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Crystal Structure Prediction (csp) is one of the central and most challenging problems in materials science and computational chemistry. In csp, the goal is to find a configuration of ions in 3D space that yields the lowest potential…

Computational Complexity · Computer Science 2023-06-22 Duncan Adamson , Argyrios Deligkas , Vladimir Gusev , Igor Potapov

We developed a density functional theory-free approach for crystal structure prediction via combing graph network (GN) and Bayesian optimization (BO). GN is adopted to establish the correlation model between crystal structure and formation…

Materials Science · Physics 2020-11-24 Guanjian Cheng , Xin-Gao Gong , Wan-Jian Yin

Crystal structure predictions based on the combination of first-principles calculations and machine learning have achieved significant success in materials science. However, most of these approaches are limited to predicting specific…

Materials Science · Physics 2025-01-28 Zongguo Wang , Ziyi Chen , Yang Yuan , Yangang Wang

Deep Neural Networks (DNNs) on hardware is facing excessive computation cost due to the massive number of parameters. A typical training pipeline to mitigate over-parameterization is to pre-define a DNN structure first with redundant…

Neural and Evolutionary Computing · Computer Science 2019-12-19 Xiaocong Du , Zheng Li , Yufei Ma , Yu Cao

This study presents a deep learning approach to predicting structural and electronic properties of materials using Graph Neural Networks (GNNs). Leveraging data from the Materials Project database, we construct graph representations of…

Disordered Systems and Neural Networks · Physics 2024-12-20 Selva Chandrasekaran Selvaraj

We have developed a powerful method for crystal structure prediction from "scratch" through particle swarm optimization (PSO) algorithm within the evolutionary scheme. PSO technique is dramatically different with the genetic algorithm and…

Materials Science · Physics 2012-05-11 Yanchao Wang , Jian Lv , Li Zhu , Yanming Ma

Crystal structure prediction has been a subject of topical interest, but remains a substantial challenge, especially for complex structures as it deals with the global minimization of the extremely rugged high-dimensional potential energy…

Materials Science · Physics 2022-01-26 Xuecheng Shao , Jian Lv , Peng Liu , Sen Shao , Pengyue Gao , Hanyu Liu , Yanchao Wang , Yanming Ma

Crystal structure determines properties of materials. With the crystal structure of a chemical substance, many physical and chemical properties can be predicted by first-principles calculations or machine learning models. Since it is…

Materials Science · Physics 2021-09-22 Wenhui Yang , Edirisuriya M. Dilanga Siriwardane , Rongzhi Dong , Yuxin Li , Jianjun Hu

Molecular crystal structure prediction (CSP) seeks the most stable periodic structure given the chemical composition of a molecule and pressure-temperature conditions. Modern CSP solvers use global optimization methods to search for…

Optimization and Control · Mathematics 2023-02-21 Miloslav Torda , John Y. Goulermas , Roland Púček , Vitaliy Kurlin

First-principles based crystal structure prediction (CSP) methods have revealed an essential tool for the discovery of new materials. However, in solids close to displacive phase transitions, which are common in ferroelectrics,…

Materials Science · Physics 2026-04-17 Hao Gao , Yue-Wen Fang , Ion Errea

Structure is the most basic and important property of crystalline solids; it determines directly or indirectly most materials characteristics. However, predicting crystal structure of solids remains a formidable and not fully solved…

Materials Science · Physics 2021-01-04 Haotong Liang , Valentin Stanev , A. Gilad Kusne , Ichiro Takeuchi

The recently proposed crystal graph convolutional neural network (CGCNN) offers a highly versatile and accurate machine learning (ML) framework by learning material properties directly from graph-like representations of crystal structures…

Computational Physics · Physics 2020-07-01 Cheol Woo Park , Chris Wolverton

Machine learning potentials (MLPs) have become indispensable for conducting accurate large-scale atomistic simulations and for the efficient prediction of crystal structures. Polynomial MLPs, defined by polynomial rotational invariants,…

Materials Science · Physics 2024-08-05 Atsuto Seko

Crystal structure prediction remains a major challenge in materials science, directly impacting the discovery and development of next-generation materials. We introduce TCSP 2.0, a substantial evolution of our template-based crystal…

Materials Science · Physics 2025-04-01 Lai Wei , Rongzhi Dong , Nihang Fu , Sadman Sadeed Omee , Jianjun Hu

A novel Genetic Algorithm is described that is suitable for determining the global minimum energy configurations of crystal structures and which can also be used as a polymorph search technique. This algorithm requires no prior assumptions…

Other Condensed Matter · Physics 2007-05-23 N. L. Abraham , M. I. J. Probert

Historically, materials informatics has relied on human-designed descriptors of materials structures. In recent years, graph neural networks (GNNs) have been proposed for learning representations of crystal structures from data end-to-end…

Materials Science · Physics 2023-03-29 Sheng Gong , Tian Xie , Yang Shao-Horn , Rafael Gomez-Bombarelli , Jeffrey C. Grossman

Crystal structures can be predicted from first-principles using ab initio random structure searching AIRSS and density functional theory (DFT). AIRSS provides a method to sample the potential energy landscape and DFT provides a robust and…

Materials Science · Physics 2025-09-30 Lewis J. Conway , Chris J. Pickard

Crystal structure prediction algorithms have become powerful tools for materials discovery in recent years, however, they are usually limited to relatively small systems. The main challenge is that the number of local minima grows…

Materials Science · Physics 2022-02-09 Hao Gao , Junjie Wang , Yu Han , Jian Sun

Determining the stability of chemical compounds is essential for advancing material discovery. In this study, we introduce a novel deep neural network model designed to predict a crystal's formation energy, which identifies its stability…

Materials Science · Physics 2026-04-21 V. Torlao , E. A. Fajardo

Crystal graph neural networks predict materials properties by propagating information through local atomic environments. In conventional crystal graph convolutional neural networks (CGCNNs), this propagation depth is increased by stacking…

Materials Science · Physics 2026-05-18 Satadeep Bhattacharjee