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The Gibbs free energy is the fundamental thermodynamic potential underlying the relative stability of different states of matter under constant-pressure conditions. However, computing this quantity from atomic-scale simulations is far from…

Materials Science · Physics 2018-02-14 Bingqing Cheng , Michele Ceriotti

Machine learning offers an unprecedented perspective for the problem of classifying phases in condensed matter physics. We employ neural-network machine learning techniques to distinguish finite-temperature phases of the strongly correlated…

Strongly Correlated Electrons · Physics 2017-09-12 Kelvin Ch'ng , Juan Carrasquilla , Roger G. Melko , Ehsan Khatami

We develop an artificial neural network model to predict quantum heat engines working within the experimentally realized framework of electromagnetically induced transparency. We specifically focus on {\Lambda}-type alkali-based cold atomic…

Quantum Physics · Physics 2025-01-07 Manash Jyoti Sarmah , Himangshu Prabal Goswami

Experimental calibration of dynamic thermal models is required for model predictive control and characterization of building energy performance. In these applications, the uncertainty assessment of the parameter estimates is decisive; this…

Applications · Statistics 2019-04-25 L. Raillon , Christian Ghiaus

The application of deep learning to non-stationary temporal datasets can lead to overfitted models that underperform under regime changes. In this work, we propose a modular machine learning pipeline for ranking predictions on temporal…

Computational Finance · Quantitative Finance 2023-08-11 Thomas Wong , Mauricio Barahona

Understanding and predicting the glassy dynamics of polymers remain fundamental challenges in soft matter physics. While the Elastically Collective Nonlinear Langevin Equation (ECNLE) theory has been successful in describing relaxation…

Soft Condensed Matter · Physics 2025-07-09 Anh D. Phan , Ngo T. Que , Nguyen T. T. Duyen , Phan Thanh Viet , Quach K. Quang , Baicheng Mei

We introduce a simple and predictive model for determining the phase stability of ternary phospholipid-cholesterol mixtures. Assuming that competition between the liquid and gel order of the phospholipids is the main driving force behind…

Soft Condensed Matter · Physics 2011-04-01 Jean Wolff , Carlos M. Marques , Fabrice Thalmann

Accurate phase diagram prediction is crucial for understanding alloy thermodynamics and advancing materials design. While traditional CALPHAD methods are robust, they are resource-intensive and limited by experimentally assessed data. This…

Materials Science · Physics 2025-07-08 Siya Zhu , Raymundo Arróyave , Doğuhan Sarıtürk

We introduce a machine-learning approach to predict the complex non-Markovian dynamics of supercooled liquids from static averaged quantities. Compared to techniques based on particle propensity, our method is built upon a theoretical…

Disordered Systems and Neural Networks · Physics 2023-03-17 Simone Ciarella , Massimiliano Chiappini , Emanuele Boattini , Marjolein Dijkstra , Liesbeth M. C. Janssen

Critical heat flux is a key quantity in boiling system modeling due to its impact on heat transfer and component temperature and performance. This study investigates the development and validation of an uncertainty-aware hybrid modeling…

Machine Learning · Computer Science 2025-07-17 Aidan Furlong , Xingang Zhao , Robert Salko , Xu Wu

Machine learning models have emerged as a very effective strategy to sidestep time-consuming electronic-structure calculations, enabling accurate simulations of greater size, time scale and complexity. Given the interpolative nature of…

Knowledge Distillation (KD) trains a smaller student model using a large, pre-trained teacher model, with temperature as a key hyperparameter controlling the softness of output probabilities. Traditional methods use a fixed temperature…

Machine Learning · Computer Science 2025-11-19 Sibgat Ul Islam , Jawad Ibn Ahad , Fuad Rahman , Mohammad Ruhul Amin , Nabeel Mohammed , Shafin Rahman

We propose an efficient ab initio framework to compute the Gibbs energy of the transition state in vacancy-mediated diffusion including the relevant thermal excitations at density-functional-theory level. With the aid of a bespoke…

Materials Science · Physics 2024-10-08 Xi Zhang , Sergiy V. Divinski , Blazej Grabowski

We develop a thermodynamic theory for machine learning (ML) systems. Similar to physical thermodynamic systems which are characterized by energy and entropy, ML systems possess these characteristics as well. This comparison inspire us to…

Machine Learning · Computer Science 2024-04-23 Dong Zhang

Model predictive control has gained popularity for its ability to satisfy constraints and guarantee robustness for certain classes of systems. However, for systems whose dynamics are characterized by a high state dimension, substantial…

Systems and Control · Electrical Eng. & Systems 2024-11-26 Demetrius Gulewicz , Uduak Inyang-Udoh , Trevor Bird , Neera Jain

We compute the phase separation of the immiscible liquid alloy Fe-Cu-Ni. Our computational approach uses a virtual semigrand canonical Widom approach to determine differences in excess chemical potentials between different species. Using an…

Materials Science · Physics 2025-07-09 Dallas R. Trinkle

Neural network potentials (NNPs) offer a powerful alternative to traditional force fields for molecular dynamics (MD) simulations. Accurate and stable MD simulations, crucial for evaluating material properties, require training data…

Machine Learning · Computer Science 2025-06-23 Naoki Matsumura , Yuta Yoshimoto , Yuto Iwasaki , Meguru Yamazaki , Yasufumi Sakai

Standard enthalpies of formation are used for assessing the efficiency and safety of chemical processes in the chemical industry. However, the number of compounds for which the enthalpies of formation are available is many orders of…

Computational Engineering, Finance, and Science · Computer Science 2013-02-05 Ana L. Teixeira , Rui C. Santos , Joao P. Leal , Jose A. Martinho Simoes , Andre O. Falcao

Temperature is a fundamental regulator of chemical and biochemical kinetics, yet capturing nonlinear thermal effects directly from experimental data remains a major challenge due to limited throughput and model flexibility. Recent advances…

Quantitative Methods · Quantitative Biology 2025-12-23 Mamoru Saita , Yutaka Hori

Accurate prediction of thermodynamic properties is pivotal in chemical engineering for optimizing process efficiency and sustainability. Physical group-contribution (GC) methods are widely employed for this purpose but suffer from…

Chemical Physics · Physics 2025-01-28 Nicolas Hayer , Thorsten Wendel , Stephan Mandt , Hans Hasse , Fabian Jirasek