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On the basis of density functional theory (DFT) calculations thermoelectric properties are derived for Sb-doped skutterudites MPt$_4$Ge$_{12-x}$Sb$_x$ with M=Ba,La,Th. It is predicted that the originally very small absolute values of…

Materials Science · Physics 2012-07-06 M. X. Chen , R. Podloucky , S. Humer , E. Bauer , P. Rogl

The conventional understanding that a bandstructure that produces a Dirac delta function transport distribution (or transmission in the Landauer framework) maximizes the thermoelectric figure of merit, ZT, is revisited. Thermoelectric (TE)…

Materials Science · Physics 2015-05-27 Changwook Jeong , Raseong Kim , Mark Lundstrom

In this work, we have proposed a data-driven screening framework combining the interpretable machine learning with high-throughput calculations to identify a series of metal oxides that exhibit both high-temperature tolerance and high power…

Materials Science · Physics 2024-05-01 Shengluo Ma , Yongchao Rao , Xiang Huang , Shenghong Ju

Thermoelectric properties of two-dimensional (2D) Dirac materials are calculated within linearized Boltzmann transport theory and relaxation time approximation. We find that the gapless 2D Dirac material exhibits poorer thermoelectric…

Mesoscale and Nanoscale Physics · Physics 2019-09-04 Eddwi H. Hasdeo , Lukas P. A. Krisna , Muhammad Y. Hanna , Bobby E. Gunara , Nguyen T. Hung , Ahmad. R. T. Nugraha

We derive a thermoelectric inequality in thermoelectric conversion between the material figure of merit (ZT) and the module effective ZT using the Constant Seebeck-coefficient Approximation combining with the Wiedemann-Franz law. In a P-N…

Low band gap thermoelectric materials suffer from bipolar effects at high temperatures, with increased electronic thermal conductivity and reduced Seebeck coefficient, leading to reduced power factor and low ZT figure of merit. In this work…

Materials Science · Physics 2022-03-14 Patrizio Graziosi , Zhen Li , Neophytos Neophytou

We report a strategy based on introduction of point defects for improving the thermoelectric properties of FeSb2, a promising candidate for low temperature applications. Introduction of Sb deficiency to the tune of 20% leads to enhancement…

Materials Science · Physics 2015-05-01 Anup V. Sanchela , Ajay D. Thakur , C. V. Tomy

Systemic optimization of thermoelectric materials is arduous due to their conflicting electrical and thermal properties. A strategy based on Design of Experiments and machine learning is developed to optimize the thermoelectric efficiency…

Directed Energy Deposition (DED) offers significant potential for manufacturing complex and multi-material parts. However, internal defects such as porosity and cracks can compromise mechanical properties and overall performance. This study…

Computer Vision and Pattern Recognition · Computer Science 2025-02-12 Israt Zarin Era , Fan Zhou , Ahmed Shoyeb Raihan , Imtiaz Ahmed , Alan Abul-Haj , James Craig , Srinjoy Das , Zhichao Liu

Whether porosity can effectively improve thermoelectric performance is still an open question. Herein we report that thermoelectric performance can be significantly enhanced by creating porosity in n-type Mg3.225Mn0.025Sb1.5Bi0.49Te0.01,…

Thermoelectric materials offer a promising pathway to directly convert waste heat to electricity. However, achieving high performance remains challenging due to intrinsic trade-offs between electrical conductivity, the Seebeck coefficient,…

Conventional metals, insulators, and semimetals are constrained by fundamental limitations in terms of their thermoelectric performance. Topological materials offer certain features that allow them to circumvent these constraints, and…

Materials Science · Physics 2026-03-26 Brian Skinner , Poulomi Chakraborty , Joshua Scales , Joseph P. Heremans

Thermoelectric (TE) materials are among very few sustainable yet feasible energy solutions of present time. This huge promise of energy harvesting is contingent on identifying/designing materials having higher efficiency than presently…

Over the last two decades a plethora of new thermoelectric materials, their alloys, and their nanostructures were synthesized. The ZT figure of merit, which quantifies the thermoelectric efficiency of these materials increased from values…

Materials Science · Physics 2023-07-27 Neophytos Neophytou , Pankaj Priyadarshi , Zhen Li , Patrizio Graziosi

This work builds on the previous introduction [1] of a coupled experimental-computational system devised to fully characterize the thermal behavior of complex 3D submicron electronic devices. The new system replaces the laser-based surface…

Materials Science · Physics 2007-09-13 Peter E. Raad , Pavel L. Komarov , M. Burzo

The thermoelectric properties of a semiconduct quantum dot chain (SQDC) connected to metallic electrodes are theoretically investigated in the Coulomb blockade regime. An extended Hubbard model is employed to simulate the SQDC system…

Mesoscale and Nanoscale Physics · Physics 2013-01-11 David M. -T. Kuo , Yia-Chung Chang

We have investigated the effect of Sb-deficiency on the thermoelectric figure of merit (zT) of Zn4Sb3 prepared by solid state reaction route. At high temperatures, the Seebeck coefficient (S) and electrical conductivity ({\sigma}) increase…

Materials Science · Physics 2015-05-06 Anup V. Sanchela , Ajay D. Thakur , C. V. Tomy

We report the machine learning (ML)-based approach allowing thermoelectric generator (TEG) efficiency evaluation directly from 5 parameters: 2 physical properties - carriers density and energy gap, and 3 engineering parameters - external…

Materials Science · Physics 2024-08-23 Anastasiia Tukmakova , Patrizio Graziosi

We explore the possibility to perform an in-situ transmission electron microscopy (TEM) thermoelectric characterization of materials. A differential heating element on a custom in-situ TEM microchip allows to generate a temperature gradient…

Materials Science · Physics 2025-01-14 Simon Hettler , Mohammad Furqan , Andres Sotelo , Raul Arenal

We performed the first-principles calculation on common thermoelectric semiconductors $\rm Bi_2Te_3$, $\rm Bi_2Se_3$, $\rm SiGe$, and $\rm PbTe$ in bulk three-dimension (3D) and two-dimension (2D). We found that miniaturization of materials…

Materials Science · Physics 2020-11-13 Kevin Octavian , Eddwi H. Hasdeo