Related papers: Crossover between the zeptosecond and attosecond p…
We investigate the characteristic effects of nuclear motion on attosecond transient absorption spectra in molecules by calculating the spectrum for different model systems. Two models of the hydrogen molecular ion are considered: one where…
Whereas collisions between atoms and molecules are largely understood, collisions between two molecules have proven much harder to study. In both experiment and theory, our ability to determine quantum state-resolved bimolecular cross…
At ultralow energies, atoms and molecules undergo collisions and reactions that are best described in terms of quantum mechanical wave functions. In contrast, at higher energies these processes can be understood quasiclassically. Here, we…
We study single- and multi-quantum transitions of the nuclear spins of ionized arsenic donors in silicon and find quadrupolar effects on the coherence times, which we link to fluctuating electrical field gradients present after the…
In systems of ultracold atoms, pairwise interactions are resonantly enhanced by the application of an oscillating magnetic field that is parallel to the spin-quantization axis of the atoms. The resonance occurs when the frequency of the…
The extremely small probability of quantum tunneling through an almost classical potential barrier may become not small under the action of the specially adapted nonstationary field. The tunneling rate has a sharp peak as a function of the…
A new pathway of strong laser field induced ionization of an atom is identified which is based on recollisions under the tunneling barrier. With an amended strong field approximation, the interference of the direct and the under-the-barrier…
First time-resolved photoemission experiments employing attosecond streaking of electrons emitted by an XUV pump pulse and probed by a few-cycle NIR pulse found a time delay of about 100 attoseconds between photoelectrons from the…
Within the framework of quantization of the macroscopic electromagnetic field, equations of motion and an effective Hamiltonian for treating both the resonant dipole-dipole interaction between two-level atoms and the resonant atom-field…
Attosecond pulses can be used to initiate and control electron dynamics on a sub-femtosecond time scale. The first step in this process occurs when an atom absorbs an ultraviolet photon leading to the formation of an attosecond electron…
We report attosecond-scale probing of the laser-induced dynamics in molecules. We apply the method of high-harmonic spectroscopy, where laser-driven recolliding electrons on various trajec- tories record the motion of their parent ion.…
Quantum time dilation occurs when a clock moves in a superposition of relativistic momentum wave packets. We utilize the lifetime of an excited hydrogen-like atom as a clock to demonstrate how quantum time dilation manifests in a…
Nuclear fusion reactions, at energies, far below the Coulomb barrier play a significant role in the synthesis of light elements in the primordial nucleosynthesis as well as in the interior of compact stellar objects. Many different kinds of…
The implementation of attosecond photoelectron-photoion coincidence spectroscopy for the investigation of atomic and molecular dynamics calls for a high-repetition-rate driving source combined with experimental setups characterized by…
Processes that break molecular bonds are typically observed with molecules occupying a mixture of quantum states and successfully described with quasiclassical models, while a few studies have explored the distinctly quantum mechanical…
We show that time ordering underlying time-dependent quantum dynamics is a physical observable accessible by attosecond streaking. We demonstrate the extraction of time ordering for the prototypical case of time-resolved two-photon double…
The possibility of detection of 5.5 MeV and 14.4 keV solar axions by observing axion-induced nuclear and atomic transitions is investigated. The presence of nuclear transitions between spin-orbit partners can be manifested by the subsequent…
When a pulse of light traverses a material, it incurs a time delay referred to as the group delay. Should the group delay experienced by photons be attributed to the time they spend as atomic excitations? However reasonable this connection…
Alpha particles emitted from an excited projectile-like fragment (PLF*) formed in a peripheral collision of two intermediate-energy heavy ions exhibit a strong preference for emission towards the target-like fragment (TLF). The interplay of…
Numerical attoclock is a theoretical model of attosecond angular streaking driven by a very short, nearly a single oscillation, circularly polarized laser pulse. The reading of such an attoclock is readily obtained from a numerical solution…