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The Doyle-Fuller-Newman framework is the most popular physics-based continuum-level description of the chemical and dynamical internal processes within operating lithium-ion-battery cells. With sufficient flexibility to model a wide range…

The pseudo-4D Doyle-Fuller-Newman (DFN) model enables predictive simulation of lithium-ion batteries with three-dimensional electrode architectures and particle-scale diffusion, extending the standard pseudo-2D (P2D) formulation to fully…

Accurately predicting aging of lithium-ion batteries would help to prolong their lifespan, but remains a challenge owing to the complexity and interrelation of different aging mechanisms. As a result, aging prediction often relies on…

Parameterisation of coupled degradation mechanisms in lithium-ion batteries is a major challenge. Interactions between the mechanisms depend on usage conditions: C-rate, rest state-of-charge (SoC), depth-of-discharge (DoD) and temperature.…

Materials Science · Physics 2026-04-13 Ganesh Madabattula

Heterogeneities in lithium ion batteries can be significant factors in electrode under utilisation and degradation while charging. Bilayer electrodes have been proposed as a convenient and scalable way to homogenise the electrode response.…

Dynamical Systems · Mathematics 2025-11-11 E. C. Tredenick , A. M. Boyce , R. Drummond , S. R. Duncan

Growing demand for fast charging and optimised battery designs is fuelling significant interest in electrochemical models of Li-ion batteries. However, estimating parameter values for these models remains a major challenge. In this paper, a…

Systems and Control · Electrical Eng. & Systems 2020-12-04 Ross Drummond , Stephen R. Duncan

The physics-based Doyle-Fuller-Newman (DFN) model, widely adopted for its precise electrochemical modeling, stands out among various simulation models of lithium-ion batteries (LIBs). Although the DFN model is powerful in forward predictive…

Computational Engineering, Finance, and Science · Computer Science 2025-04-30 Weipeng Xu , Kaiqi Yang , Yuzhi Zhang , Shichao Sun , Sheng Mao , Tianju Xue

The standard continuum model of a lithium-ion battery, the Doyle-Fuller-Newman (DFN) model, is computationally expensive to solve. Typically simpler models, such as the single particle model (SPM), are used to provide insight for control…

Chemical Physics · Physics 2019-11-07 Scott G. Marquis , Valentin Sulzer , Robert Timms , Colin P. Please , S. Jon Chapman

Battery health assessment and recuperation play a crucial role in the utilization of second-life Li-ion batteries. However, due to ambiguous aging mechanisms and lack of correlations between the recovery effects and operational states, it…

Signal Processing · Electrical Eng. & Systems 2024-04-04 Riko I Made , Jing Lin , Jintao Zhang , Yu Zhang , Lionel C. H. Moh , Zhaolin Liu , Ning Ding , Sing Yang Chiam , Edwin Khoo , Xuesong Yin , Guangyuan Wesley Zheng

Accurate battery lifetime prediction is important for preventative maintenance, warranties, and improved cell design and manufacturing. However, manufacturing variability and usage-dependent degradation make life prediction challenging.…

Machine Learning · Computer Science 2024-04-23 Tingkai Li , Zihao Zhou , Adam Thelen , David Howey , Chao Hu

In this study we construct a data-driven model describing Lithium plating in a battery cell, which is a key process contributing to degradation of such cells. Starting from the fundamental Doyle-Fuller-Newman (DFN) model, we use asymptotic…

Chemical Physics · Physics 2024-08-28 Avesta Ahmadi , Kevin J. Sanders , Gillian R. Goward , Bartosz Protas

Battery aging is a natural process that contributes to capacity and power fade, resulting in a gradual performance degradation over time and usage. State of Charge (SOC) and State of Health (SOH) monitoring of an aging battery poses a…

Systems and Control · Electrical Eng. & Systems 2021-06-25 Anirudh Allam , Simona Onori

This work presents a comprehensive study on the aging behavior of 18650-type lithium-ion batteries, focusing on the uneven intercalation of lithium ions during fast charging processes. It introduces a novel approach using color visual…

Materials Science · Physics 2025-04-17 Yihan Shi , Qingrui Pan , Jitao Li , Xiaoze Shi , Youchang Wang , Peng Xiao

Accurately predicting the lifespan of lithium-ion batteries is crucial for optimizing operational strategies and mitigating risks. While numerous studies have aimed at predicting battery lifespan, few have examined the interpretability of…

Machine Learning · Computer Science 2024-04-12 Jaewook Lee , Seongmin Heo , Jay H. Lee

Batteries are ubiquitous today, with applications ranging from smartphones, watches, and laptops to electric cars, drones, and electric aircraft. Lithium-ion batteries are widely used in these applications due to their high energy density,…

Computational Engineering, Finance, and Science · Computer Science 2026-03-03 Vikram C Patil

The Doyle-Fuller-Newman model is arguably the most ubiquitous electrochemical model in lithium-ion battery research. Since it is a highly nonlinear model, its input-output relations are still poorly understood. Researchers therefore often…

Battery degradation, which is the reduction of performance over time, is one of the main roadblocks to the wide deployment of lithium-ion batteries. Physics-based models, such as those based on the Doyle-Fuller-Newman model, are invaluable…

Chemical Physics · Physics 2023-06-06 Ferran Brosa Planella , W. Dhammika Widanage

Present theories of irreversible energy losses and heat generation within Li-ion cells are unsatisfactory because they are not compatible with energy conservation. This work aims to provide a consistent theoretical treatment of energy…

Applied Physics · Physics 2021-08-20 G. Richardson , I. Korotkin

Accurate assessment of lithium-ion battery ageing is challenged by cell-to-cell variability, heterogeneous cycling protocols, and limited transferability of data-driven models across datasets. In particular, robust identification of…

Machine Learning · Computer Science 2026-04-21 Agnieszka Pregowska , Stefan Marynowicz

Batteries are dynamic systems with complicated nonlinear aging, highly dependent on cell design, chemistry, manufacturing, and operational conditions. Prediction of battery cycle life and estimation of aging states is important to…

Systems and Control · Electrical Eng. & Systems 2024-10-11 Joachim Schaeffer , Giacomo Galuppini , Jinwook Rhyu , Patrick A. Asinger , Robin Droop , Rolf Findeisen , Richard D. Braatz
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