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Methods for estimating the correlation energy of molecules and other electronic systems are discussed based on the assumption that the correlation energy can be partitioned between atomic regions. In one method, the electron density is…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

The non-relativistic electronic Hamiltonian, H(a)= Hkin + Hne + aHee, extended with coupling strength parameter (a), allows to switch the electron-electron repulsion energy off and on. First, the easier a=0 case is solved and the solution…

Chemical Physics · Physics 2019-10-08 Sandor Kristyan

The computation of the three-particle correlation function involving three hadrons started just recently after the first publications of ALICE measurements. Key elements to be considered are the correct description of the asymptotics,…

Nuclear Theory · Physics 2025-05-29 E. Garrido , A. Kievsky , R. Del Grande , L. Serksnyte , M. Viviani , L. E. Marcucci

We explore the robustness of the correlation matrix Hamiltonian reconstruction technique with respect to the choice of operator basis, studying the effects of bases that are undercomplete and over-complete -- too few or too many operators…

Strongly Correlated Electrons · Physics 2024-09-12 Lucas Z. Brito , Stephen Carr , J. Alexander Jacoby , J. B. Marston

I explore the form of the effective interaction in harmonic-oscillator-based effective theory (HOBET) in next-to-next-to-next-to-leading order (N3LO). As the included space in a HOBET (as in the shell model) is defined by the oscillator…

Nuclear Theory · Physics 2009-11-13 W. C. Haxton

Representing a strongly interacting multi-particle wave function in a finite product basis leads to errors. Simple rescaling of the contact interaction can preserve the low-lying energy spectrum and long-wavelength structure of wave…

Quantum Gases · Physics 2011-08-23 Thomas Ernst , David W. Hallwood , Jake Gulliksen , Hans-Dieter Meyer , Joachim Brand

An enhanced static approximation for the electron self energy operator is proposed for efficient calculation of quasiparticle energies. Analysis of the static COHSEX approximation originally proposed by Hedin shows that most of the error…

Materials Science · Physics 2010-11-18 Wei Kang , Mark S. Hybertsen

We investigate the possibility of using a transcorrelated Hamiltonian to describe electron correlation. Amethod to obtain transcorrelatedwavefunctionswas developed based on the mathematical framework of the bi-variational principle. This…

Chemical Physics · Physics 2024-07-23 Nicholas Lee , Alex J. W. Thom

An electrodynamical coupled cluster (CC) methodology starting from a covariant formalism and an equal time approximation, and finally based on the Dirac-Fock picture of the electron and positron fields and Coulomb gauge, is given here. The…

Atomic Physics · Physics 2019-04-30 Sambhu N. Datta

The Coulomb exchange and correlation energy density functionals for electron systems are applied to nuclear systems. It is found that the exchange functionals in the generalized gradient approximation provide agreements with the exact-Fock…

Nuclear Theory · Physics 2019-12-09 Tomoya Naito , Ryosuke Akashi , Gianluca Colò , Haozhao Liang , Xavier Roca-Maza

We discuss the problem of gauge fixing for strongly correlated electrons coupled to quantum light, described by projected low-energy models such as those obtained within tight-binding methods. Drawing from recent results in the field of…

Strongly Correlated Electrons · Physics 2021-03-12 Olesia Dmytruk , Marco Schiró

This paper investigates the influence of the basis set on the GW self-energy correction in the full-potential linearized augmented-plane-wave (LAPW) approach and similar linearized all-electron methods. A systematic improvement is achieved…

Materials Science · Physics 2007-05-23 Christoph Friedrich , Arno Schindlmayr , Stefan Blügel , Takao Kotani

The main task of an energy calibration is to find a relation between pulse-height values and the corresponding energies. Doing this for each pulse-height channel individually requires an elaborated input spectrum with an excellent counting…

Instrumentation and Detectors · Physics 2016-02-17 Daniel Maier , Olivier Limousin

A variational approach is used to calculate free energy and conformational properties in polyelectrolytes. The true bond and Coulomb potentials are approximated by a trial isotropic harmonic energy containing monomer-monomer force constants…

High Energy Physics - Lattice · Physics 2009-09-25 B. Jönsson , C. Peterson , B. Söderberg

An eikonal expansion is developed in order to provide systematic corrections to the eikonal approximation through order 1/k^2, where k is the wave number. The expansion is applied to wave functions for the Klein-Gordon equation and for the…

Nuclear Theory · Physics 2011-07-19 J. A. Tjon , S. J. Wallace

Very recently, we introduced a set of correlation consistent effective core potentials (ccECPs) constructed within full many-body approaches. By employing significantly more accurate correlated approaches we were able to reach a new level…

Materials Science · Physics 2020-02-25 Abdulgani Annaberdiyev , Cody A. Melton , M. Chandler Bennett , Guangming Wang , Lubos Mitas

Continuum states of the Dirac equation are calculated numerically for the electrostatic field generated by the charge distribution of an atomic nucleus. The behavior of the wave functions of an incoming electron with a given asymptotic…

Nuclear Theory · Physics 2007-05-23 Andreas Aste , Cyrill von Arx , Dirk Trautmann

Methods for correcting residual energy errors of configuration interaction (CI) calculations of molecules and other electronic systems are discussed based on the assumption that the energy defect can be mapped onto atomic regions. The…

Chemical Physics · Physics 2022-10-05 Jerry L. Whitten

We present the effective Hamiltonian for an electron-nucleus interaction in non-relativistic limit up to the second order in the inverse nucleon mass. This Hamiltonian takes into account the distortion of electron waves and allows to…

Nuclear Theory · Physics 2007-05-23 R. Ya. Kezerashvili

A simple formula for correlation energy $E_c$ of the $\pi$ electron systems is obtained under an approximation for the electron-electron interactions. This formula is related directly to square of the bond order matrix and the…

Other Condensed Matter · Physics 2007-05-23 Hua Zhao
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