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The quasi-two-dimensional van der Waals magnet Fe$_{5-\delta}$GeTe$_2$ has emerged as a promising platform for electronic and spintronic functionalities at room temperature, owing to its large ferromagnetic ordering temperature…

We study theoretically low-temperature phases of a recently synthesized compound Sr$_2$CoO$_3$F under pressure. The analysis combining LDA+DMFT and a strong-coupling effective model points to the existence of not only normal paramagnetic…

Strongly Correlated Electrons · Physics 2019-05-15 Juan Fernández Afonso , Andrii Sotnikov , Atsushi Hariki , Jan Kuneš

We report on a 59Co NMR investigation of the trigonal cobaltate Ca3Co2O6 carried out on a single crystal, providing precise determinations of the electric field gradient and chemical shift tensors, and of the internal magnetic fields at the…

Strongly Correlated Electrons · Physics 2015-05-20 G. Allodi , R. De Renzi , S. Agrestini , C. Mazzoli , M. R. Lees

We report the effects of cobalt doping on the magnetic properties of two-dimensional van der Waals ferromagnet Fe3GeTe2. Single crystals of (Fe{1-x}Cox)3GeTe2 with x=0-0.78 were successfully synthesized and characterized with x-ray…

Materials Science · Physics 2020-03-06 Cong-Kuan Tian , Cong Wang , Wei Ji , Jin-Chen Wang , Tian-Long Xia , Le Wang , Juan-Juan Liu , Hong-Xia Zhang , Peng Cheng

Fe5-xGeTe2 is a van der Waals material with one of the highest reported bulk Curie temperatures, $T_C$ ~ 310K. In this study, theoretical calculations and experiments are utilized to demonstrate that the magnetic ground state is highly…

Materials Science · Physics 2020-08-20 Andrew F. May , Mao-Hua Du , Valentino R. Cooper , Michael A. McGuire

The antiferromagnetic - ferromagnetic phase transition in YBaCo2O5.50 and YBaCo2O5.44 cobaltites with different types of oxygen-ion ordering in the [YO0.5/0.44] layers has been studied by neutron powder diffraction. Using the magnetic…

Materials Science · Physics 2007-05-23 D. D. Khalyavin , D. N. Argyriou , U. Amann , A. A. Yaremchenko , V. V. Kharton

Magnetic state is a partial ordered state if only part of the electrons in the system give contribution to the magnetic order. We study Heisenberg model of two sublattice spin system, on the body-centered cubic lattice, with…

Strongly Correlated Electrons · Physics 2024-09-20 N. Karchev

We report that MoX3 (X = I, Br) are rare van der Waals materials that exhibit signatures of both quantum spin chains with a spin singlet ground state and classical Neel order. Bulk single crystals grown by chemical vapor transport exhibit…

We investigate magnetic properties of CrTe$_2$ within the density functional theory (DFT) approach in ferromagnetic phase and combination of DFT and dynamical mean field theory (DFT+DMFT) approach in paramagnetic phase. We show that few…

Strongly Correlated Electrons · Physics 2026-03-03 A. A. Katanin , E. M. Agapov

We report the doping effects of cobalt on van der Waals (vdW) magnet Fe$_5$GeTe$_2$. A series of (Fe$_{1-x}$Co$_x$)$_5$GeTe$_2$ (0$\leq$x$\leq$0.44) single crystals have been successfully grown, their structural, magnetic and transport…

Mesoscale and Nanoscale Physics · Physics 2020-06-05 Congkuan Tian , Feihao Pan , Sheng Xu , Kun Ai , Tian-long Xia , Peng Cheng

The realization of long-range spin order in two-dimensions (2D) has catapulted the search for layered materials with magnetic ordering above room temperature. These efforts aim to understand and enhance the spin spin interactions in 2D. An…

Materials Science · Physics 2025-12-23 Rabindra Basnet , Ramesh C. Budhani

We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

Ferromagnetic Kondo lattice compounds are far less common than their antiferromagnetic analogs. In this work, we report the discovery of a new ferromagnetic Kondo lattice compound, YbIr3Ge7. Like almost all ferromagnetic Kondo lattice…

Strongly Correlated Electrons · Physics 2019-03-27 Binod K. Rai , Macy Stavinoha , J. Banda , D. Hafner , Katherine A. Benavides , D. A. Sokolov , Julia Chan , M. Brando , C. -L. Huang , E. Morosan

We investigate the temperature-dependent electronic structure of the van der Waals ferromagnet, CrGeTe$_3$. Using angle-resolved photoemission spectroscopy, we identify atomic- and orbital-specific band shifts upon cooling through…

Magnetic phase transitions often occur spontaneously at specific critical temperatures. The presence of more than one critical temperature (Tc) has been observed in several compounds where the coexistence of competing magnetic orders…

The peculiar field-dependent magnetism of Na0.82CoO2 has been investigated through an analysis of its DC and AC spin susceptibilities. To account for the easily activated narrow b2g-a1g gap of the crystal field for Co in the cobalt oxide…

Strongly Correlated Electrons · Physics 2016-10-04 G. J. Shu , F. C. Chou

The magnetic structure and phase diagram of the layered ferromagnetic compound Fe$_3$GeTe$_2$ has been investigated by a combination of synthesis, x-ray and neutron diffraction, high resolution microscopy, and magnetization measurements.…

Strongly Correlated Electrons · Physics 2016-01-13 Andrew F. May , Stuart Calder , Claudia Cantoni , Huibo Cao , Michael A. McGuire

The magnetic properties of the quasi-two-dimensional van der Waals magnet Fe$_{5-\delta}$GeTe$_2$ (F5GT), which has a high ferromagnetic ordering temperature $T_{\text{C}}$ $\sim$ 315 K, remains to be better understood. It has been…

Strongly Correlated Electrons · Physics 2023-04-26 Xiang Chen , Wei Tian , Yu He , Hongrui Zhang , Tyler L. Werner , Saul Lapidus , Jacob P. C. Ruff , Ramamoorthy Ramesh , Robert J. Birgeneau

Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in A-site…

Materials Science · Physics 2011-09-21 G. J. MacDougall , D. Gout , J. L. Zarestky , G. Ehlers , A. Podlesnyak , M. A. McGuire , D. Mandrus , S. E. Nagler

Phases of matter are conventionally characterized by order parameters describing the type and degree of order in a system. For example, crystals consist of spatially ordered arrays of atoms, an order that is lost as the crystal melts. Like-…

Quantum Gases · Physics 2023-07-20 D. L. Campbell , R. M. Price , A. Putra , A. Valdés-Curiel , D. Trypogeorgos , I. B. Spielman
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