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Free energy profiles serve as a fundamental bridge between microscopic atomic fluctuations and macroscopic thermodynamic observables. Estimating the free energy profile along a reaction coordinate, referred to as the potential of mean force…

Corrosion has a wide impact on society, causing catastrophic damage to structurally engineered components. An emerging class of corrosion-resistant materials are high-entropy alloys. However, high-entropy alloys live in high-dimensional…

Materials Science · Physics 2024-09-12 Cheng Zeng , Andrew Neils , Jack Lesko , Nathan Post

Federated learning (FL) necessitates that edge devices conduct local training and communicate with a parameter server, resulting in significant energy consumption. A key challenge in practical FL systems is the rapid depletion of…

Machine Learning · Computer Science 2025-06-24 Kai Zhang , Xuanyu Cao , Khaled B. Letaief

Federated learning enables a cluster of decentralized mobile devices at the edge to collaboratively train a shared machine learning model, while keeping all the raw training samples on device. This decentralized training approach is…

Machine Learning · Computer Science 2021-07-20 Young Geun Kim , Carole-Jean Wu

A data-driven model augmentation framework, referred to as Weakly-coupled Integrated Inference and Machine Learning (IIML), is presented to improve the predictive accuracy of physical models. In contrast to parameter calibration, this work…

Computational Engineering, Finance, and Science · Computer Science 2022-07-25 Vishal Srivastava , Valentin Sulzer , Peyman Mohtat , Jason B. Siegel , Karthik Duraisamy

The atomic structure of the most stable reconstructed surface of cuprous oxide (Cu$_{2}$O)(111) surface has been a longstanding topic of debate. In this study, we develop on-the-fly machine-learned force fields (MLFFs) to systematically…

Materials Science · Physics 2025-11-19 Payal Wadhwa , Michael Schmid , Georg Kresse

Federated Learning (FL) has emerged as a solution for distributed model training across decentralized, privacy-preserving devices, but the different energy capacities of participating devices (system heterogeneity) constrain real-world…

Machine Learning · Computer Science 2025-10-28 Roberto Pereira , Cristian J. Vaca-Rubio , Luis Blanco

The development of reliable and extensible molecular mechanics (MM) force fields -- fast, empirical models characterizing the potential energy surface of molecular systems -- is indispensable for biomolecular simulation and computer-aided…

The valence force field (VFF) model is a concise physical interpretation of the atomic interaction in terms of the bond and angle variations in the explicit quadratic functional form, while the machine learning (ML) method is a flexible…

Computational Physics · Physics 2018-08-07 Jing Wan , Ya-Wen Tan , Jin-Wu Jiang , Tienchong Chang , Xingming Guo

Reinforcement learning (RL) approaches based on Markov Decision Processes (MDPs) are predominantly applied in the robot joint space, often relying on limited task-specific information and partial awareness of the 3D environment. In…

Robotics · Computer Science 2026-03-09 Bingkun Huang , Yuhe Gong , Zewen Yang , Tianyu Ren , Luis Figueredo

Halide solid-state electrolytes have emerged as promising candidates for all-solid-state lithium batteries due to their high oxidative stability and deformability, yet their moderate ionic conductivity remains a bottleneck. While…

Materials Science · Physics 2026-02-02 Boyuan Xu , Chen Qian , Liyi Bai , Chenlu Wang , Feng Ding , Qisheng Wu

Federated learning (FL) and federated distillation (FD) are distributed learning paradigms that train UE models with enhanced privacy, each offering different trade-offs between noise robustness and learning speed. To mitigate their…

Machine Learning · Computer Science 2026-01-09 Yongjun Kim , Hyeongjun Park , Hwanjin Kim , Junil Choi

Accurate prediction of energy and forces for 3D molecular systems is one of fundamental challenges at the core of AI for Science applications. Many powerful and data-efficient neural networks predict molecular energies and forces from…

Chemical Physics · Physics 2026-04-23 Ali Mollahosseini , Mohammed Haroon Dupty , Wee Sun Lee

Federated learning (FL) is usually performed on resource-constrained edge devices, e.g., with limited memory for the computation. If the required memory to train a model exceeds this limit, the device will be excluded from the training.…

Machine Learning · Computer Science 2023-11-28 Kilian Pfeiffer , Ramin Khalili , Jörg Henkel

Realistic physical systems are characterised by emergent interactions across multiple length and time scales, posing a significant challenge for predictive machine learning (ML) models. Most scientific ML models focus on a narrow range of…

Understanding the mechanical properties of solid-state materials at the atomic scale is crucial for developing novel materials. For example, amorphous LiSi alloys are attractive anode materials for solid-state Li-ion batteries but face…

Disordered Systems and Neural Networks · Physics 2024-02-15 Zixiong Wei , Nongnuch Artrith

Machine learning (ML) based interatomic potentials are emerging tools for materials simulations but require a trade-off between accuracy and speed. Here we show how one can use one ML potential model to train another: we use an existing,…

Materials Science · Physics 2022-09-20 Joe D. Morrow , Volker L. Deringer

Point defects play a central role in driving the properties of materials. First-principles methods are widely used to compute defect energetics and structures, including at scale for high-throughput defect databases. However, these methods…

Machine Learning · Computer Science 2025-09-30 Evan Dramko , Yihuang Xiong , Yizhi Zhu , Geoffroy Hautier , Thomas Reps , Christopher Jermaine , Anastasios Kyrillidis

Abstract Machine learning models, trained on data from ab initio quantum simulations, are yielding molecular dynamics potentials with unprecedented accuracy. One limiting factor is the quantity of available training data, which can be…

Computational Physics · Physics 2020-06-11 Justin S. Smith , Nicholas Lubbers , Aidan P. Thompson , Kipton Barros

Meshfree simulation methods are emerging as compelling alternatives to conventional mesh-based approaches, particularly in the fields of Computational Fluid Dynamics (CFD) and continuum mechanics. In this publication, we provide a…

Machine Learning · Computer Science 2024-03-21 Paulami Banerjee , Mohan Padmanabha , Chaitanya Sanghavi , Isabel Michel , Simone Gramsch