Related papers: Intermediate phases in $\alpha$-RuCl$_3$ under in-…
In this computational study, we explore a viable route to access the Kitaev-Quantum Spin Liquid (QSL) state in recently synthesized monolayer of a so-called spin-orbit assisted Mott insulator OsCl$_3$. In addition to other magnetic ground…
The quest for quantum spin liquids has garnered significant attention due to their rich physics and disruptive prospects in quantum communication and computation. Spin-orbit coupling, electron correlation, and structural distortion play…
RuCl$_3$ was likely the first ever deliberately synthesized ruthenium compound, following the discovery of the $_{44}$Ru element in 1844. For a long time it was known as an oxidation catalyst, with its physical properties being discrepant…
Kitaev materials are promising materials for hosting quantum spin liquids and investigating the interplay of topological and symmetry-breaking phases. We use an unsupervised and interpretable machine-learning method, the tensorial-kernel…
In this work, we investigate the microscopic nature of the magnetism in honeycomb iridium-based systems by performing a systematic study of how the effective magnetic interactions in these compounds depend on various electronic microscopic…
The theoretical inception of the Kitaev honeycomb model has had defining influence on the experimental hunt for quantum spin liquids, bringing unprecedented focus onto the synthesis of materials with bond-directional interactions. Numerous…
Layered $\alpha$-RuCl3 has been discussed as a proximate Kitaev spin liquid compound. Raman and THz spectroscopy of magnetic excitations confirm that the low-temperature antiferromagnetic ordered phase features a broad Raman continuum,…
The identification of quantum spin liquid phases in Kitaev candidate materials remains a major experimental challenge. Since most Kitaev candidates develop antiferromagnetic (AFM) order at low temperatures, currently there are great…
Very recently a quantum liquid was reported to form in H$_3$LiIr$_2$O$_6$, an iridate proposed to be a close realization of the Kitaev honeycomb model. To test this assertion we perform detailed quantum chemistry calculations to determine…
$\alpha$-RuCl$_3$ has attracted enormous attention since it has been proposed as a prime candidate to study fractionalized magnetic excitations akin to Kitaev's honeycomb-lattice spin liquid. We have performed a detailed specific-heat…
The 3$d^7$ Co$^{2+}$-based insulating magnet \NCTO{} has recently been reported to have strong Kitaev interactions on a honeycomb lattice, and is thus being considered as a Kitaev quantum spin liquid candidate. However, due to the existence…
The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…
In candidate Kitaev materials, the off-diagonal $\Gamma$ and $\Gamma'$ interactions are identified to come from the spin-orbit coupling and trigonal distortion, respectively. They have generated intense research efforts because of their…
Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…
We present high-resolution measurements of the thermal expansion and the magnetostriction of TlCuCl$_{3}$ which shows field-induced antiferromagnetic order. We find pronounced anomalies in the field and temperature dependence of different…
While the existence of a spin-liquid ground state of the spin-1/2 kagome Heisenberg antiferromagnet (KHAF) is well established, the discussion of the effect of an interlayer coupling (ILC) by controlled theoretical approaches is still…
We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…
Kitaev iridates have been proposed as candidates for realizing an elusive quantum spin liquid (QSL) state, in which strong spin-orbit coupling and bond-directional exchange generate a highly frustrated and entangled ground state. However,…
Heat transport mediated by Majorana edge modes in a magnetic insulator leads to a half-integer thermal quantum Hall conductance, which has recently been reported for the two-dimensional honeycomb material $\alpha$-RuCl$_3$. While the…
We report the existence of a phase transition at high temperature in the 3D Kitaev candidate material, $\beta$-Li$_2$IrO$_3$. We show that the transition is bulk, intrinsic and orders a tiny magnetic moment with a spatially anisotropic…