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An ab initio study of magnetic exchange interactions in antiferromagnetic and strongly correlated 3d transition metal monoxides is presented. Their electronic structure is calculated using the local self-interaction correction approach,…

For accurate first-principles computations of exchange coupling constants $J_{ij}$ by the Liechtenstein method with localized basis sets, we developed a scheme using the single-site orthogonalization (SO). In contrast to the non-orthogonal…

Materials Science · Physics 2020-05-21 Asako Terasawa , Sonju Kou , Taisuke Ozaki , Yoshihiro Gohda

Theoretical prediction of the 2nd-order magnetic transition temperature (TM) used to be arduous. Here, we develop a first principle-based, fully automatic structure-to-TM method for two-dimensional (2D) magnets whose effective Hamiltonians…

Materials Science · Physics 2023-12-08 Haichang Lu , Tai Yang , Zhimei Sun , John Robertson , Weisheng Zhao

The structural transitions, magnetic properties, and electronic structures of Co(Fe)-doped MnNiSi compounds are investigated by x-ray powder diffraction (XRD), differential scanning calorimetry (DSC), magnetic measurements, and…

Materials Science · Physics 2015-04-17 Y. Li , Z. Y. Wei , E. K. Liu , G. D. Liu , S. G. Wang , W. H. Wang , G. H. Wu

We present a first-principles method based on density functional theory and many-body perturbation theory for computing spin excitations in magnetic systems with noncollinear spin textures. Traditionally, the study of magnetic excitations…

Materials Science · Physics 2025-10-21 Hsiao-Yi Chen , Ryotaro Arita , Yusuke Nomura

We have developed a fully microscopic theory of magnetic properties of the prototype molecular magnet Mn12. First, the intra-molecular magnetic properties have been studied by means of first-principles density functional-based methods, with…

Strongly Correlated Electrons · Physics 2015-06-19 V. V. Mazurenko , Y. O. Kvashnin , Fengping Jin , H. A. De Raedt , A. I. Lichtenstein , M. I. Katsnelson

We demonstrate that the magnetic nanoskyrmion lattice on the Fe monolayer on Ir(111) and the positions of the Fe atoms can be resolved simultaneously using magnetic exchange force microscopy. Thus, the relation between magnetic and atomic…

Materials Science · Physics 2017-08-18 Josef Grenz , Arne Köhler , Alexander Schwarz , Roland Wiesendanger

Despite its great technological importance, the magnetoelectric (ME) couplings in \BF are barely understood. By using a first-principles approach, we uncover the {\it dynamic} ME couplings of the long-range spin-cycloid in BiFeO$_3$. Based…

Strongly Correlated Electrons · Physics 2016-04-01 Jun Hee Lee , Istvan Kézsmáki , Randy S. Fishman

We propose a dynamical mean field approach for calculating the electronic structure of strongly correlated materials from first principles. The scheme combines the GW method with dynamical mean field theory, which enables one to treat…

Strongly Correlated Electrons · Physics 2009-11-07 S. Biermann , F. Aryasetiawan , A. Georges

In this concept paper, the development of strategies for the integration of first-principles methods with crystallographic database mining for the discovery and design of novel ferroelectric materials is discussed, drawing on the results…

Materials Science · Physics 2012-10-24 Joseph W. Bennett , Karin M. Rabe

Given the scarcity of experimentally confirmed magnetic structures, the reliable prediction of magnetic ground states is crucial; however, it remains a long-sought challenge because of the complex magnetic potential energy landscape. Here,…

Materials Science · Physics 2025-12-29 Yuhui Li , Sike Zeng , Xiaobing Chen , Renzheng Xiong , Yutong Yu , Yu-Jun Zhao , Qihang Liu

We present results of a density functional theory study of MnO in the wurtzite structure. Our motivation is provided by recent experiments reporting ferromagnetism in Mn-doped wurtzite structure ZnO. We find that wurtzite MnO a) is not…

Materials Science · Physics 2009-11-10 Priya Gopal , Nicola Spaldin , Umesh. V. Waghmare

We introduce a general first-principles methodology for computing electronic structure in a finite uniform magnetic field which allows for an arbitrary rational magnetic flux and nonlocal pseudopotentials, at a comparable time complexity of…

Materials Science · Physics 2025-10-07 Chengye Lü , Yingwei Chen , Yuzhi Wang , Zhihao Dai , Zhong Fang , Xin-Gao Gong , Quansheng Wu , Hongjun Xiang

A recently developed dynamical mean-field theory in the iterated perturbation theory approximation was used as a basis for construction of the "first principles" calculation scheme for investigating electronic structure of strongly…

Strongly Correlated Electrons · Physics 2009-10-30 V. I. Anisimov , A. I. Poteryaev , M. A. Korotin , A. O. Anokhin , G. Kotliar

We study the behavior of the magnetization and the magnetic susceptibility of molecular magnets with complex bridging structure. Our computations are based on a post-Hartree-Fock method accounting for the intricate network of interatomic…

Strongly Correlated Electrons · Physics 2020-03-30 M. Georgiev , H. Chamati

Magnetic materials are typically described in terms of the Heisenberg model, which provides an accurate account of thermodynamic properties when combined with first principles calculations. This approach is usually based on an energy…

Materials Science · Physics 2020-12-04 Daniele Torelli , Thomas Olsen

Materials that combine magnetic and ferroelectric properties have generated increasing interest over the last few years, due to both their diverse properties and their potential utility in new types of magnetoelectric device applications.…

Materials Science · Physics 2014-11-17 Claude Ederer , Nicola A. Spaldin

The recent development in the field of 2D magnetic materials urges reliable theoretical methodology for determination of magnetic properties. Among the available methods, ab initio four-state energy mapping based on Density Functional…

Mesoscale and Nanoscale Physics · Physics 2020-08-05 Denis Sabani , Cihan Bacaksiz , Milorad Milosevic

We investigated the reliability and applicability of so-called magnetic force linear response method to calculate spin-spin interaction strengths from first-principles. We examined the dependence on the numerical parameters including the…

Strongly Correlated Electrons · Physics 2018-03-28 Hongkee Yoon , Taek Jung Kim , Jae-Hoon Sim , Seung Woo Jang , Taisuke Ozaki , Myung Joon Han

The magnetic properties of Nd${}_2$Fe${}_{14}$B (NFB)/transition metal (TM = Fe, Co) multilayer systems are studied on the basis of first-principles density functional calculations. We optimize the model structure under a variety of…

Mesoscale and Nanoscale Physics · Physics 2016-01-13 Nobuyuki Umetsu , Yuta Toga , Akimassa Sakuma