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Femtosecond time-resolved x-ray diffraction is employed to study the dynamics of the periodic lattice distortion (PLD) associated with the charge-density-wave (CDW) in K0.3MoO3. Using a multi-pulse scheme we show the ability to extend the…

We introduce and demonstrate a new approach to measuring coherent electron wave packets using high-harmonic spectroscopy. By preparing a molecule in a coherent superposition of electronic states, we show that electronic coherence opens…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , S. B. Zhang , A. Gijsbertsen , R. R. Lucchese , N. Rohringer , H. J. Wörner

The elimination of defects from SiC has facilitated its move to the forefront of the optoelectronics and power-electronics industries. Nonetheless, because the electronic states of SiC defects can have sharp optical and spin transitions,…

We propose and study the use of photon-mediated interactions for the generation of long-range steady-state entanglement between N atoms. Through the judicious use of coherent drives and the placement of the atoms in a network of Cavity QED…

Quantum Physics · Physics 2016-03-25 Camille Aron , Manas Kulkarni , Hakan E. Türeci

Developing efficient path integral (PI) methods for atomistic simulations of vibrational spectra in heterogeneous condensed phases and interfaces has long been a challenging task. Here, we present the h-CMD method, short for hybrid centroid…

Chemical Physics · Physics 2025-05-08 Dil K. Limbu , Nathan London , Md Omar Faruque , Mohammad R. Momeni

We investigate the coherence properties of individual nuclear spin quantum bits in diamond [Dutt et al., Science, 316, 1312 (2007)] when a proximal electronic spin associated with a nitrogen-vacancy (NV) center is being interrogated by…

High harmonic emissions from crystalline solids contain rich information on the dynamics of electrons driven by intense infrared laser fields and have been intensively studied owing to their potential use as a probe of microscopic…

Materials Science · Physics 2023-05-01 K. Uchida , K. Tanaka

Achieving long-range ferrimagnetic order in purely organic systems remains a major challenge in molecular magnetism. Here we report the synthesis and characterization of heterospin-coupling motifs, formed by covalently linking spin-1/2 and…

Mesoscale and Nanoscale Physics · Physics 2026-04-10 Elia Turco , Fupeng Wu , Annika Bernhardt , Nils Krane , Ji Ma , Roman Fasel , Michal Juriček , Xinliang Feng , Pascal Ruffieux

Quantum mechanical phenomena, such as electronic coherence and entanglement, play a key role in achieving the unrivalled efficiencies of light-energy conversion in natural photosynthetic light-harvesting complexes, and triggered the growing…

Quantum Physics · Physics 2011-02-02 Richard Hildner , Daan Brinks , Niek F. van Hulst

We report an investigation to establish the physical mechanisms responsible for decoherence in the generation of photon pairs from atomic ensembles, via the protocol of Duan et. al for long distance quantum communication [Nature (London)…

Quantum Physics · Physics 2009-11-11 D. Felinto , C. W. Chou , H. de Riedmatten , S. V. Polyakov , H. J. Kimble

Decoherence for a one-dimensional coupled-resonator waveguide with a two-level system inside one of resonators, induced by their interaction with corresponding environments, is investigated. Each environment is modeled as a continuum of…

Quantum Physics · Physics 2015-05-19 Jing Lu , Lan Zhou , H. C. Fu , Le-Man Kuang

Coherent wave control exploits the interference among multiple waves impinging on a system to suppress or enhance outgoing signals based on their relative phase and amplitude. This process inherently requires non-Hermiticity, in order to…

Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…

Mesoscale and Nanoscale Physics · Physics 2016-04-14 M. Hohenleutner , F. Langer , O. Schubert , M. Knorr , U. Huttner , S. W. Koch , M. Kira , R. Huber

Erbium-doped solids are prime candidates for optical quantum communication networks due to erbium's telecom C-band emission. A long-lived electron spin of erbium with millisecond coherence time is highly desirable for establishing…

Quantum Physics · Physics 2023-10-16 Shobhit Gupta , Xuntao Wu , Haitao Zhang , Jun Yang , Tian Zhong

A remarkable amount of theoretical research has been carried out to elucidate the physical origins of the recently observed long-lived quantum coherence in the electronic energy transfer process in biological photosynthetic systems.…

Quantum Physics · Physics 2015-03-19 Sangwoo Shim , Patrick Rebentrost , Stéphanie Valleau , Alan Aspuru-Guzik

Quantum technologies are built on the power of coherent superposition. Atomic coherence is typically generated from optical coherence, most often via Rabi oscillations. However, canonical coherent states of light create imperfect resources;…

Quantum Physics · Physics 2020-11-03 Aaron Z. Goldberg , Aephraim M. Steinberg

Coherent electrons coupled to the quantized electromagnetic field undergo decoherence which can be viewed as due either to fluctuations of the Aharonov-Bohm phase or to photon emission. When the electromagnetic field is in a squeezed vacuum…

Quantum Physics · Physics 2009-01-09 Jen-Tsung Hsiang , L. H. Ford

In this Letter we show that the strong coupling between a disordered set of molecular emitters and surface plasmons leads to the formation of spatially coherent hybrid states extended on acroscopic distances. Young type interferometric…

We propose and investigate a hybrid optomechanical system consisting of a micro-mechanical oscillator coupled to the internal states of a distant ensemble of atoms. The interaction between the systems is mediated by a light field which…

Quantum Physics · Physics 2015-04-28 B. Vogell , T. Kampschulte , M. T. Rakher , A. Faber , P. Treutlein , K. Hammerer , P. Zoller

Optical imaging plays a critical role in advancing our understanding of three dimensional dynamics of biological systems. Coherent imaging (CI) methods exploit spatial phase information, encoded through propagation of coherent signal light…

Optics · Physics 2015-07-24 Jeffrey J. Field , David G. Winters , Randy A. Bartels
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