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With a view towards optimizing gas storage and separation in crystalline and disordered nanoporous carbon-based materials, we use ab initio density functional theory calculations to explore the effect of chemical functionalization on gas…

The electronic, thermal and optical properties of a monolayer BeO with Boron (B) and Nitrogen (N) co-dopant atoms are studied by means of a density functional theory computation. Our calculations reveal that BeO with BN-codopant atoms can…

Materials Science · Physics 2022-01-07 Nzar Rauf Abdullah , Botan Jawdat Abdullah , Vidar Gudmundsson

We present the findings of the superconductivity observed in the silicon nanostructures prepared by short time diffusion of boron on the n-type Si(100) surface. These Si-based nanostructures represent the p-type ultra-narrow self-assembled…

Superconductivity · Physics 2009-11-11 N. T. Bagraev , W. Gehlhoff , L. E. Klyachkin , A. M. Malyarenko , V. V. Romanov , S. A. Rykov

Inorganic-organic interfaces are important for enhancing the power conversion efficiency of silicon-based solar cells through singlet exciton fission (SF). We elucidated the structure of the first monolayers of tetracene (Tc), a SF…

Thin-film self-assembly of three-dimensional (3D) microsystems presents a compelling route to integrate complex functionalities into ultra-compact volumes, yet strategies for incorporating tunable ion-conducting elements remain limited.…

We investigated transport properties of organic heterointerfaces formed by single-crystals of two organic donor-acceptor molecules, tetramethyltetraselenafulvalene (TMTSF) and 7,7,8,8-tetracyanoquinodimethane (TCNQ). Whereas the individual…

Materials Science · Physics 2015-05-18 M. Nakano , H. Alves , A. S. Molinari , S. Ono , N. Minder , A. F. Morpurgo

The anchoring of benzene molecules on lithium adsorption sites at the surface of graphene and nanoribbons thereof are investigated. The effects of adsorbate densities, specific adsorption locations, and spin states on the structural…

Materials Science · Physics 2013-10-01 Dana Krepel , Oded Hod

There is a strong interest to attach nanoparticles non-covalently to one-dimensional systems like boron nitride nanotubes to form composites. The combination of those materials might be used for catalysis, in solar cells, or for water…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 Mirjam Volkmann , Michaela Meyns , Rostyslav Lesyuk , Hauke Lehmann , Christian Klinke

We have studied the adsorption of bisphenol-A-polycarbonate (BPA-PC) on the alpha-Al2O3(0001) surface using density-functional theory (DFT) with van der Waals (vdW) corrections. The BPA-PC polymer can be divided into its chemical fragments…

Materials Science · Physics 2012-05-30 Janne Blomqvist , Petri Salo

The structures and energetics of organic molecules adsorbed onto clean and H-passivated Si(001)-(2$\times$1) surfaces have been calculated using density functional theory. For benzene adsorbed on the clean Si surface the tight-bridge…

Materials Science · Physics 2009-11-13 Karen Johnston , Risto M. Nieminen

Boron-doped multi-walled carbon nanotubes (MWNTs) were synthesized using a methanol solution of boric acid as a source material. Accurate measurements of the electrical resistivity of an individual boron-doped MWNT was performed with a…

The puckered surface of black phosphorus represents an ideal substrate for an unconventional arrangement of physisorbed species and the resulting specific two-dimensional chemistry of this system. This opens the way to investigate the…

Charge transfer from a metal substrate stabilizes honeycomb borophene, whose electron deficit would otherwise spoil the hexagonal order of a $\pi$-bonded 2D atomic network. However, the coupling between the substrate and the boron overlayer…

Materials Science · Physics 2022-11-30 Mandana Safari , Erik Vesselli , Stefano de Gironcoli , Stefano Baroni

Three-dimensional epitaxial heterostructures are based on covalently-bonded interfaces, whereas those from 2-dimensional (2D) materials exhibit van der Waals interactions. Under the right conditions, however, material structures with mixed…

In recent years, graphene-like boron carbide and carbon nitride nanosheets have attracted remarkable attentions, owing to their semiconducting electronic nature and outstanding mechanical and heat transport properties. Graphene-like BC6N is…

Materials Science · Physics 2021-06-15 Bohayra Mortazavi

Understanding the interaction of organic molecules with TiO2 surfaces is important for a wide range of technological applications. While density functional theory (DFT) calculations can provide valuable insight about these interactions,…

Materials Science · Physics 2015-06-23 Marcus Tillotson , Peter Brett , Roger A. Bennett , Ricardo Grau-Crespo

Very recently, two-dimensional(2D) boron sheets (borophene) with rectangular structure has been grown successfully on single crystal Ag(111) substrates.The fabricated boroprene is predicted to have unusual mechanical properties. We…

Mesoscale and Nanoscale Physics · Physics 2016-08-10 Haifeng Wang , Qingfang Li , Yan Gao , F. Miao , Xiang-Feng Zhou , X. G. Wan

Sliding and twisting van der Waals layers with respect to each other gives rise to moir\'e structures with emergent electronic properties. Electrons in these moir\'e structures feel weak potentials that are typically in the tens of…

Mesoscale and Nanoscale Physics · Physics 2020-07-14 Drew Edelberg , Hemant Kumar , Vivek Shenoy , Héctor Ochoa , Abhay N. Pasupathy

Isolated and full monolayer adsorption of various carboranethiol (C$_2$B$_{10}$H$_{12}$S) isomers on gold (111) surface have been investigated using both the standard and van der Waals density functional theoretical calculations. The effect…

Materials Science · Physics 2020-05-20 Ersen Mete , Ayşen Yılmaz , M. Fatih Danışman

We study the assembling of P3HT chains in vacuo by means of a combination of first principles density functional theory and model potential molecular dynamics. We find that, in the absence of any external constraints, the pi-pi interchain…

Soft Condensed Matter · Physics 2010-06-30 Claudio Melis , Alessandro Mattoni , Luciano Colombo