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Using the evolutionary algorithm USPEX and DFT+U calculations, we predicted a high-symmetry geometric structure of bare Ti8O12 cluster composed of 8 Ti atoms forming a cube, which O atoms are at midpoints of all of its edges, in excellent…

Atomic and Molecular Clusters · Physics 2015-12-09 Xiaohu Yu , Artem R. Oganov , Guangrui Qian , Ivan A. Popov , Alexander I. Boldyrev

The preference for the occupation of solute atoms like B, C, N, and O at various sites in iron is generally explained by the size of the solute and the volume available for the solute atoms to occupy. Such an explanation based on the size…

Magnetism in bare uncapped gold nano-clusters is explored from a density functional theory perspective with scalar relativistic effects included via the pseudo-potential. The computed electronic structures of various nano-clusters reveal…

Materials Science · Physics 2007-05-23 R. J. Magyar , V. Mujica , M. Marquez , C. Gonzalez

Large electron-electron Coulomb-interactions in correlated systems can lead to a periodic arrangement of localized electrons, the so called "charge-order". The latter is here proposed as a driving force behind ferroelectricity in iron…

Materials Science · Physics 2015-05-14 Kunihiko Yamauchi , Silvia Picozzi

Structure and electronic properties of two unusual boron clusters obtained by fusion of borozene rings has been studied by means of first principles calculations, based on the generalized-gradient approximation of the density functional…

Materials Science · Physics 2015-05-13 G. Forte , A. La Magna , I. Deretzis , R. Pucci

We have used density functional perturbation theory to investigate the stiffness of interatomic bonds in small clusters of Si, Sn and Pb. As the number of atoms in a cluster is decreased, there is a marked shortening and stiffening of…

Other Condensed Matter · Physics 2007-05-23 Raghani Pushpa , Umesh Waghmare , Shobhana Narasimhan

This study investigates the photocatalytic nitrogen fixation on a cation-doped surface (Bi$_{x}$M$_{y}$)$_2$MoO$_6$ where (M = Fe, La, Yb) in both the orthorhombic and monoclinic configurations using a density functional theory (DFT)…

Materials Science · Physics 2018-12-13 Alhassan S. Yasin , Botong Liu , Nianqiang Wu , Terence Musho

We present a Density Functional Theory (DFT) study of the structural and electronic properties of bare rutile VO$_{2}$(110) surfaces and its oxygen-rich terminations. We discuss the performance of various DFT functionals, including PBE,…

Materials Science · Physics 2021-08-31 Jakub Planer , Florian Mittendorfer , Josef Redinger

Distortions of the oxygen octahedra influence the fundamental electronic structure of perovskite oxides, such as their bandwidth and exchange interactions. Utilizing a fully ab-initio methodology based on density functional theory plus…

Strongly Correlated Electrons · Physics 2021-07-02 Alexander Hampel , Jeremy Lee-Hand , Antoine Georges , Cyrus E. Dreyer

Two (so-called left and right) variants of N-centered ensemble density-functional theory (DFT) [Senjean and Fromager, Phys. Rev. A 98, 022513 (2018)] are presented. Unlike the original formulation of the theory, these variants allow for the…

Strongly Correlated Electrons · Physics 2020-02-25 Bruno Senjean , Emmanuel Fromager

First principles based DFT calculations performed to insight structural and electronic properties of Boron doped Magnesium atom decorated graphene sheet for application of hydrogen storage. The four H2 molecules stably binds magnesium atom…

Materials Science · Physics 2020-03-31 Baliram Lone

Boron-doped diamond (BDD) has attracted much attentions in semi-/super-conductor physics and electrochemistry, where the surface structures play crucial roles. Herein, we systematically re-examined the probable surface reconstructions of…

Materials Science · Physics 2020-10-30 Le The Anh , Shota Iizuka , Yasuaki Einaga , Celine Catalan , Yousoo Kim , Yoshitaka Tateyama

Based on density functional theory the noncentrosymmetric superconductor Mo_3Al_2C in its well established {\beta}-Mn type ($P4_{1}32$) crystal structure is investigated. In particular, its thermodynamical and dynamical stabilities are…

Materials Science · Physics 2013-05-30 D. Reith , C. Blaas-Schenner , R. Podloucky

We study the effects of electron-electron interactions and hole doping on the electronic structure of Cu-doped NaFeAs using the density functional theory plus dynamical mean-field theory (DFT+DMFT) method. In particular, we employ an…

Strongly Correlated Electrons · Physics 2021-04-14 S. L. Skornyakov , V. I. Anisimov , I. Leonov

Atomically precise thiolate-stabilized gold nanoclusters are currently of interest for many cross-disciplinary applications in chemistry, physics and molecular biology. Very recently, synthesis and electronic properties of "nanoalloy"…

Atomic and Molecular Clusters · Physics 2011-09-05 Sami Malola , Hannu Häkkinen

Low-energy deposition of neutral Pd_N clusters (N=2-7 and 13) on a MgO(001) surface F-center (FC) was studied by spin-density-functional molecular dynamics simulations. The incident clusters are steered by an attractive "funnel" created by…

Materials Science · Physics 2009-11-07 M. Moseler , H. Hakkinen , U. Landman

We derive an exact representation of the exchange-correlation energy within density functional theory (DFT) which spawns a class of approximations leading to correct long-range asymptotic behavior. In what amounts to be the simplest…

Materials Science · Physics 2009-11-10 Roi Baer , Daniel Neuhauser

The atomic and magnetic structures of (Cu$X$)LaNb$_2$O$_7$ ($X$=Cl and Br) are investigated using the density-functional calculations. Among several dozens of examined structures, an orthorhombic distorted $2\times 2$ structure, in which…

Strongly Correlated Electrons · Physics 2015-05-14 Chung-Yuan Ren , Ching Cheng

We perform first-principles quantum mechanical studies of dioxygen ligand binding to the hemocyanin protein. Electronic correlation effects in the functional site of hemocyanin are investigated using a state-of-the-art approach, treating…

Strongly Correlated Electrons · Physics 2019-09-23 Mohamed Ali al-Badri , Edward Linscott , Antoine Georges , Daniel J. Cole , Cédric Weber

We present a cluster-based density-functional approach to model charge transport through molecular and atomic contacts. The electronic structure of the contacts is determined in the framework of density functional theory, and the parameters…

Mesoscale and Nanoscale Physics · Physics 2008-12-04 F. Pauly , J. K. Viljas , U. Huniar , M. Hafner , S. Wohlthat , M. Burkle , J. C. Cuevas , G. Schon
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