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We show that combining vibrational spectroscopy with signal processing can result in a scheme for ultrasensitive detection of molecules. We consider the vibrational spectrum as a signal on the energy axis and apply a matched filter on that…

Computational Physics · Physics 2018-12-10 Tay Yong Boon , Ian Tay Rongde , Loy Liang Yi , Aw Ke Fun , Ong Zhi Li , Sergei Manzhos

The ultrastrong and deep strong coupling regimes exhibit a variety of intriguing physical phenomena. In this work, we utilize the Hopfield model of a two-mode bosonic system, with each mode interacts with a heat reservoir, to research the…

Quantum Physics · Physics 2026-01-28 Yu-qiang Liu , Qiulin Long , Yi-jia Yang , Zheng Liu , Ting-ting , Ma , Bao-qing , Guo , Xingdong , Zhao , Zunlue , Zhu , Wuming , Liu , Chang-shui Yu

We explore the nonlinear dynamics of a cavity optomechanical system. Our realization consisting of a drumhead nano-electro-mechanical resonator (NEMS) coupled to a microwave cavity, allows for a nearly ideal platform to study the…

Virtual excitations, inherent to ultrastrongly coupled light-matter systems, induce measurable modifications in system properties, offering a novel resource for quantum technologies. In this work, we demonstrate how these virtual…

Quantum Physics · Physics 2025-09-12 Christoph Hotter , Adam Miranowicz , Karol Gietka

A vibrational model of transport properties of dense fluids assumes that solid-like oscillations of atoms around their temporary equilibrium positions dominate the dynamical picture. The temporary equilibrium positions of atoms do not form…

Soft Condensed Matter · Physics 2024-01-09 Sergey Khrapak

Motivated by a proposed olfactory mechanism based on a vibrationally-activated molecular switch, we study electron transport within a donor-acceptor pair that is coupled to a vibrational mode and embedded in a surrounding environment. We…

Mesoscale and Nanoscale Physics · Physics 2015-02-12 Agata Checinska , Felix A. Pollock , Libby Heaney , Ahsan Nazir

Dissipative Kerr solitons (DKSs) intrinsically exhibit two degrees of freedom through their group and phase rotation velocity. Periodic extraction of the DKS into a waveguide produces a pulse train and yields the resulting optical frequency…

We studied the interaction of a two-level atom with a frequency modulated cavity mode in an ideal optical cavity. The system, described by a Jaynes-Cumming Hamiltonian, gave rise to a set of stiff nonlinear first order equations solved…

Quantum Physics · Physics 2013-01-22 U. Pishipati , I. Almakremi , Amitabh Joshi , Juan D. Serna

The problems of cavity atom optics in the presence of an external strong coherent field are formulated as the problems of potential scattering of doubly-dressed atomic wave packets. Two types of potentials produced by various multiphoton…

Quantum Physics · Physics 2009-11-07 Gagik Yu. Kryuchkyan

Time-resolved photoemission spectroscopy provides a unique and direct way to explore the real-time nonequilibrium dynamics of electrons and holes. The formal theory of the spectral function evolution requires inclusion of electronic…

Materials Science · Physics 2025-05-09 Thomas Blommel , Enrico Perfetto , Gianluca Stefanucci , Vojtěch Vlček

The latest molecular data - potential energy curves and Rydberg$/$valence interactions - characterizing the super-excited electronic states of CO are reviewed, in order to provide inputs for the study of their fragmentation dynamics.…

We expand iterative numerically-exact influence functional path-integral tools and present a method capable of following the nonequilibrium time evolution of subsystems coupled to multiple bosonic and fermionic reservoirs simultaneously.…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Lena Simine , Dvira Segal

The photochemistry of a molecular ensemble coupled to a resonance cavity and triggered by a femtosecond laser pulse is investigated from a real-time, quantum dynamics perspective with the multi-configuration time-dependent Hartree method.…

Chemical Physics · Physics 2018-06-20 Oriol Vendrell

The appearence of a new type of fast nonlinear traveling wave states in binary fluid convection with increasing Soret effect is elucidated and the parameter range of their bistability with the common slower ones is evaluated numerically.…

patt-sol · Physics 2009-10-30 St. Hollinger , P. Buechel , M. Luecke

Terahertz molecular motions are often probed by high-frequency molecular oscillators in different types of non-linear vibrational spectroscopy. Recently developed two-dimensional terahertz-infrared-visible spectroscopy allows direct…

Chemical Physics · Physics 2023-04-19 Pankaj Seliya , Mischa Bonn , Maksim Grechko

Scattering induced mode splitting in active microcavities is demonstrated. Below the lasing threshold, quality factor enhancement by optical gain allows resolving, in the wavelength-scanning transmission spectrum, the resonance dips of the…

Optics · Physics 2010-11-19 Lina He , Sahin Kaya Ozdemir , Jiangang Zhu , Lan Yang

Diffusing-wave spectroscopy is a powerful technique which consists in measuring the temporal correlation function of the intensity of light multiply scattered by a medium. In this paper, we apply this technique to cold atoms under purely…

Recent experiments in polariton chemistry have demonstrated that reaction rates can be modified by vibrational strong coupling to an optical cavity mode. Importantly, this modification only occurs when the frequency of the cavity mode is…

Chemical Physics · Physics 2023-05-15 Marit R. Fiechter , Johan E. Runeson , Joseph E. Lawrence , Jeremy O. Richardson

For a small fraction of hot CO2 molecules immersed in a liquid-phase CO2 thermal bath, classical cavity molecular dynamics simulations show that forming collective vibrational strong coupling (VSC) between the C=O asymmetric stretch of CO2…

Chemical Physics · Physics 2021-05-11 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

The quantum dynamics of vibrational polaritonic states arising from the interaction of a bistable molecule with the quantized mode of a Fabry-Perot microcavity is investigated using an asymmetric double-well potential as a simplified…

Chemical Physics · Physics 2024-01-11 Loïse Attal , Florent Calvo , Cyril Falvo , Pascal Parneix