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Magnetism in transition-metal compounds (TMCs) has traditionally been associated with spin degrees of freedom, because the orbital magnetic moments are typically largely quenched. On the other hand, magnetic order in 4f- and 5d-electron…

Strongly Correlated Electrons · Physics 2015-10-26 A. Jain , M. Krautloher , J. Porras , G. H. Ryu , D. P. Chen , D. L. Abernathy , J. T. Park , A. Ivanov , J. Chaloupka , G. Khaliullin , B. Keimer , B. J. Kim

We explore the effects of disordered charged defects on the electronic excitations observed in the photoemission spectra of doped transition metal oxides in the Mott insulating regime by the example of the $R_{1-x}$Ca$_x$VO$_3$ perovskites,…

Strongly Correlated Electrons · Physics 2018-04-09 Adolfo Avella , Andrzej M. Oleś , Peter Horsch

Oxides with $4d$/$5d$ transition metal ions are physically interesting for their particular crystalline structures as well as the spin-orbit coupled electronic structures. Recent experiments revealed a series of $4d$/$5d$ transition metal…

Materials Science · Physics 2017-01-27 Bin Gao , Yakui Weng , Jun-Jie Zhang , Huimin Zhang , Yang Zhang , Shuai Dong

We study the effects of electron doping in Mott insulators containing d^4 ions such as Ru4+, Os4+, Rh5+, and Ir5+ with J=0 singlet ground state. Depending on the strength of the spin-orbit coupling, the undoped systems are either…

Strongly Correlated Electrons · Physics 2016-01-12 Jiří Chaloupka , Giniyat Khaliullin

Moir\'e heterostructures of transition metal dichalcogenides exhibit Mott-insulating behaviour both at half-filling as well as at fractional fillings, where electronic degrees of freedom form self-organized Wigner crystal states. An open…

Strongly Correlated Electrons · Physics 2024-01-31 Urban F. P. Seifert , Leon Balents

Magnetic order is usually associated with well-defined magnon excitations. Exotic magnetic fluctuations with fractional, topological or multipolar character, have been proposed for radically different forms of magnetic matter such as…

CoO has an odd number of electrons in its unit cell, and therefore is expected to be metallic. Yet, CoO is strongly insulating owing to significant electronic correlations, thus classifying it as a Mott insulator. We investigate the…

Motivated by experimental and theoretical interest in realizing multipolar orders in $d$-orbital materials, we discuss the quantum magnetism of $J\!=\!2$ ions which can be realized in spin-orbit coupled oxides with $5d^2$ transition metal…

Strongly Correlated Electrons · Physics 2020-03-18 Arun Paramekanti , Dalini D. Maharaj , Bruce D. Gaulin

The interplay of magnetic excitations and itinerant charge carriers is a ubiquitous phenomenon in strongly correlated electron systems. In the vicinity of magnetically ordered phases, strong interactions between itinerant quasiparticles and…

We demonstrate that magnetic $3d$ impurities with $S=3/2$ spins and no orbital degree of freedom induce changes of spin-orbital order in a $4d^4$ Mott insulator with $S=1$ spins. Impurities act either as spin defects which decouple from the…

Strongly Correlated Electrons · Physics 2016-03-02 Wojciech Brzezicki , Mario Cuoco , Andrzej M. Oleś

Polarons and spin-orbit (SO) coupling are distinct quantum effects that play a critical role in charge transport and spin-orbitronics. Polarons originate from strong electron-phonon interaction and are ubiquitous in polarizable materials…

We study the magnetic order and excitations in strong spin-orbit coupled, Van Vleck-type, $d^4$ Mott insulators on a square lattice. Extending the previous work, we include the tetragonal crystal field splitting and explore its effects on…

Strongly Correlated Electrons · Physics 2014-07-29 Alireza Akbari , Giniyat Khaliullin

Protected by the interplay of on-site Coulomb interactions and spin-orbit coupling, Sr$_2$IrO$_4$ at high pressure is a rare example of a Mott insulator with a paramagnetic ground state. Here, using optical Raman scattering, we measure both…

Strongly Correlated Electrons · Physics 2021-11-29 Xiang Li , S. E. Cooper , A. Krishnadas , A. de la Torre , R. S. Perry , F. Baumberger , D. M. Silevitch , D. Hsieh , T. F. Rosenbaum , Yejun Feng

We study a two-dimensional single band Hubbard Hamiltonian with antisymmetric spin-orbit coupling. We argue that this is the minimal model to understand the electronic properties of locally non-centrosymmetric transition-metal (TM) oxides…

Strongly Correlated Electrons · Physics 2021-04-30 Mehdi Biderang , Alireza Akbari , Jesko Sirker

Transition metal compounds with the $(t_{2g})^4$ electronic configuration are expected to be nonmagnetic atomic singlets both in the weakly interacting regime due to spin-orbit coupling, as well as in the Coulomb dominated regime with…

Strongly Correlated Electrons · Physics 2017-01-16 Christopher Svoboda , Mohit Randeria , Nandini Trivedi

Motivated by recent experiments on Mott insulators, in both iridates and ultracold atoms, we theoretically study the effects of magnetic order on the Mott-Hubbard excitons. In particular, we focus on spin-mediated doublon-holon pairing in…

Strongly Correlated Electrons · Physics 2024-04-23 T. -S. Huang , C. L. Baldwin , M. Hafezi , V. Galitski

Evolution of composite spin-orbital order and coupled spin-orbital excitations is studied in a variety of $d^4$ systems with $n$=$4$ electrons in the $t_{2g}$ orbital sector using the generalised self-consistent + fluctuations approach for…

Strongly Correlated Electrons · Physics 2025-04-30 Shahid Ahmad , Harshvardhan Parmar , Shubhajyoti Mohapatra , Avinash Singh

The emergence of quasiparticles in quantum many-body systems underlies the rich phenomenology in many strongly interacting materials. In the context of doped Mott insulators, magnetic polarons are quasiparticles that usually arise from an…

Quantum Gases · Physics 2025-02-12 Max L. Prichard , Benjamin M. Spar , Ivan Morera , Eugene Demler , Zoe Z. Yan , Waseem S. Bakr

The mechanisms of magnetic and orbital interactions due to double exchange (DE) and superexchange (SE) in transition metal oxides with degenerate e_g orbitals are presented. Specifically, we study the effective spin-orbital models derived…

Strongly Correlated Electrons · Physics 2009-10-31 A. M. Oles , M. Cuoco , N. B. Perkins

We show how the general and basic asymmetry between two fundamental degrees of freedom present in strongly correlated oxides, spin and orbital, has very profound repercussions on the elementary spin and orbital excitations. Whereas the…

Strongly Correlated Electrons · Physics 2011-09-30 Krzysztof Wohlfeld , Maria Daghofer , Satoshi Nishimoto , Giniyat Khaliullin , Jeroen van den Brink
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