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The accumulation of helium bubbles at grain boundaries (GBs) critically degrades the mechanical integrity of structural materials in nuclear reactors. While GBs act as sinks for radiation-induced defects, their inherent structural…
As the rapid development of nonlinear optics, the enhancement of optical third harmonic generation becomes a pop research realm in the fields of physics, chemistry, biology, materials science, information science and other fields. In this…
Nonlinear optical microscopy such as in the optical second-harmonic generation (SHG) modality has become a popular tool today for probing materials in the physical and biological sciences. While imaging and spectroscopy are widely used in…
Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…
Two-dimensional (2D) tin(II) sulfide (SnS) crystals belong to a class of orthorhombic semiconducting materials that are lately attracting significant interest, given their remarkable properties, such as in-plane anisotropic optical and…
Interstellar grain alignment studies are currently experiencing a renaissance due to the development of a new quantitative theory based on Radiative Alignment Torques (RAT). One of the distinguishing predictions of this theory is a…
We report on a comprehensive experimental and theoretical study of optical third harmonic generation (THG) on the exciton-polariton resonances in the zinc-blende semiconductors GaAs, CdTe, and ZnSe subject to an external magnetic field,…
Second harmonic generation (SHG) is forbidden in centrosymmetric molecular materials. However, a signal is frequently observed from interfaces where the symmetry is broken. Whereas the effect can be phenomenologically accommodated, an ab…
Star formation is a series of mass assembly processes and starless cores, those cold and dense condensations in molecular clouds, play a pivotal role as initial seeds of stars. With only a limited sample of known starless cores, however,…
The optimization of nonlinear optical processes at the nanoscale is a crucial step for the development of nanoscale photon sources for quantum-optical networks. The development of innovative plasmonic nanoantenna designs and hybrid…
We study the effect of anisotropic radiation illumination on the alignment of polycyclic aromatic hydrocarbons (PAHs) and report that cross-sectional mechanism of alignment earlier considered in terms of gas-grain interactions can also be…
High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…
We present a calculation of Third Harmonic Generation (THG) for two-band systems using the length gauge that avoids unphysical divergences otherwise present in the evaluation of the third order current density response. The calculation is…
The notion of spontaneous symmetry breaking has been used to describe phase transitions in a variety of physical systems. In crystalline solids, the breaking of certain symmetries, such as mirror symmetry, is difficult to detect…
We study the effects of crystal anisotropy on optical phonon resonances in the second harmonic generation (SHG) from silicon carbide (SiC) in its Reststrahl region. By comparing experiments and simulations for isotropic 3C-SiC and…
Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…
Polarized continuum emission from aligned grains in disks around young stellar objects can be used to probe the magnetic field, radiation anisotropy, or drift between dust and gas, depending on whether the non-spherical grains are aligned…
High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…
Pulsar-timing collaborations have recently reported evidence for the detection of an isotropic stochastic gravitational-wave background consistent with one sourced by a population of inspiralling supermassive black hole binaries. However, a…
W-band ({\nu} ca. 94 GHz) electron paramagnetic resonance (EPR) spectroscopy was used for a single-crystal study of a star-shaped Fe3Cr single-molecule magnet (SMM) with crystallographically imposed trigonal symmetry. The high resolution…