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The electron spin polarization on half-metallic double-perovskites is usually conditioned to the ordered rock-salt arrangement of the transition-metal ions along the lattice. In this work, we investigate a polycrystalline sample of the…

Defect chemistry, strain, and structural, magnetic and electronic degrees of freedom constitute a rich space for the design of functional properties in transition metal oxides. Here, we show that it is possible to engineer polarity and…

Materials Science · Physics 2021-09-15 Chiara Ricca , Ulrich Aschauer

Perovskite bilayers with (111)-orientation combine a honeycomb lattice as a key feature with the strongly correlated, multiorbital nature of electrons in transition metal oxides. In a systematic DFT+$U$ study of (111)-oriented…

Materials Science · Physics 2016-05-04 David Doennig , Santu Baidya , Warren E. Pickett , Rossitza Pentcheva

The crystal structure determines many of the physical properties of oxide perovskites (ABO$_3$) and only a tiny modification of the lattice structure causes major changes in the functional properties through the interplay among spin,…

Novel interplay of spin-orbit coupling and electron correlations in complex Ir oxides recently emerged as a new paradigm for correlated electron physics. Because of a large spin-orbit coupling of ~0.5 eV, which is comparable to the transfer…

Strongly Correlated Electrons · Physics 2015-06-22 Jobu Matsuno , Kota Ihara , Shugen Yamamura , Hiroki Wadati , Kenji Ishii , V. Vijay Shankar , Hae-Young Kee , Hidenori Takagi

The ability to probe symmetry breaking transitions on their natural time scales is one of the key challenges in nonequilibrium physics. Stripe ordering represents an intriguing type of broken symmetry, where complex interactions result in…

In this paper we present results of our calculations of the non-collinear spin density distribution in the systems with frustrated triangular magnetic structure (Mn-based antiperovskite compounds, Mn_{3}AN (A=Ga, Zn)) in the ground state…

Materials Science · Physics 2015-05-14 Pavel Lukashev , Renat F. Sabirianov , Kirill Belashchenko

It is well known that if a crystal structure has no inversion symmetry, it may allow for Dzyaloshinskii-Moriya magnetic interactions, operating between different crystallographic unit cells, which in turn should lead to the formation of…

Materials Science · Physics 2012-03-19 I. V. Solovyev

Candidates for correlated topological insulators, originated from the spin-orbit coupling as well as Hubbard type correlation, are expected in the ($111$) bilayer of perovskite-structural transition-metal oxides. Based on the…

Materials Science · Physics 2015-11-11 Yakui Weng , Xin Huang , Yugui Yao , Shuai Dong

Time-of-flight inelastic neutron scattering measurements have been carried out on polycrystalline samples of the 4$d^3$ and 5$d^3$ double pervoskite antiferromagnets La$_2$LiRuO$_6$ and La$_2$LiOsO$_6$. These reveal the development of an…

Strongly Correlated Electrons · Physics 2018-10-03 D. D. Maharaj , G. Sala , C. A. Marjerrison , M. B. Stone , J. E. Greedan , B. D. Gaulin

We use the LDA+U method to study the possibility of exciton condensation in perovskites of transition metals with $d^6$ electronic configuration such as LaCoO$_3$. For realistic interaction parameters we find several distinct solutions…

Strongly Correlated Electrons · Physics 2017-03-17 J. Fernandez Afonso , J. Kunes

Spin crossover plays a central role in the structural instability, net magnetic moment modification, metallization, and even in superconductivity in corresponding materials. Most reports on the pressure-induced spin crossover with a large…

We present results of local spin density approximation (LSDA) pseudopotential calculations for the perovskite structure oxide, bismuth manganite (BiMnO3). The origin of the differences between bismuth manganite and other perovskite…

Materials Science · Physics 2009-10-31 Nicola A. Hill , Karin M. Rabe

We present a detailed study of the local atomic and magnetic structure of the type-I multiferroic perovskite system (Sr,Ba)(Mn,Ti)O$_3$ using x-ray and neutron pair distribution function (PDF) analysis, polarized neutron scattering, and…

We present a combined study of Ni $K$-edge resonant x-ray scattering and density functional calculations to probe and distinguish electronically driven ordering and lattice distortions in nickelate heterostructures. We demonstrate that due…

We used high-resolution resonant inelastic x-ray scattering (RIXS) at the Ni $L_3$ edge to simultaneously investigate high-energy interband transitions characteristic of Ni-O bond ordering and low-energy collective excitations of the Ni…

The model developed for LaMnO$_3$ addresses the spin-orbital order by superexchange and Jahn-Teller orbital interactions in the cubic (perovskite) symmetry up to now whereas real crystal structure is strongly deformed. We identify and…

Strongly Correlated Electrons · Physics 2018-03-28 Mateusz Snamina , Andrzej M. Oleś

Inorganic-organic lead halide perovskites, particularly methylammonium lead halide (MAPbI$_3$) perovskite, is perceived to be a promising material for optoelectronics and spintronics. However, lead toxicity and instability under air and…

Materials Science · Physics 2022-12-07 Megha Arya , Preeti Bhumla , Sajjan Sheoran , Suraj , S Bhattacharya

The dynamic dielectric nonlinearity of barium strontium titanate (Ba1-x,Srx)TiO3 ceramics is investigated in their paraelectric phase. With the goal to contribute to the identification of the mechanisms that govern the dielectric…

Materials Science · Physics 2017-05-24 Sina Hashemizadeh , Dragan Damjanovic

The ground state and excited state properties of the perovskite LaMnO$_3$ are calculated based on the generalized-gradient-corrected relativistic full-potential method. The electronic structure, magnetism and energetics of various spin…

Strongly Correlated Electrons · Physics 2009-11-07 P. Ravindran , A. Kjekshus , H. Fjellvåg , A. Delin , O. Eriksson