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In charged water microdroplets, which occur in nature or in the lab upon ultrasonication or in electrospray processes, the thermodynamics for reactive chemistry can be dramatically altered relative to the bulk phase. Here, we provide a…

Chemical Physics · Physics 2024-05-06 Joseph P. Heindel , R. Allen LaCour , Teresa Head-Gordon

We use photo-electrons as a non-contact probe to measure local electrical potentials in a solid-oxide electrochemical cell. We characterize the cell in operando at near-ambient pressure using spatially-resolved X-ray photoemission…

X-ray diffraction pattern and Raman spectrum authenticate the monoclinic P21/n structure of polycrystalline Pr$_2$ZnMnO$_6$ (PZM) synthesized by the solid-state reaction technique. The X-ray photoemission spectrum suggests the existence of…

Materials Science · Physics 2023-07-04 Moumin Rudra , H. S. Tripathi , Alo Dutta , T. P. Sinha

Molecular hydrogen (H$_2$) production by electrochemical hydrogen evolution reaction (HER) is being actively explored for non-precious-metal based electrocatalysts that are earth-abundant and low cost like MoS$_2$. Although it is…

Materials Science · Physics 2022-08-18 Arunima Singh , Preeti Bhumla , Manjari Jain , Saswata Bhattacharya

We prepared Na$_x$TO$_2$ (T = Mn, Co) nanostructures to use as cathode material in Na-ion batteries. The Rietveld refinement of x-ray diffraction data confirms the hexagonal symmetry. Scanning and transmission electron microscopy…

Materials Science · Physics 2018-06-06 Mahesh Chandra , Rishabh Shukla , Muhammad Rashid , Amit Gupta , Suddhasatwa Basu , R. S. Dhaka

In this study, we employ first-principles density functional theory (DFT) calculations to investigate the electrochemical properties of Nb2C and Nb2CO2 MXenes as potential anode materials for sodium-ion (SIBs) and lithium-ion batteries…

Materials Science · Physics 2025-04-15 Nishat Sultana , Abdullah A. Amin , Eric J. Payton , Woo Kyun Kim

Metal oxide nanostructures are widely used in energy applications like super capacitors and Li-on battery. Smaller size nanocrystals show better stability, low ion diffusion time, higher-ion flux and low pulverization than bigger size…

Materials Science · Physics 2016-05-12 V. Bonu , B. Gupta , S. Chandra , A Das , S. Dhara , A. K. Tyagi

Solute-intercalation-induced phase separation creates spatial heterogeneities in host materials, a phenomenon ubiquitous in batteries, hydrogen storage, and other energy devices. Despite many efforts, probing intercalation processes at the…

We evaluated for the first time the use of nanostructured layered perovskites of formulae LnBaCo2O6-d with Ln = Sm and Gd (SBCO and GBCO, respetively) as SOFC cathodes, finding promising electrochemical properties in the intermediate…

Materials Science · Physics 2017-04-26 Augusto E. Mejía Gómez , Diego G. Lamas , Ana Gabriela Leyva , Joaquín Sacanell

Recent reports on the formation of hydrogen peroxide (H$_2$O$_2$) in water microdroplets produced via pneumatic spraying or capillary condensation have garnered significant attention. How covalent bonds in water could break under such…

A simple one-pot hydrothermal synthesis of single crystalline beta-MnO2 nanorods with diameters in the range of 10-40nm is reported. During the synthesis process, the acid molarities were varied from 1.1M down to 0.2M in steps of 0.3M while…

Mesoscale and Nanoscale Physics · Physics 2018-09-12 Niraj Kumar , P. Dineshkumar , R. Rameshbabu , Arijit Sen

Supercapacitors or ultracapacitors are promising for efficient energy storage applications, owing to their high power density, high charge-discharge rates, and long cycle life performance. To achieve this goal, a large specific surface…

Materials Science · Physics 2019-10-10 Qingqing Ke , Cao Guan , Xiao Zhang , Minrui Zheng , Yong-Wei Zhang , Yongqing Cai , Hua Zhang , John Wang

Possible candidates for the Mg2B3Ox nanostructures observed in bulk of polycrystalline MgB2 (Ref.1) have been studied using a combination of Z-contrast imaging, electron energy loss spectroscopy (EELS) and first-principles calculations. The…

Superconductivity · Physics 2009-11-10 Juan C. Idrobo , Serdar Ogut , Taner Yildirim , Robert F. Klie , Nigel D. Browning

A comprehensive comparison between Bi$_{25}$FeO$_{40}$-reduced graphene oxide(rGO) nanocomposite and BiFeO$_{3}$-rGO nanocomposite has been performed to investigate their photocatalytic abilities in degradation of Rhodamine B dye and…

Materials Science · Physics 2022-02-08 M. A. Basith , Ragib Ahsan , Ishrat Zarin , M. A. Jalil

We report the synthesis of MnO2−delta microspheres using hydrothermal and conventional chemical reaction methods. The microspheres of MnO2−delta consist of nanowires having a diameter of 20-50 nm and a length of 2-8 micro m. The…

Materials Science · Physics 2009-11-10 J. B. Yang , X. D. Zhou , W. J. James , S. K. Malik , C. S. Wang

Monolayer films of transition metal dichalcogenides (in particular, MoS2, MoSe2, WS2, and WSe2) can be considered as ideal systems for the studies of high-temperature electron-hole liquids. The quasi-two-dimensional nature of electrons and…

Mesoscale and Nanoscale Physics · Physics 2020-05-12 P. L. Pekh , P. V. Ratnikov , A. P. Silin

Electrolysis has been performed on a fused mixture of magnesium chloride, potassium chloride, and magnesium borate at 600 oC under an Ar atmosphere using a graphite anode and a Pt cathode. Magnetic measurements and X-ray diffractometry have…

Superconductivity · Physics 2007-05-23 Hideki Abe , Kenji Yoshii

Due to the severe self-interaction errors associated with some density functional approximations, conventional density functionals often fail to dissociate the hemibonded structure of water dimer radical cation (H2O)2+ into the correct…

Chemical Physics · Physics 2017-08-23 Piin-Ruey Pan , You-Sheng Lin , Ming-Kang Tsai , Jer-Lai Kuo , Jeng-Da Chai

Here we develop a class off face centred cubic structure of metallic silver nanocrystals, to enable high ORR activity process. Silver nanoparticles deposited within different carbon supports: carboxylated-graphene, SiO2-doted reduced-…

This study investigates the lithium conversion behavior of a hydrogen storage material based on vanadium oxide added magnesium hydride. To understand the chemical interaction between vanadium oxide and magnesium hydride, detailed X ray…

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