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The Stokes-Einstein (SE) relation has been widely applied to quantitatively describe the Brownian motion. Notwithstanding, here we show that even for a simple fluid, the SE relation may not be completely applicable. Namely, although the SE…

Statistical Mechanics · Physics 2021-03-17 Hanqing Zhao , Hong Zhao

Highly supercooled liquids with soft-core potentials are studied via molecular dynamics simulations in two and three dimensions in quiescent and sheared conditions.We may define bonds between neighboring particle pairs unambiguously owing…

Soft Condensed Matter · Physics 2009-10-31 Ryoichi Yamamoto , Akira Onuki

We perform molecular dynamics simulation on a glass-forming liquid binary mixture with the soft-core potential in three dimensions. We investigate crossover of the configuration changes caused by stringlike jump motions. With lowering the…

Soft Condensed Matter · Physics 2015-06-11 Takeshi Kawasaki , Akira Onuki

Glass formers exhibit a viscoelastic behavior: at the laboratory timescale, they behave like (glassy) solids at low temperatures, and like liquids at high temperatures. Based on this observation, elastic models relate the long time…

Chemical Physics · Physics 2017-08-01 Emmanuel Guillaud , Laurent Joly , Dominique De Ligny , Samy Merabia

We experimentally investigate the superfluid properties of a two-dimensional, weakly interacting Bose-Einstein condensate in the zero-temperature regime, when it is subjected to a triangular optical lattice potential. We implement an…

Quantum Gases · Physics 2025-11-07 F. Rabec , G. Brochier , S. Wattellier , G. Chauveau , Y. Li , S. Nascimbene , J. Dalibard , J. Beugnon

In simulations of supercooled, high-density liquid silica we study a range of temperature T in which we find both crystal nucleation, as well as the characteristic dynamics of a glass forming liquid, including a breakdown of the…

Materials Science · Physics 2015-05-14 Ivan Saika-Voivod , Richard K. Bowles , Peter H. Poole

We investigate the dynamics of kinetically frozen block copolymer micelles of different softness across a wide range of particle concentrations, from the fluid to the onset of glassy behavior, through a combination of rheology, dynamic…

Hydrodynamic interactions are important for diverse fluids especially those with low Reynold's number such as microbial and particle-laden suspensions, and proteins diffusing in membranes. Unfortunately, while far-field (asymptotic)…

Soft Condensed Matter · Physics 2023-02-10 Noman Hanif Barbhuiya , A. G. Yodh , Chandan K. Mishra

The diffusion of glycerol molecules decreases with decreasing temperature as its viscosity increases in a manner simply described by the Stokes-Einstein(SE) relation. Approaching the glass transition, this relation breaks down as it does…

Disordered Systems and Neural Networks · Physics 2007-05-23 Bo Chen , Eric E. Sigmund , W. P. Halperin

The Stokes-Einstein relation (SER) is one of the most robust and widely employed results from the theory of liquids. Yet sizable deviations can be observed for self-solvation, which cannot be explained by the standard hydrodynamic…

Statistical Mechanics · Physics 2018-06-15 Benoit Charbonneau , Patrick Charbonneau , Grzegorz Szamel

Kinetically constrained models (KCMs) have gained much interest as models that assign the origins of interesting dynamic properties of supercooled liquids to dynamical facilitation mechanisms that have been revealed in many expreiments and…

Soft Condensed Matter · Physics 2015-10-22 Seo-Woo Choi , Soree Kim , YounJoon Jung

In supercooled liquids, at a temperature between the glass transition temperature Tg and the melting point Tm, thermodynamic properties remain continuous, while dynamic behavior exhibits anomalies. The origin of such thermodynamics-dynamic…

Soft Condensed Matter · Physics 2025-06-17 X. R. Tian , D. M. Zhang , B. Zhang , D. Y. Sun , X. G. Gong

We present a review on the study of metastable silicon, primarily focusing mainly on the aspects of liquid-liquid transition, critical point and phase behaviour, structural and dynamic properties of liquid phase as well as crystal…

Materials Science · Physics 2021-09-01 Vishwas V. Vasisht , Srikanth Sastry

The existence of a phase transition between two distinct liquid phases in single-component network-forming liquids (e.g., water, silica, silicon) has elicited considerable scientific interest. The challenge, both for experiments and…

Soft Condensed Matter · Physics 2022-05-30 Yagyik Goswami , Srikanth Sastry

We present Monte Carlo simulation results on the equilibrium relaxation of the two dimensional lattice Coulomb gas with fractional charges, which exhibits a close analogy to the primary relaxation of fragile supercooled liquids. Single…

Statistical Mechanics · Physics 2007-05-23 S. J. Lee , B. Kim , J. -R. Lee

We investigate the heterogeneity of dynamics, the breakdown of the Stokes-Einstein relation and fragility in a model glass forming liquid, a binary mixture of soft spheres with a harmonic interaction potential, for spatial dimensions from 3…

Soft Condensed Matter · Physics 2021-08-20 Monoj Adhikari , Smarajit Karmakar , Srikanth Sastry

A self-consistent model of the superfluid (SF) state of a Bose liquid with strong interaction between bosons is considered, in which at T=0, along with a weak single-particle Bose-Einstein condensate (BEC), there exists an intensive pair…

Soft Condensed Matter · Physics 2007-05-23 E. A. Pashitskii , S. V. Mashkevich , S. I. Vilchynskyy

We consider the diffusion constant, D, of a probe particle coupled to the East model, extending previous numerical results for this model to encompass a total of twelve orders of magnitude in relaxation time, {\tau}. Our considerations thus…

Statistical Mechanics · Physics 2013-09-24 YounJoon Jung , Soree Kim , Juan P. Garrahan , David Chandler

Dynamics of a coarse-grained model for the room-temperature ionic liquid, 1-ethyl-3-methylimidazolium hexafluorophosphate, couched in the united-atom site representation are studied via molecular dynamics simulations. The dynamically…

Soft Condensed Matter · Physics 2017-03-15 Daun Jeong , M. Y. Choi , Hyung. J. Kim , YounJoon Jung

We examine dynamic heterogeneities in a model glass-forming fluid, a binary harmonic sphere mixture, above and below the mode-coupling temperature T_c. We calculate the ensemble independent susceptibility chi_4(tau_alpha) and the dynamic…

Statistical Mechanics · Physics 2015-06-12 Elijah Flenner , Grzegorz Szamel