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Studying the excited states of doublets is challenging for their typically multiconfigurational character. We employ light-scanning-tunneling microscopy (light-STM) to investigate photon-induced currents on a single open-shell PTCDA anion…

Atomic and Molecular Clusters · Physics 2025-02-14 Rodrigo Cezar de Campos Ferreira , Amandeep Sagwal , Jiří Doležal , Tomáš Neuman , Martin Švec

The exceptionally strong coupling realizable between superconducting qubits and photons stored in an on-chip microwave resonator allows for the detailed study of matter-light interactions in the realm of circuit quantum electrodynamics…

Mesoscale and Nanoscale Physics · Physics 2009-12-21 J. M. Fink , M. Baur , R. Bianchetti , S. Filipp , M. Göppl , P. J. Leek , L. Steffen , A. Blais , A. Wallraff

We consider trasfer-ionization in collisions of fast (3.6 -- 11 MeV/u) protons, alpha-particles and lithium nuclei with helium atoms. There are just a few basic mechanisms contributing to this process which can be grouped into correlated…

Atomic Physics · Physics 2015-06-05 A. B. Voitkiv , X. Ma

Many superconducting qubit systems use the dispersive interaction between the qubit and a coupled harmonic resonator to perform quantum state measurement. Previous works have found that such measurements can induce state transitions in the…

Organic semiconducting polymers are currently of broad interest as potential low-cost materials for photovoltaic and light-emitting display applications. I will give an overview of our work in developing a consistent quantum dynamical…

Materials Science · Physics 2007-05-23 Eric R. Bittner , John Glen S. Ramon

Quantum computation will rely on quantum error correction to counteract decoherence. Successfully implementing an error correction protocol requires the fidelity of qubit operations to be well-above error correction thresholds. In…

We present a theoretical framework to describe state-resolved ionization dynamics of neon atoms driven by ultraintense x-ray free-electron-laser pulses. In general, x-ray multiphoton ionization dynamics of atoms have been described by…

Atomic Physics · Physics 2023-01-10 Laura Budewig , Sang-Kil Son , Robin Santra

Qubit initialization is a critical task in quantum computation and communication. Extensive efforts have been made to achieve this with high speed, efficiency and scalability. However, previous approaches have either been measurement-based…

We develop an efficient numerical approach for simulating the high-power dispersive readout in circuit quantum electrodynamics. In the numerical simulations of the high-power readout, a large-amplitude coherent state induced in a cavity is…

Quantum Physics · Physics 2023-10-17 Shimpei Goto , Kazuki Koshino

We experimentally studied the microwave response of a transmon artificial atom coupled to two closely spaced resonant modes. When the atom is under driven with one of the modes, the atom state and mode photons are superposed, forming the…

Quantum Physics · Physics 2019-06-18 Yu-Han Chang , Dmytro Dubyna , Wei-Chen Chien , Chien-Han Chen , Cen-Shawn Wu , Watson Kuo

A superconducting qubit coupled to a read-out resonator is currently the building block of multiple quantum computing as well as quantum optics experiments. A typical qubit-resonator system is coupled in the dispersive regime, where the…

Quantum Physics · Physics 2023-11-27 Arvind Mamgain , Samarth Hawaldar , Athreya Shankar , Baladitya Suri

Excited state proton transfer is an ubiquitous phenomenon in biology and chemistry, spanning from the ultrafast reactions of photo-bases and acids to light-driven, enzymatic catalysis and photosynthesis. However, the simulation of such…

Chemical Physics · Physics 2024-10-18 Brieuc Le Dé , Simon Huppert , Riccardo Spezia , Alex W. Chin

We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

Atomic Physics · Physics 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

Data for inelastic processes due to hydrogen atom collisions with iron are needed for accurate modelling of the iron spectrum in late-type stars. Excitation and charge transfer in low-energy Fe+H collisions is studied theoretically using a…

Solar and Stellar Astrophysics · Physics 2018-05-09 P. S. Barklem

The dissociation dynamics of the $\tilde{A}$-state of ammonia have been studied using a resonant multiphoton ionisation probe in a photoelectron spectroscopy experiment. The use of a resonant intermediate in the multiphoton ionisation…

Excitation and charge transfer in low-energy O+H collisions is studied; it is a problem of importance for modelling stellar spectra and obtaining accurate oxygen abundances in late-type stars including the Sun. The collisions have been…

Solar and Stellar Astrophysics · Physics 2018-02-28 P. S. Barklem

Coherent time evolution of highly excited Rydberg states in Rb (98 < n < 150) under pulsed electric field in high slew-rate regime was investigated with the field ionization detection. The electric field necessary to ionize the Rydberg…

Atomic Physics · Physics 2007-05-23 M. Tada , Y. Kishimoto , I. Ogawa , H. Funahashi , K. Yamamoto , S. Matsuki

Superconducting quantum circuits rely on strong drives to implement fast gates, high-fidelity readout, and state stabilization. However, these drives can induce uncontrolled excitations, so-called "ionization", that compromise the fidelity…

The description of excited state dynamics in multichromophoric systems constitutes both a theoretical and experimental challenge in modern physical chemistry. An experimental protocol which can systematically characterize both coherent and…

Quantum Physics · Physics 2011-10-31 Joel Yuen-Zhou , Jacob J. Krich , Masoud Mohseni , Alán Aspuru-Guzik

We investigate a ionising electronic transition under resonant pumping. We demonstrate that, above a critical value of the pump intensity, a novel metastable electronic bound state is created, which can decay into the free electron…

Atomic Physics · Physics 2025-12-24 Erika Cortese , Simone De Liberato