atomic emission due to its prevalence in plasmas. However, accurately determining plasma parameters like electron density,…
We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…
Imaging the structure of molecules in transient excited states remains a challenge due to the extreme requirements for spatial and temporal resolution. Ultrafast electron diffraction from aligned molecules (UEDAM) provides atomic resolution…