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Related papers: Mitigating decoherence in molecular spin qudits

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Molecular Nanomagnets may enable the implementation of qudit-based quantum error-correction codes which exploit the many spin levels naturally embedded in a single molecule, a promising step towards scalable quantum processors. To fully…

The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…

Quantum Physics · Physics 2025-04-28 Conor Ryan , Valerio Briganti , Cathal Hogan , Mark O'Neill , Alessandro Lunghi

Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise…

Quantum Physics · Physics 2026-05-06 Timothy J. Krogmeier , James Bradley , Anthony W. Schlimgen , Kade Head-Marsden

We investigate decoherence due to pure dephasing of a localized spin qubit interacting with a nuclear spin bath. Although in the limit of a very large magnetic field the only decoherence mechanism is spectral diffusion due to dipolar…

Mesoscale and Nanoscale Physics · Physics 2009-06-18 L. Cywinski , W. M. Witzel , S. Das Sarma

We briefly review the oscillator and spin bath models of quantum environments, which can be used to describe the low-energy dynamics of open quantum systems. We then use them to discuss both the mechanisms causing decoherence at low $T$,…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 M. Dube , P. C. E. Stamp

Decoherence in Nature has become one of the most pressing problems in physics. Many applications, including quantum information processing, depend on understanding it; and fundamental theories going beyond quantum mechanics have been…

Mesoscale and Nanoscale Physics · Physics 2011-07-27 S. Takahashi , I. S. Tupitsyn , J. van Tol , C. C. Beedle , D. N. Hendrickson , P. C. E. Stamp

Quantum states are described by wave functions whose phases cannot be directly measured, but which play a vital role in quantum effects such as interference and entanglement. The loss of the relative phase information, termed decoherence,…

Chemical Physics · Physics 2019-12-20 Jia Chen , Cong Hu , John F. Stanton , Stephen Hill , Hai-Ping Cheng , Xiao-Guang Zhang

We investigate pure dephasing decoherence (free induction decay and spin echo) of a spin qubit interacting with a nuclear spin bath. While for infinite magnetic field B the only decoherence mechanism is spectral diffusion due to dipolar…

Mesoscale and Nanoscale Physics · Physics 2009-02-03 L. Cywinski , W. M. Witzel , S. Das Sarma

Molecular spins are promising candidates for quantum information science, leveraging coherent electronic spin states for quantum sensing and computation. However, the practical application of these systems is hindered by electronic spin…

Quantum Physics · Physics 2026-03-03 Timothy J. Krogmeier , Anthony W. Schlimgen , Kade Head-Marsden

The decoherence of mixed electron-nuclear spin qubits is a topic of great current importance, but understanding is still lacking: while important decoherence mechanisms for spin qubits arise from quantum spin bath environments with slow…

Mesoscale and Nanoscale Physics · Physics 2015-05-26 S. J. Balian , Gary Wolfowicz , John J. L. Morton , T. S. Monteiro

The prospect of developing magnetic qubits is discussed. The first part of the article makes suggestions on how to achieve the coherent quantum superposition of spin states in small ferromagnetic clusters, weakly uncompensated…

Statistical Mechanics · Physics 2007-05-23 Eugene M. Chudnovsky

The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules…

Spin decoherence poses a significant challenge in molecular magnets, with the nuclear spin bath serving as a prominent source. Intriguingly, spin qubits at the clock transition exhibit remarkable insensitivity to the surrounding nuclear…

Quantum Physics · Physics 2025-10-14 Xiao Chen , Haechan Park , Silas Hoffman , Shuanglong Liu , Hai-Ping Cheng

This mini-review presents a simple and accessible summary on the fascinating physics of quantum nanomagnets coupled to a nuclear spin bath. These chemically synthesized systems are an ideal test ground for the theories of decoherence in…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Andrea Morello

There are several important solid-state systems, such as defects in solids, superconducting circuits and molecular qubits, for attractive candidates of quantum computations. Molecular qubits, which benefit from the power of chemistry for…

Quantum Physics · Physics 2017-06-29 Yingqiu Dai , Zhifu Shi , Yue Fu , Xi Qin , Shiwei Mu , Yang Wu , Ji-Hu Su , Lei Qin , Yuan-Qi Zhai , Yi-Fei Deng , Xing Rong , Jiangfeng Du

Interaction of solid state qubits with environmental degrees of freedom strongly affects the qubit dynamics, and leads to decoherence. In quantum information processing with solid state qubits, decoherence significantly limits the…

Mesoscale and Nanoscale Physics · Physics 2010-02-26 Luca Chirolli , Guido Burkard

In many realizations of electron spin qubits the dominant source of decoherence is the fluctuating nuclear spin bath of the host material. The slowness of this bath lends itself to a promising mitigation strategy where the nuclear spin bath…

Mesoscale and Nanoscale Physics · Physics 2010-11-30 Hendrik Bluhm , Sandra Foletti , Diana Mahalu , Vladimir Umansky , Amir Yacoby

The realisation of quantum computers based on molecular electronic spins requires the design of qubits with very long coherence times, T2. Dephasing can proceed over several different microscopic pathways, active at the same time and in…

Materials Science · Physics 2020-01-08 Alessandro Lunghi , Stefano Sanvito

Decoherence of electron spins in nanoscale systems is important to quantum technologies such as quantum information processing and magnetometry. It is also an ideal model problem for studying the crossover between quantum and classical…

Mesoscale and Nanoscale Physics · Physics 2017-03-06 Wen Yang , Wen-Long Ma , Ren-Bao Liu

The realization of spin-based logical gates crucially depends on magnetically-coupled spin qubits. Thus, understanding decoherence when spin qubits are in close proximity will become a roadblock to overcome. Herein, we provide a general…

Mesoscale and Nanoscale Physics · Physics 2019-08-21 L. Escalera-Moreno , A. Gaita-Ariño , E. Coronado
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