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Raman spectroscopy is a label-free, chemically specific optical technique which provides detailed information about the chemical composition and structure of the excited analyte. Because of this, there is growing research interest in…

Raman spectroscopy is a very powerful probe to study the nature of quasi-particle excitations in condensed matter physics. The work presented in this thesis is focused on two different families of novel materials, namely the iron-based…

Materials Science · Physics 2015-01-19 Pradeep Kumar

We employed femtosecond pump probe technique to investigate the dynamics of coherent optical phonons in iron garnet. A phenomenological symmetry-based consideration reveals that oscillations of the terahertz T2g mode are excited. Selective…

Surface Enhanced Raman Spectroscopy (SERS) is a well-established technique for enhancing Raman signals. Recently photonic integrated circuits have been used, as an alternative to microscopy based excitation and collection, to probe SERS…

Two-dimensional (2D) graphene and graphene-related materials (GRMs) show great promise for future electronic devices. Nevertheless, GRMs result distinct properties under the influence of the substrate that serves as support through uneven…

Knowing the band structure of materials is one of the prerequisites to understand their properties. Therefore, especially in the last decades, angle-resolved photoemission spectroscopy (ARPES) has become a highly demanded experimental tool…

Materials Science · Physics 2017-10-17 A. M. Shuvaev , V. Dziom , N. N. Mikhailov , Z. D. Kvon , Y. Shao , D. N. Basov , A. Pimenov

Attenuated total reflection (ATR) by surface plasmon polariton (SPP) is a method for evaluating the dispersion relation of SPP from the position of a dip in the reflection spectrum. However, recent studies have shown that the dips are…

Micro-Raman spectroscopy has become an important tool in probing thermophysical behavior in emerging functional materials such as two-dimensional (2D) layered structures. Localized heating by the focused Raman excitation laser beam is…

Mesoscale and Nanoscale Physics · Physics 2022-11-10 Peter Sokalski , Zherui Han , Gabriella Coloyan Fleming , Brandon Smith , Sean E. Sullivan , Rui Huang , Xiulin Ruan , Li Shi

The dichroism and birefringence effects in stumulated Raman scattering (SRS) in polyatomic molecules were studied theoretically. General expressions have been derived describing the change of the intensity and polarization of the probe…

Chemical Physics · Physics 2023-11-07 Bogdan V. Semak , Yaroslav M. Beltukov , Oleg S. Vasyutinskii

Raman spectroscopy is widely used to assess the quality of 2D materials thin films. This report focuses on $\rm{PtSe_2}$, a noble transition metal dichalcogenide which has the remarkable property to transit from a semi-conductor to a…

Angle-resolved photoemission spectroscopy (ARPES) is one of the most direct methods of studying the electronic structure of solids. By measuring the kinetic energy and angular distribution of the electrons photoemitted from a sample…

Strongly Correlated Electrons · Physics 2009-11-10 Andrea Damascelli

Coherent Raman scattering techniques as coherent anti-Stokes Raman scattering (CARS), offer significant advantages in terms of pixel dwell times and speed as compared to spontaneous Raman scattering for investigations of crystalline…

A new numerical method is introduced for calculating the polarizability of an arbitrary dielectric object with position dependent complex permittivity. Three separate numerical approaches are provided to calculate the dipole moment of a…

Materials Science · Physics 2022-03-18 Daniel B. Murray , Caleb H. Netting , Robin D. Mercer , Lucien Saviot

Resonance Raman scattering, a very effective and sensitive technique for atomically thin semiconducting transition metal dichalcogenide, can be used to observe the phonons from the entire Brillouin zone. In addition to the significance of…

Materials Science · Physics 2023-02-06 Deepu Kumar , Nasaru Khan , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

We report the first investigation on continuous-wave Raman lasing in high-quality-factor aluminum nitride (AlN) microring resonators. Although wurtzite AlN is known to exhibit six Raman-active phonons, single-mode Raman lasing with low…

We demonstrate low-frequency interferometric impulsive stimulated Raman scattering (ISRS) imaging with high robustness to distortions by optical scattering. ISRS is a pump-probe coherent Raman spectroscopy that can capture Raman vibrational…

We review recent development in Raman techniques and diamond anvil cell technology, that allow measurements of Raman of metals in the megabar pressure range. The Raman technique includes holographic transmission optics and single-stage…

Phonon-phonon anharmonic effects have a strong influence on the phonon spectrum; most prominent manifestation of these effects are the softening (shift in frequency) and broadening (change in FWHM) of the phonon modes at finite temperature.…

We discuss the effect of the local field polarization in metallic nanostructures where large field enhancements can be induced by excitation of localized surface plasmons. To demonstrate the importance of these effects, we study a few model…

Chemical Physics · Physics 2007-05-23 E. C. Le Ru , P. G. Etchegoin

Resonance ultrasound spectroscopy (RUS) is a non-destructive technique for evaluating elastic and an-elastic material properties. The frequencies of free vibrations for a carefully crafted sample are measured, and material properties can be…

Materials Science · Physics 2021-08-11 Christopher L Sevigney , Onome E. Scott-Emuakpor , Farhad Farzbod
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