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Related papers: Efficient Computation of the Long-Range Exact Exch…

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We assess the accuracy of common hybrid exchange-correlation (XC) functionals (PBE0, PBE0-1/3, HSE06, HSE03, and B3LYP) within Kohn-Sham density functional theory (KS-DFT) for the harmonically perturbed electron gas at parameters relevant…

Chemical Physics · Physics 2023-03-08 Zhandos A. Moldabekov , Mani Lokamani , Jan Vorberger , Attila Cangi , Tobias Dornheim

We present efficient approximation of the error function obtained by Fourier expansion of the exponential function $\exp [{- {(t - 2 \sigma)^2}/4}]$. The error analysis reveals that it is highly accurate and can generate numbers that match…

Numerical Analysis · Mathematics 2013-08-16 S. M. Abrarov , B. M. Quine

In this paper a spline based integral approximation is utilized to propose a sequence of approximations to the error function that converge at a significantly faster manner than the default Taylor series. The approximations can be improved…

General Mathematics · Mathematics 2022-07-27 Roy M. Howard

We construct exact Kohn-Sham potentials for the ensemble density-functional theory (EDFT) from the ground and excited states of helium. The exchange-correlation (XC) potential is compared with the quasi-local-density approximation and both…

Various properties of the general two-center two-electron integral over the explicitly correlated exponential function are analyzed for the potential use in high precision calculations for diatomic molecules. A compact one dimensional…

Chemical Physics · Physics 2015-06-11 Krzysztof Pachucki

An exchange-correlation energy functional $ E_{\mathrm xc} $ and the resultant exchange-correlation potential $ v_{\mathrm xc}({\bf r}) $ in density-functional theory are proposed using orbital-dependent coupling-constant-averaged pair…

Strongly Correlated Electrons · Physics 2007-05-23 Hiroshi Yasuhara , Masahiko Higuchi , Yoshiyuki Kawazoe

Density-functional theory simplifies many-electron calculations by approximating the exchange and correlation interactions with a one-electron operator that is a functional of the density. Hybrid functionals incorporate some amount of exact…

Materials Science · Physics 2021-02-03 John Vinson

We lay out the extension of range-separated density-functional theory to a four-component relativistic frame-work using a Dirac-Coulomb-Breit Hamiltonian in the no-pair approximation. This formalism combines a wave-function method for the…

Chemical Physics · Physics 2018-12-12 Julien Paquier , Julien Toulouse

We study the effect of Coulomb potential on high-order harmonic generation (HHG) numerically and analytically. We focus on the influence of Coulomb potential on emission times of HHG associated with specific electron trajectories. By using…

Atomic Physics · Physics 2022-09-21 X. J. Xie , R. H. Xu , S. J. Yu , X. Liu , W. Li , Y. J. Chen

A new sampling methodology based on incomplete cosine expansion series is presented as an alternative to the traditional sinc function approach. Numerical integration shows that this methodology is efficient and practical. Applying the…

Numerical Analysis · Mathematics 2015-03-24 S. M. Abrarov , B. M. Quine

The exchange-correlation (XC) functional in density functional theory is used to approximate multi-electron interactions. A plethora of different functionals is available, but nearly all are based on the hierarchy of inputs commonly…

Density functionals with a range-separated treatment of the exchange energy are known to improve upon their semilocal forerunners and fixed-fraction hybrids. The conversion of a given semilocal functional into its short-range analog is not…

Chemical Physics · Physics 2019-09-09 Dimitri N. Laikov

We propose a method to compute, for a given potential model, an arbitrary coefficient of the effective-range function expanded as a power series in energy. The method is based on a set of recurrence relations at low energy, that allows a…

Nuclear Theory · Physics 2013-08-09 O. L. Ramírez Suárez , J-M. Sparenberg

In this paper we apply a well-tested approximation of electron Coulomb distortion effects to the exclusive reaction (e,e'p) in the quasielastic region. We compare the approximate treatment of Coulomb distortion effects to the exact…

Nuclear Theory · Physics 2008-11-26 K. S. Kim , L. E. Wright

An enhanced static approximation for the electron self energy operator is proposed for efficient calculation of quasiparticle energies. Analysis of the static COHSEX approximation originally proposed by Hedin shows that most of the error…

Materials Science · Physics 2010-11-18 Wei Kang , Mark S. Hybertsen

In this work we show the advantages of using the Coulomb-hole plus screened-exchange (COHSEX) approach in the calculation of potential energy surfaces. In particular, we demonstrate that, unlike perturbative $GW$ and partial self-consistent…

Chemical Physics · Physics 2021-06-14 J. Arjan Berger , Pierre-François Loos , Pina Romaniello

The differential and partially integrated cross sections are considered for bremsstrahlung from high-energy electrons in atomic field with the exact account of this field. The consideration exploits the quasiclassical electron Green's…

High Energy Physics - Phenomenology · Physics 2009-11-10 R. N. Lee , A. I. Milstein , V. M. Strakhovenko , O. Ya. Schwarz

We examine the performance of our recently developed LFAs-PBE exchange-correlation (XC) potential [C.-R. Pan, P.-T. Fang, and J.-D. Chai, Phys. Rev. A, 2013, 87, 052510] for the high-order harmonic generation (HHG) spectra and related…

Chemical Physics · Physics 2016-06-14 Hsiao-Ling Sun , Wei-Tao Peng , Jeng-Da Chai

The Heyd-Scuseria-Ernzerhof (HSE) density functionals are popular for their ability to improve the accuracy of standard semilocal functionals such as Perdew-Burke-Ernzerhof (PBE), particularly for semiconductor band gaps. They also have a…

Materials Science · Physics 2025-10-07 Jonathan E. Moussa , Peter A. Schultz , James R. Chelikowsky

The Bethe-Salpeter Equation (BSE) can be applied to compute from first-principles optical spectra that include the effects of screened electron-hole interactions. As input, BSE calculations require single-particle states, quasiparticle…

Materials Science · Physics 2020-01-01 Joshua Elliott , Nicola Colonna , Margherita Marsili , Nicola Marzari , Paolo Umari
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