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We propose an alternative formulation of the sensor method presented in [Phys. Rev. Lett 109, 183601 (2012)] for the calculation of frequency-filtered and time-resolved photon correlations. Our approach is based on an algebraic expansion of…

Quantum Physics · Physics 2018-12-26 David I. H. Holdaway , Valentina Notararigo , Alexandra Olaya-Castro

We describe a method to probe the spectral fluctuations of a transition over broad ranges of frequencies and timescales with the high spectral resolution of Fourier spectroscopy, and a temporal resolution as high as the excited state…

Photon correlations are a cornerstone of Quantum Optics. Recent works [NJP 15 025019, 033036 (2013), PRA 90 052111 (2014)] have shown that by keeping track of the frequency of the photons, rich landscapes of correlations are revealed.…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 A. Gonzalez-Tudela , E. del Valle , F. P. Laussy

In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…

Quantum Physics · Physics 2026-04-24 Arunangshu Debnath , Shaul Mukamel

Frequency-resolved photon correlations have proven to be a useful resource to unveil nonlinearities hidden in standard observables such as the spectrum or the standard (color-blind) photon correlations. In this manuscript, we analyze the…

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

Quantum light is increasingly recognized as a promising resource for developing optical measurement techniques. Particular attention has been paid to enhancing the precision of the measurements beyond classical techniques by using…

Chemical Physics · Physics 2023-10-03 Yuta Fujihashi , Kuniyuki Miwa , Masahiro Higashi , Akihito Ishizaki

We summarise the main results that follow from our theory of frequency- and time-resolved photon correlations, which provides exact computations in nontrivial systems. We illustrate the theory with original results as interesting cases can…

Quantum Physics · Physics 2018-03-05 Juan Camilo López Carreño , Elena del Valle , Fabrice P. Laussy

We demonstrate quantum interference of three photons that are distinguishable in time, by resolving them in the conjugate parameter, frequency. We show that the multiphoton interference pattern in our setup can be manipulated by tuning the…

We investigate two-color photon correlations in the light emitted by strongly coupled two-level emitters. Spectral filtering allows us to manipulate the collected light statistics and we show that the resonances induced by dipole-dipole…

Quantum Physics · Physics 2021-05-12 Elnaz Darsheshdar , Mathilde Hugbart , Romain Bachelard , Celso Jorge Villas-Boas

We develop a formalism based on a time-dependent wave-function ansatz to study correlations of photons emitted from a collection of two-level quantum emitters. We show how to simulate the system dynamics and evaluate the intensity of the…

A common challenge in quantum information processing with photons is the limited ability to manipulate and measure correlated states. An example is the inability to measure picosecond scale temporal correlations of a multi-photon state,…

In this work we investigate quantum-enhanced target detection in the presence of large background noise using multidimensional quantum correlations between photon pairs generated through spontaneous parametric down-conversion. Until now…

The development of spectroscopic techniques able to detect and verify quantum coherence is a goal of increasing importance given the rapid progress of new quantum technologies, the advances in the field of quantum thermodynamics, and the…

Quantum Physics · Physics 2020-05-27 Carlos Sánchez Muñoz , Frank Schlawin

Spectrally correlated photon pairs can be used to improve performance of long range fiber based quantum communication protocols. We present a source based on spontaneous parametric down-conversion producing polarization entangled photons…

Optics · Physics 2014-03-28 Thomas Lutz , Piotr Kolenderski , Thomas Jennewein

We apply our recently developed theory of frequency-filtered and time-resolved N-photon correlations to study the two-photon spectra of a variety of systems of increasing complexity: single mode emitters with two limiting statistics (one…

Quantum Physics · Physics 2014-03-06 A. Gonzalez-Tudela , F. P. Laussy , C. Tejedor , M. J. Hartmann , E. del Valle

Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…

The excited state population of single solid-state emitters is subjected to energy fluctuations around the equilibrium driven by the bath and relaxation through the emission of phonons or photons. Simultaneous measurement of the associated…

Quantum Physics · Physics 2021-05-12 Hendrik Utzat , Moungi G. Bawendi

A theory of correlations between N photons of given frequencies and detected at given time delays is presented. These correlation functions are usually too cumbersome to be computed explicitly. We show that they are obtained exactly through…

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