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Multilayered van der Waals structures often lack periodicity, which difficults their modeling. Building on previous work for bilayers, we develop a tight-binding based, momentum space formalism capable of describing incommensurate…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 B. Amorim , Eduardo V. Castro

Van der Waals (vdW) heterostructures ---formed by stacking or growing two-dimensional (2D) crystals on top of each other--- have emerged as a new promising route to tailor and engineer the properties of 2D materials. Twisted bilayer…

Mesoscale and Nanoscale Physics · Physics 2020-08-05 G. Catarina , B. Amorim , Eduardo V. Castro , J. M. Viana Parente Lopes , N. M. R. Peres

We determined a full 3D atomic structure of a dumbbell-shaped Pt nanoparticle formed by a coalescence of two nanoclusters using deep learning assisted atomic electron tomography. Formation of double twin boundary was clearly observed at the…

Materials Science · Physics 2022-02-09 Juhyeok Lee , Chaehwa Jeong , Yongsoo Yang

We investigate imaging of moire structures in free-standing twisted bilayer graphene (TBG) carried out by transmission electron microscopy (TEM) in diffraction and in-line Gabor holography modes. Electron diffraction patterns of TBG…

Mesoscale and Nanoscale Physics · Physics 2018-11-30 Tatiana Latychevskaia , Conrad Escher , Hans-Werner Fink

Convergent beam electron diffraction is routinely applied for studying deformation and local strain in thick crystals by matching the crystal structure to the observed intensity distributions. Recently, it has been demonstrated that CBED…

Mesoscale and Nanoscale Physics · Physics 2020-03-31 Tatiana Latychevskaia , Colin Robert Woods , Yi Bo Wang , Matthew Holwill , Eric Prestat , Sarah J. Haigh , Kostya S. Novoselov

Graphene is a truly two-dimensional atomic crystal with exceptional electronic and mechanical properties. Whereas conventional bulk and thin-film materials have been studied extensively, the key mechanical properties of graphene, such as…

Materials Science · Physics 2010-05-25 Dipanjan Sen , Kostya S. Novoselov , Pedro M. Reis , Markus J. Buehler

From ripples to defects, edges and grain boundaries, the 3D atomic structure of 2D materials is critical to their properties. However the damage inflicted by conventional 3D analysis precludes its use with fragile 2D materials, particularly…

Applied Physics · Physics 2022-06-22 Christoph Hofer , Kimmo Mustonen , Viera Skakalova , Timothy J. Pennycook

Chemical bonding in 2D layered materials and van der Waals solids is central to understanding and harnessing their unique electronic, magnetic, optical, thermal and superconducting properties. Here we report the discovery of spontaneous,…

Nanomaterials with core-shell architectures are prominent examples of strain-engineered materials, where material properties can be designed by fine-tuning the misfit strain at the interface. Here, we elucidate the full 3D atomic structure…

Allotropes of carbon, including one-dimensional carbon nanotubes and two-dimensional graphene sheets, continue to draw attention as promising platforms for probing the physics of electrons in lower dimensions. Recent research has shown that…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Benedetta Flebus , Allan H. MacDonald

Grain boundaries (GBs) in complex oxides play critical roles in governing their functional properties, which are intrinsically linked to their three-dimensional (3D) atomic configurations and local chemical environments that can deviate…

We present a scheme of the high-precise three-dimensional (3D) localization by the measurement of the atomic-level population. The scheme is applied to a four-level tripod-type atom coupled by three strong standing waves and a probe running…

Atomic Physics · Physics 2014-12-10 Vladimir S. Ivanov , Yuri V. Rozhdestvensky , Kalle-Antti Suominen

By virtue of being atomically thin, the electronic properties of heterostructures built from two-dimensional materials are strongly influenced by atomic relaxation. The atomic layers behave as flexible membranes rather than rigid crystals.…

Strongly Correlated Electrons · Physics 2025-01-07 Mohammed M. Al Ezzi , Gayani N. Pallewela , Christophe De Beule , E. J. Mele , Shaffique Adam

We investigate bilayers of nanoporous graphene (NPG), laterally bonded carbon nanoribbons, and graphene. The electronic and transport properties are explored as a function of the interlayer twist angle using an atomistic tight-binding model…

Mesoscale and Nanoscale Physics · Physics 2024-08-12 Xabier Diaz de Cerio , Aleksander Bach Lorentzen , Mads Brandbyge , Aran Garcia-Lekue

An uncertainty in studying twisted bilayer graphene (TBG) is the minimum energy geometry, which strongly affects the electronic structure. The minimum energy geometry is determined by the potential energy surface, which is dominated by van…

Mesoscale and Nanoscale Physics · Physics 2023-11-14 Kittithat Krongchon , Tawfiqur Rakib , Shivesh Pathak , Elif Ertekin , Harley T. Johnson , Lucas K. Wagner

Two-dimensional materials are expected to play an important role in next-generation electronics and optoelectronic devices. Recently, twisted bilayer graphene and transition metal dichalcogenides have attracted significant attention due to…

Imposing incommensurable periodicity on the periodic atomic lattice can lead to complex structural phases consisting of locally periodic structure bounded by topological defects. Twisted trilayer graphene (TTG) is an ideal material platform…

Staking layered materials revealed to be a very powerful method to tailor their electronic properties. It has indeed been theoretically and experimentally shown that twisted bilayers of graphene (tBLG) with a rotation angle $\theta$,…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Omid Faizy Namarvar , Ahmed Missaoui , Laurence Magaud , Didier Mayou , Guy Trambly de Laissardière

Moir\'e materials, and in particular twisted bilayer graphene (TBG), exhibit a range of fascinating phenomena, that emerge from the interplay of band topology and interactions. We show that the non-linear second-order photoresponse is an…

Mesoscale and Nanoscale Physics · Physics 2021-07-21 Swati Chaudhary , Cyprian Lewandowski , Gil Refael

Twist, as a simple and unique degree of freedom, could lead to enormous novel quantum phenomena in bilayer graphene. A small rotation angle introduces low-energy van Hove singularities (VHSs) approaching the Fermi level, which result in…

Materials Science · Physics 2018-02-07 Wei-Jie Zuo , Jia-Bin Qiao , Dong-Lin Ma , Long-Jing Yin , Gan Sun , Jun-Yang Zhang , Li-Yang Guan , Lin He