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We investigated the effect of fluorine-terminated diamond surface on the charged state of shallow nitrogen vacancy defect centers (NVs). Fluorination is achieved with CF4 plasma and the surface chemistry is confirmed with x-ray…

Materials Science · Physics 2013-04-05 Shanying Cui , Evelyn L. Hu

Nitrogen-vacancy (NV) centers in diamond are extensively utilized as quantum sensors for imaging fields at the nanoscale. The ultra-high sensitivity of NV magnetometers has enabled the detection and spectroscopy of individual electron…

We investigate the effect of surface termination on the charge state of nitrogen vacancy centers, which have been ion-implanted few nanometers below the surface of diamond. We find that, when changing the surface termination from oxygen to…

Shallow nitrogen-vacancy (NV-) centers in diamond are among the most promising quantum sensors, offering high sensitivity and nanoscale spatial resolution. These systems are, however, prone to decoherence due to coupling with surface…

Materials Science · Physics 2025-05-19 Arsineh Apelian , Mariya Romanova , Vojtech Vlcek

The performance of nitrogen vacancy (NV$^{-}$) based magnetic sensors strongly depends on the stability of nitrogen vacancy centers near the diamond surface. The sensitivity of magnetic field detection is diminished as the NV$^{-}$ turns…

Mesoscale and Nanoscale Physics · Physics 2016-11-18 Arthur N. Newell , Dontray A. Dowdell , D. H. Santamore

We present a density functional theory analysis of the negatively charged nitrogen-vacancy (NV$^-$) defect complex in diamond located in the vicinity of (111)- or (100)-oriented surfaces with mixed (N,H)-terminations. We assess the…

Materials Science · Physics 2022-02-21 Wolfgang Körner , Reyhaneh Ghassemizadeh , Daniel F. Urban , Christian Elsässer

Although the spin properties of superficial shallow nitrogen-vacancy (NV) centers have been the subject of extensive scrutiny, considerably less attention has been devoted to studying the dynamics of NV charge conversion near the diamond…

Mesoscale and Nanoscale Physics · Physics 2018-07-03 Siddharth Dhomkar , Harishankar Jayakumar , Pablo R. Zangara , Carlos A. Meriles

The interaction of solid-state electronic spins with deformations of their host crystal is an important ingredient in many experiments realizing quantum information processing schemes. Here, we theoretically characterize that interaction…

Mesoscale and Nanoscale Physics · Physics 2018-08-08 Péter Udvarhelyi , Vladyslav O. Shkolnikov , Adam Gali , Guido Burkard , András Pályi

Nitrogen-Vacancy (NV) centers in diamond have been identified over the past few years as promising systems for a variety of applications, ranging from quantum information science to magnetic sensing. This relies on the unique optical and…

Quantum Physics · Physics 2018-12-19 I. Meirzada , Y. Hovav , S. A. Wolf , N. Bar-Gill

The nitrogen vacancy (NV) center in diamond exhibits spin-dependent fluorescence and long spin coherence times under ambient conditions, enabling applications in quantum information processing and sensing. NV centers near the surface can…

Nitrogen vacancy centers (NV) in proximity to diamond surfaces are promising nanoscale quantum sensors. However, their coherence properties are negatively affected by magnetic and electric surface noise, whose origin and detailed impact…

Quantum Physics · Physics 2025-12-12 Jonah Nagura , Mykyta Onizhuk , Giulia Galli

We show that electric field noise from surface charge fluctuations can be a significant source of spin decoherence for near-surface nitrogen-vacancy (NV) centers in diamond. This conclusion is based on the increase in spin coherence…

Mesoscale and Nanoscale Physics · Physics 2015-08-26 M. Kim , H. J. Mamin , M. H. Sherwood , K. Ohno , D. D. Awschalom , D. Rugar

Sensitive nanoscale magnetic resonance imaging (MRI) of target spins using nitrogen-vacancy (NV) centers in diamond will require a quantitative understanding of dominant noise at the surface. We probe this noise by applying dynamical…

Mesoscale and Nanoscale Physics · Physics 2014-07-11 Bryan A. Myers , Matthieu C. Dartiailh , Kenichi Ohno , Ananda Das , David D. Awschalom , Ania C. Bleszynski Jayich

Nitrogen-vacancy (NV) centers in diamond can be used for nanoscale sensing with atomic resolution and sensitivity; however, it has been observed that their properties degrade as they approach the diamond surface. Here we report that in…

The nitrogen-vacancy (NV) center in diamond enables optical initialization and readout of its electronic spin, forming the basis of a wide range of quantum sensing and metrology applications. A central challenge in such measurements is the…

Mesoscale and Nanoscale Physics · Physics 2026-04-16 Neil B. Manson , Morgan Hedges , Michael S. J. Barson , Carlos A. Meriles , Ronald Ulbricht , Marcus W. Doherty

Near-surface nitrogen-vacancy (NV) centers have been created in diamond through low energy implantation of 15N to sense electron spins that are external to the diamond. By performing double resonance experiments, we have verified the…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 H. J. Mamin , M. H. Sherwood , D. Rugar

We study the photo-physical stability of ensemble near-surface nitrogen vacancy (NV) centers in diamond under vacuum and air. The optically detected magnetic resonance contrast of the NV centers was measured following exposure to laser…

Scalable realizations of quantum network technologies utilizing the nitrogen vacancy center in diamond require creation of optically coherent NV centers in close proximity to a surface for coupling to optical structures. We create single NV…

Mesoscale and Nanoscale Physics · Physics 2021-09-01 Srivatsa Chakravarthi , Christian Pederson , Zeeshawn Kazi , Andrew Ivanov , Kai-Mei C. Fu

Nitrogen-vacancy centers in diamond are a promising platform for nanoscale nuclear magnetic resonance sensing. Despite significant progress towards using NV centers to detect and localize nuclear spins down to the single spin level,…

Fluorescent nanodiamonds (NDs) are crystal defect-based light-emitting nanoparticles that can be applied to quantum information science and quantum sensing. Of particular interest are nitrogen vacancy (NV) centers that allow optical access…

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