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Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…

A laser pulse composed of a fundamental and an appropriately phased second harmonic can drive a time-dependent current of photoionized electrons that generates broadband THz radiation. Over the propagation distances relevant to many…

We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

Quantum Physics · Physics 2023-02-15 Marvin Reuner , Daria Popova-Gorelova

Attosecond pulses can be used to initiate and control electron dynamics on a sub-femtosecond time scale. The first step in this process occurs when an atom absorbs an ultraviolet photon leading to the formation of an attosecond electron…

Atomic Physics · Physics 2007-12-11 P. Johnsson , J. Mauritsson , T. Remetter , A. LHuillier , K. J. Schafer

We demonstrate a remarkably effective single-stage compression technique for ultrafast pulses in the visible electromagnetic spectrum using second-harmonic pulses at 515 nmderived from a 1030 nm Yb-based femtosecond regenerative amplifier.…

X-ray free-electron lasers (XFELs) as the world's brightest light sources provide ultrashort X-ray pulses with a duration typically in the order of femtoseconds. Recently, they have approached and entered the attosecond regime, which holds…

Generating ever-shorter and brighter light pulses has long been a central pursuit in ultrafast science, as it benchmarks our ability to create and manipulate the coherence on the intrinsic timescale of sub-atomic electron motion. The…

If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

A technique is proposed to generate attosecond pulse trains of radiation from a Free-Electron Laser amplifier. The optics-free technique synthesises a comb of longitudinal modes by applying a series of spatio-temporal shifts between the…

Optics · Physics 2008-11-26 N. R. Thompson , B. W. J. McNeil

Semiconductor quantum dots are excellent candidates for ultrafast coherent manipulation of qubits by laser pulses on picosecond timescales or even faster. In inhomogeneous ensembles a macroscopic optical polarization decays rapidly due to…

Mesoscale and Nanoscale Physics · Physics 2020-06-11 A. N. Kosarev , H. Rose , S. V. Poltavtsev , M. Reichelt , C. Schneider , M. Kamp , S. Hoefling , M. Bayer , T. Meier , I. A. Akimov

Frequency synthesis and spectro-temporal control of optical wave packets are central to ultrafast science, with supercontinuum (SC) generation standing as one remarkable example. Through passive manipulation, femtosecond (fs) pulses from…

Attosecond observations of coherent electron dynamics in molecules and nanostructures can be achieved by combining conventional scanning tunneling microscopy (STM) with ultrashort femtosecond laser pulses. While experimental studies in the…

Quantum Physics · Physics 2024-10-01 Boyang Ma , Michael Krüger

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

Temporal correlations in pulsed electron beams reflect the microscopic dynamics of emission and interparticle interaction. In femtosecond electron emission from nanoscale field emitters, Coulomb interactions result in structured…

Mesoscale and Nanoscale Physics · Physics 2025-05-16 Rudolf Haindl , Valerio Di Giulio , Armin Feist , Claus Ropers

Photoemission driven by a strong electric field of near-infrared or visible light, referred to as strong-field photoemission, produces attosecond electron pulses that are synchronized to the waveform of the incident light, and this…

We analyse the temporal properties of the optical pulse wave that is obtained by applying a set of spectral $\pi/2$ phase shifts to continuous-wave light that is phase-modulated by a temporal sinusoidal wave. We develop an analytical model…

Instruments to visualize transient structural changes of inhomogeneous materials on the nanometer scale with atomic spatial and temporal resolution are demanded to advance materials science, bioscience, and fusion sciences. One such…

Accelerator Physics · Physics 2017-03-20 X. Shen , R. K. Li , U. Lundström , T. J. Lane , A. H. Reid , S. P. Weathersby , X. J. Wang

Generation of ultrashort X-ray pulses in a free-electron laser relies on high-density electron bunches with a precisely adjusted current and energy distribution. To this end, robust and flexible electron bunch manipulation techniques are…

Accelerator Physics · Physics 2025-08-21 Ph. Amstutz , W. Helml , S. Khan , C. Mai , Ch. Gerth , Ch. Mahnke , E. A. Schneidmiller

Time-dependent nonlinear media, such as rapidly generated plasmas produced via laser ionization of gases, can increase the energy of individual laser photons and generate tunable high-order harmonic pulses. This phenomenon, known as photon…

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