Related papers: Spectroscopic evidence for possible quantum spin l…
Strong electron correlation drives 1T-TaS2 from a half-filled metallic state into a Mott insulating phase, coexisting with a charge density wave at low temperatures. Under external stimuli such as pressure or ionic gating, superconductivity…
Quantum spin liquids (QSLs) are highly entangled, disordered magnetic states that arise in frustrated Mott insulators and host exotic fractional excitations such as spinons and chargons. Despite being charge insulators some QSLs are…
Two-dimensional triangular-lattice antiferromagnets are predicted under some conditions to exhibit a quantum spin liquid ground state whose low-energy behavior is described by a spinon Fermi surface. Directly imaging the resulting spinons,…
The electrodynamic response of organic spin liquids with highly-frustrated triangular lattices has been measured in a wide energy range. While the overall optical spectra of these Mott insulators are governed by transitions between the…
Mott insulators are commonly pictured with electrons localized on lattice sites. Their low-energy degrees of freedom involve spins only. Here we observe emerging charge degrees of freedom in a molecule-based Mott insulator…
Magnetic structures of organic Mott insulators X[Pd(dmit)2]2 (X=Me4P, Me4Sb), of which electronic states are located near quantum spin liquid (X=EtMe3Sb), are demonstrated by 13C NMR. Antiferromagnetic spectra and nuclear relaxations show…
Quantum spin liquid (QSL) has become an exciting topic in interacting spin systems that do not order magnetically down to the lowest experimentally accessible temperature; however, conclusive experimental evidence remains lacking. Motivated…
Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are…
The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…
Strongly enhanced quantum fluctuations often lead to a rich variety of quantum-disordered states. A representative case is liquid helium, in which zero-point vibrations of the helium atoms prevent its solidification at low temperatures. A…
The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…
In Mott insulators, the strong electron-electron Coulomb repulsion prevents metallicity and charge excitations are gapped. In dimensions greater than one, their spins are usually ordered antiferromagnetically at low temperatures.…
1T-TaS$_2$ undergoes successive phase transitions upon cooling and eventually enters an insulating state of mysterious origin. Some consider this state to be a band insulator with interlayer stacking order, yet others attribute it to Mott…
In this paper, we study the non-magnetic insulator state near Mott transition of 2D pi-flux Hubbard model on square lattice and find that such non-magnetic insulator state is quantum spin liquid state with nodal fermionic excitations -…
Recent theoretical investigations of quantum spin liquids have described phenomenology amenable to experimental observation using scanning tunneling microscopy. This includes characteristic resonances found at the edge of the upper Hubbard…
Unique features of non-magnetic insulator phase are shown, and phase diagram for t-t' Hubbard model on square lattice is presented. Using the path-integral renormalization group method, we find antiferromagnetic phase for small next-nearest…
Mott state in 1T-TaS2 is predicted to host quantum spin liquids (QSL). However, its insulating mechanism is controversial due to complications from interlayer coupling. Here, we study the Mott state in monolayer 1T-NbSe2, an electronic…
The electronic structure of a quantum spin liquid compound, EtMe3Sb[Pd(dmit)2]2, has been studied with angle-resolved photoemission spectroscopy, together with two other Pd(dmit)2 salts in the valence bond solid or antiferromagnetic state.…
The quest for entangled spin excitations has stimulated intense research on frustrated magnetic systems. For almost two decades, the triangular-lattice Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been the hottest candidate for…
Correlated electrons often crystalize to the Mott insulator usually with some magnetic orders, whereas the "quantum spin liquid" has been a long-sought issue. We report numerical evidences that a nonmagnetic insulating (NMI) phase gets…