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Molecular quantum magnets adsorbed on surfaces exhibit rich spin and orbital excitations that can be probed by scanning tunneling microscopy with inelastic electron tunneling spectroscopy (STM-IETS). However, the quantitative extraction of…

Mesoscale and Nanoscale Physics · Physics 2026-01-28 Greta Lupi , Adolfo O. Fumega , Mohammad Amini , Robert Drost , Peter Liljeroth , Jose L. Lado

Nanoscale engineered spin systems, ranging from spins on surfaces to nanographenes, provide flexible platforms to realize entangled quantum magnets from a bottom up approach. However, assessing the quantum many-body Hamiltonian realized in…

Mesoscale and Nanoscale Physics · Physics 2025-10-22 Netta Karjalainen , Greta Lupi , Rouven Koch , Adolfo O. Fumega , Jose L. Lado

Extracting Hamiltonian parameters from available experimental data is a challenge in quantum materials. In particular, real-space spectroscopy methods such as scanning tunneling spectroscopy allow probing electronic states with atomic…

Mesoscale and Nanoscale Physics · Physics 2024-01-23 Maryam Khosravian , Rouven Koch , Jose L. Lado

Impurities in quantum materials have provided successful strategies for learning properties of complex states, ranging from unconventional superconductors to topological insulators. In quantum magnetism, inferring the Hamiltonian of an…

Mesoscale and Nanoscale Physics · Physics 2025-06-23 Greta Lupi , Jose L. Lado

Interacting spins in quantum magnet can cooperate and exhibit exotic states like the quantum spin liquid. To explore the materialization of such intriguing states, the determination of effective spin Hamiltonian of the quantum magnet is…

Strongly Correlated Electrons · Physics 2021-09-01 Sizhuo Yu , Yuan Gao , Bin-Bin Chen , Wei Li

Hamiltonian parameter estimation is crucial in condensed matter physics, but time and cost consuming in terms of resources used. With advances in observation techniques, high-resolution images with more detailed information are obtained,…

Disordered Systems and Neural Networks · Physics 2019-11-15 Dingchen Wang , Songrui Wei , Anran Yuan , Fanghua Tian , Kaiyan Cao , Qizhong Zhao , Dezhen Xue , Sen Yang

We propose a quantum algorithm for inferring the molecular nuclear spin Hamiltonian from time-resolved measurements of spin-spin correlators, which can be obtained via nuclear magnetic resonance (NMR). We focus on learning the anisotropic…

Efficiently characterising quantum systems, verifying operations of quantum devices and validating underpinning physical models, are central challenges for the development of quantum technologies and for our continued understanding of…

Hamiltonian learning is an important procedure in quantum system identification, calibration, and successful operation of quantum computers. Through queries to the quantum system, this procedure seeks to obtain the parameters of a given…

Quantum Physics · Physics 2023-08-25 Arkopal Dutt , Edwin Pednault , Chai Wah Wu , Sarah Sheldon , John Smolin , Lev Bishop , Isaac L. Chuang

It is natural to measure the observables from the Hamiltonian-based quantum dynamics, and its inverse process that Hamiltonians are estimated from the measured data also is a vital topic. In this work, we propose a recurrent neural network…

Quantum Physics · Physics 2021-06-30 Liangyu Che , Chao Wei , Yulei Huang , Dafa Zhao , Shunzhong Xue , Xinfang Nie , Jun Li , Dawei Lu , Tao Xin

Two-dimensional noncollinear magnetic states, such as spin-spiral magnets, offer an excellent platform for investigating fundamental phenomena, with potential for advancing stray-field-free spintronics. However, detection and…

Mesoscale and Nanoscale Physics · Physics 2026-04-06 Fedor Nigmatulin , Greta Lupi , Jose L. Lado , Zhipei Sun

We build upon recent work on using Machine Learning models to estimate Hamiltonian parameters using continuous weak measurement of qubits as input. We consider two settings for the training of our model: (1) supervised learning where the…

Quantum Physics · Physics 2025-02-17 Kris Tucker , Amit Kiran Rege , Conor Smith , Claire Monteleoni , Tameem Albash

We develop a computational method to learn a molecular Hamiltonian matrix from matrix-valued time series of the electron density. As we demonstrate for three small molecules, the resulting Hamiltonians can be used for electron density…

Computational Physics · Physics 2020-09-01 Harish S. Bhat , Karnamohit Ranka , Christine M. Isborn

We introduce a Hamiltonian-based quantum feature extraction method that generates complex features via the dynamics of $k$-local many-body spins Hamiltonians, enhancing machine learning performance. Classical feature vectors are embedded…

Determining the Hamiltonian of a quantum system is essential for understanding its dynamics and validating its behavior. Hamiltonian learning provides a data-driven approach to reconstruct the generator of the dynamics from measurements on…

Characterization of qubit couplings in many-body quantum systems is essential for benchmarking quantum computation and simulation. We propose a tomographic measurement scheme to determine all the coupling terms in a general many-body…

Quantum Physics · Physics 2015-10-06 Sheng-Tao Wang , Dong-Ling Deng , Lu-Ming Duan

We present a machine-learning method for predicting sharp transitions in a Hamiltonian phase diagram by extrapolating the properties of quantum systems. The method is based on Gaussian Process regression with a combination of kernels chosen…

Other Condensed Matter · Physics 2019-04-26 Rodrigo A. Vargas-Hernández , John Sous , Mona Berciu , Roman V. Krems

We study the problem of learning the parameters for the Hamiltonian of a quantum many-body system, given limited access to the system. In this work, we build upon recent approaches to Hamiltonian learning via derivative estimation. We…

Quantum Physics · Physics 2024-01-10 Andi Gu , Lukasz Cincio , Patrick J. Coles

Characterizing quantum many-body systems is a fundamental problem across physics, chemistry, and materials science. While significant progress has been made, many existing Hamiltonian learning protocols demand digital quantum control over…

Quantum Physics · Physics 2025-10-10 Sitan Chen , Jordan Cotler , Hsin-Yuan Huang

An isolated system of interacting quantum particles is described by a Hamiltonian operator. Hamiltonian models underpin the study and analysis of physical and chemical processes throughout science and industry, so it is crucial they are…

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