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This paper describes a new photoelectron emission lifetime detection system. It is based on a recently developed Radio Frequency Timing technique of keV electrons and a 40 MHz, ultrafast pulsed laser. The photoelectron emission lifetimes…

The energy dependence of the relaxation rate of hot electrons due to interaction with the Fermi sea is studied. We consider 2D and 3D systems, quasi-1D quantum wires with multiple transverse bands, as well as single-channel 1D wires. Our…

Mesoscale and Nanoscale Physics · Physics 2018-05-29 M. Bard , I. V. Protopopov , A. D. Mirlin

We simulate from first-principles the energetic, structural, and electronic properties of ferroelectric domains in ultrathin capacitors made of a few unit cells of BaTiO$_3$ between two metallic SrRuO$_3$ electrodes in short circuit. The…

Materials Science · Physics 2007-10-09 Pablo Aguado-Puente , Javier Junquera

The electron-phonon interaction in thin Ag-nanofilms epitaxially grown on Cu(111) is investigated by temperature-dependent and angle-resolved photoemission from silver quantum-well states. Clear oscillations in the electron-phonon coupling…

Other Condensed Matter · Physics 2009-11-11 S. Mathias , M. Wiesenmayer , M. Aeschlimann , M. Bauer

The transient response of Ba(Fe(1-x)Co(x))2As2, x=0.08 was studied by pump-probe optical reflectivity. After ultrafast photoexcitation, hot electrons were found to relax with two different characteristic times, indicating the presence of…

Femtosecond (fs)-resolved photoemission electron micrographs of single and few-layer MoSe$_2$ track exciton dynamics in this model 2D quantum material system with joint nanometer (nm)-fs resolution. We illustrate the latter using two-photon…

Chemical Physics · Physics 2021-09-27 Paul M. Sass , Patrick Z. El-Khoury

We have performed an angle-resolved photoemission study of the electron-doped high-Tc superconductors (HTSCs) Sm_{1.85}Ce_{0.15}CuO_{4} (SCCO) and Eu_{1.85}Ce_{0.15}CuO_{4} (ECCO). Around the nodal point (pi/2, pi/2), we observed an energy…

Superconductivity · Physics 2007-11-14 M. Ikeda , T. Yoshida , A. Fujimori , M. Kubota , K. Ono , K. Unozawa , T. Sasagawa , H. Takagi

In thin film ferroelectric capacitor the chemical and electronic structure of the electrode/FE interface can play a crucial role in determining the kinetics of polarization switching. We investigate the electronic structure of a…

We present measurements of the magnetoresistance of long and narrow quasi one-dimensional gold wires containing magnetic iron impurities. The electron phase coherence time extracted from the weak antilocalisation shows a pronounced plateau…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 F. Schopfer , C. Bäuerle , W. Rabaud , L. Saminadayar

Understanding the microscopic spatio-temporal dynamics of nonequilibrium charge carriers in heterosystems promises optimization of process and device design towards desired energy transfer. Hot electron transport is governed by scattering…

We have studied the possibly half metallic Co2FeSi full Heusler alloy by means of spin- and time-resolved photoemission spectroscopy. For excitation, the second and fourth harmonic of femtosecond Ti:sapphire lasers were used, with photon…

Materials Science · Physics 2016-08-16 J. -P. Wüstenberg , M. Cinchetti , M. Sánchez Albaneda , M. Bauer , M. Aeschlimann

We study the ferroelectric stability and surface structural properties of an oxygen-terminated hexagonal YMnO$_3$ ultra-thin film using density functional theory. Under an open circuit boundary condition, the ferroelectric state with the…

Materials Science · Physics 2009-04-14 Na Sai , Craig J. Fennie , Alexander A. Demkov

Electrons mediate many of the interactions between atoms in a solid. Their propagation in a material determines its thermal, electrical, optical, magnetic and transport properties. Therefore, the constant energy contours characterizing the…

Electrons photoemitted by extreme ultraviolet attosecond pulses derive spatially from the first few atomic surface layers and energetically from the valence band and highest atomic orbitals. As a result, it is possible to probe the emission…

In the paper we consider size effects of phase transitions and polar properties of the thin antiferroelectric films. We modified phenomenological approach proposed by Kittel. The Euler-Lagrange equations were solved by direct variational…

Materials Science · Physics 2007-05-23 E. A. Eliseev , M. D. Glinchuk , A. N. Morozovska

Hafnium oxide (HfO2), particularly at low-dimensional scales, exhibits extensive promising applications in ultrahigh density devices like low-power logic and non-volatile memory devices due to its compatibility with current semiconductor…

We study dynamics of incoherent exciton formation under interband photoexcitation in Cu$_2$O using time-and angle-resolved photoemission spectroscopy at 90 K. Hot electrons injected by allowed optical transitions with 3.40-eV photons show…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 H. Tanimura , K. Tanimura , P. H. M. van Loosdrecht

We use ultrafast x-ray diffraction to study non-equilibrium pathways of the phase transition in FeRh parametrized by the structural response. By increasing the pump-pulse duration beyond the electron-phonon coupling time, we suppress the…

Rare earth permanent magnets (REPMs) with both localized moments and itinerant conduction bands are not only important for fundamental research but also have significant technological applications. In particular, Sm$_{\rm 2}$Co$_{\rm 17}$…