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Intercalation is a robust method for tuning the physical properties of a vast number of van der Waals (vdW) materials. However, the prospects of using intercalation to modify magnetism in vdWs systems and the associated mechanisms have not…

We report results of magnetization and ac susceptibility measurements down to very low fields on a single crystal of the perovskite manganite, La$_{0.82}$Ca$_{0.18}$MnO$_3$. This composition falls in the intriguing ferromagnetic insulator…

Strongly Correlated Electrons · Physics 2014-03-17 P. Anil Kumar , R. Mathieu , P. Nordblad , Sugata Ray , Olof Karis , Gabriella Andersson , D. D. Sarma

Phase coexistence phenomena have been intensively studied in strongly correlated materials where several ordered states simultaneously occur or compete. Material properties critically depend on external parameters and boundary conditions,…

We report the mechanisms of atomic ordering in Fe$_{1-x}$Pt$_{x}$ alloys using density functional theory (DFT) and machine-learning interatomic potential Monte Carlo (MLIP-MC) simulations. We clarified that the formation enthalpy of the…

Fe$_3$GeTe$_2$ is a prototypical metallic van der Waals ferromagnet with itinerant magnetism and a highly tunable Curie temperature, yet how electronic excitations couple to spin and lattice degrees of freedom across its magnetic transition…

The structural and magnetic properties of two mixed-valence cobaltites with formal population of 0.30 Co$^{4+}$ ions per f.u., (Pr$_{1-y}$Y$_{y}$)$_{0.7}$Ca$_{0.3}$CoO$_3$ ($y=0$ and 0.15), have been studied down to very low temperatures by…

Materials Science · Physics 2015-06-17 K. Knizek , J. Hejtmanek , M. Marysko , P. Novak , E. Santava , Z. Jirak , T. Naito , H. Fujishiro , C. R. dela Cruz

The cobalt-intercalated transition metal dichalcogenide Co$_x$TaS$_2$ hosts a rich landscape of magnetic phases that depend sensitively on $x$. While the stoichiometric compound with $x=1/3$ exhibits a single magnetic transition, samples…

Strongly Correlated Electrons · Physics 2025-07-18 Jonathon Kruppe , Josue Rodriguez , Catherine Xu , James Analytis , Joseph Orenstein , Veronika Sunko

We have studied the magnetic ordering in Na doped BaFe$_2$As$_2$ by unpolarized and polarized neutron diffraction using single crystals. Unlike previously studied FeAs-based compounds that magnetically order, Ba$_{1-x}$Na$_x$Fe$_2$As$_2$…

Superconductivity · Physics 2015-06-22 F. Wasser , A. Schneidewind , Y. Sidis , S. Aswartham , S. Wurmehl , B. Buchner , M. Braden

We investigated the spin-lattice coupling in orthorhombic pseudobrookite FeTi2O5 single crystal with highly ordered $ Fe^{2+} / Ti^{4+}$ occupation, which consists of quasi-1D S=2 chains running along a-axis. Both the magnetization and…

Strongly Correlated Electrons · Physics 2024-05-31 Hao-Hang Xu , Jian Liu , L. L. Tao , Xian-Jie Wang , Sergey V. Streltsov , Yu Sui

Van der Waals materials provide a versatile toolbox for the emergence of new quantum phenomena and the fabrication of functional heterostructures. Among them, the trihalide VI3 stands out for its unique magnetic and structural landscape.…

Materials Science · Physics 2024-02-07 A. De Vita , R. Sant , V. Polewczyk , G. van der Laan , N. B. Brookes , T. Kong , R. J. Cava , G. Rossi , G. Vinai , G. Panaccione

CeTe$_3$ is a van der Waals antiferromagnet composed of magnetic [CeTe]$^+$ layers coupled to highly conducting Te$^{0.5-}$ square nets. Its simple quasi-two-dimensional electronic structure and cleavable nature make it an appealing…

Strongly Correlated Electrons · Physics 2026-04-29 Ryutaro Okuma , Yuita Fujisawa , Natsumi Maekawa , Akiko Nakao , Yoshihisa Ishikawa , Riki Kobayashi , Yoshinori Okada , Daichi Ueta

We show that in colloidal models of artificial kagome and modified square ice systems, a variety of ordering and disordering regimes occur as a function of biasing field, temperature, and colloid-colloid interaction strength, including…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 C. J. Olson Reichhardt , A. Libal , C. Reichhardt

We present the study of magnetization, thermal expansion, specific heat, resistivity, and a.c. susceptibility of (Pr$_{1-y}$Eu$_y$)$_{0.7}$Ca$_{0.3}$CoO$_3$ cobaltites. The measurements were performed on ceramic samples with $y = 0.12 -…

Pr-containing perovskite cobaltites exhibit unusual valence transitions, coupled to coincident structural, spin-state, and metal-insulator transitions. Heteroepitaxial strain was recently used to control these phenomena in the model…

Strong electronic interactions can drive a system into a state with a symmetry breaking. Lattice frustration or competing interactions tend to prevent a symmetry breaking, leading to quantum disordered phases. In spin systems frustration…

Magnetization, magnetocaloric, calorimetric, neutron and X-ray diffraction and inelastic neutron scattering measurements are performed on single crystals of BaCdVO(PO$_4$)$_2$. The low-temperature crystal structure is found to be of a lower…

Strongly Correlated Electrons · Physics 2019-11-07 V. K. Bhartiya , K. Yu. Povarov , D. Blosser , S. Bettler , Z. Yan , S. Gvasaliya , S. Raymond , E. Ressouche , K. Beauvois , J. Xu , F. Yokaichiya , A. Zheludev

Two-dimensional (2D) van der Waals (vdW) magnetic materials with high coercivity and high $T_\text{C}$ are desired for spintronics and memory storage applications. Fe$_3$GeTe$_2$ (F3GT) is one such 2D vdW ferromagnet with a reasonably high…

We report site disorder driven ferromagnetic ordering of nearly 8$\%$ Ce atoms in single crystalline Ce${_3}$Os${_4}$Ge$_{13}$ below 0.5~K. Ce${_3}$Os${_4}$Ge$_{13}$ crystallizes in a cubic structure with space group $\it{Pm\bar{3}n}$. The…

Strongly Correlated Electrons · Physics 2016-02-26 Om Prakash , A. Thamizhavel , S. Ramakrishnan

Quantum phase transitions in the two-dimensional Kugel-Khomski model on a square lattice are studied using the plaquette mean field theory and the entanglement renormalization ansatz. When $3z^2-r^2$ orbitals are favored by the crystal…

Strongly Correlated Electrons · Physics 2012-12-06 Wojciech Brzezicki , Jacek Dziarmaga , Andrzej M. Oleś

The crystal and magnetic structures of the three-leg ladder compound Fe3BO5 have been investigated by single crystal x-ray diffraction and neutron powder diffraction. Fe3BO5 contains two types of three-leg spin ladders. It shows a charge…

Strongly Correlated Electrons · Physics 2009-04-15 Pierre Bordet , Emmanuelle Suard