Related papers: High-Order Harmonic Generation in Organic Molecula…
High-harmonic generation (HHG), a typical nonlinear optical effect, has been actively studied in electron systems such as semiconductors and superconductors. As a natural extension, we theoretically study HHG from electric polarization,…
High-harmonic generation (HHG) is a nonlinear process in which a strong driving field interacts with a material, resulting in the frequency up-conversion of the driver into its high-order harmonics. This process is highly sensitive to the…
High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…
We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…
Direct imaging of molecular dynamics is a long-standing goal in physics and chemistry. As an emerging tool, high-harmonic spectroscopy (HHS) enables accessing molecular dynamics on femtosecond to attosecond time scales. However, decoding…
High-harmonic generation (HHG) in solids is an emerging method to probe ultrafast electron dynamics in solids at attosecond timescale. In this work, we study HHG from monolayer and bilayer graphene. Bilayer graphenes with AA and AB stacking…
High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full…
High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in…
An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…
We report theoretical investigations of the tomographic procedure suggested by Itatani {\it et al.} [Nature, {\bf 432} 867 (2004)] for reconstructing highest occupied molecular orbitals (HOMO) using high-order harmonic generation (HHG).…
High-harmonic generation (HHG) is one of the fundamental processes at the heart of attosecond physics. Traditionally viewed as an effective single-particle effect, recent advances have focused on contributions beyond this single-particle…
A theoretical model for high-order harmonic generation (HHG) in bulk solids is considered. Our approach treats laser-induced inter- and intraband currents on an equal footing. The sum of these currents is the source of the high-order…
We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…
High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational…
High harmonic generation (HHG) enables extreme ultraviolet radiation with table-top setups. Its exceptional properties, such as coherence and (sub)-femtosecond pulse durations, have led to a diversity of applications. Some of these require…
We present a study of photon statistics associated with high-order harmonic generation (HHG) involving one-mode and intermodal correlations of the high harmonic photons. The aim of the paper is to give insight into the nonclassical…
Organic molecular crystals are appealing for next-generation optoelectronic applications, most notably due to their multiexciton generation process that can increase the efficiency of photovoltaic devices. However, a general understanding…
Because the commonly adopted viewpoint that the Keldysh parameter $\gamma $ determines the dynamical regime in strong field physics has long been demonstrated to be misleading, one can ask what happens as relevant physical parameters, such…
We study high-order harmonic generation (HHG) in model atoms driven by plasmonic-enhanced fields. These fields result from the illumination of plasmonic nanostructures by few-cycle laser pulses. We demonstrate that the spatial inhomogeneous…
To clarify the microscopic origin of chirality-induced optical effect, we develop an analytical method that extracts the chiral part of the Hamiltonian of molecular electronic states. We demonstrate this method in a model chiral molecule…