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Non-relativistic spin splitting in antiferromagnets has recently attracted considerable attention. Here we present a universal framework for controlling such spin splitting by identifying and manipulating the key atomic distortions that…

Materials Science · Physics 2025-09-25 Aniruddha Ray , Subhadeep Bandyopadhyay , Sayantika Bhowal

Using results of the band structure calculations in the local-spin-density approximation we demonstrate how the crystal distortions affect the magnetic structure of orthorhombically distorted perovskites leading to a non-collinear spin…

Materials Science · Physics 2009-11-10 I. V. Solovyev , N. Hamada , K. Terakura

Hybrid organic-inorganic perovskites are famous for the diversity of their chemical compositions, phases and phase transitions, and associated physical properties. We use a combination of experimental and computational techniques to reveal…

Antiferromagnetic antiperovskites, of the form Mn$_3B$N ($B$ = Ni, Cu, Zn, Sn, Ir, and Pt), have shown an outstanding behavior in which, giant negative thermal expansion and chiral magnetic structures are intertwined. As such, aiming to…

Materials Science · Physics 2022-09-07 L. Florez-Gomez , W. Ibarra-Hernandez , A. C. Garcia-Castro

Recently, spin splitting of non-relativistic origin in compensated antiferromagnets has drawn growing attention in condensed matter research. Although many materials, now known to exhibit such spin splitting, have been studied for decades,…

Materials Science · Physics 2025-10-24 Sayantika Bhowal , Arnab Bose

Perovskite oxide heterostructures offer an important path forward for stabilizing and controlling low-dimensional magnetism. One of the guiding design principles for these materials systems is octahedral connectivity. In superlattices…

Materials Science · Physics 2017-11-08 Charles L. Flint , Arturas Vailionis , Hua Zhou , Hoyoung Jang , Jun-Sik Lee , Yuri Suzuki

The momentum-dependent Rashba and Dresselhaus spin-splitting has gained much attention for its highly promising applications in spintronics. In the present work, ab initio density functional theory calculations are performed to study the…

Materials Science · Physics 2022-08-02 Sajjan Sheoran , Manish Kumar , Preeti Bhumla , Saswata Bhattacharya

Crystal and magnetic structures of the high-pressure stabilized perovskite phase of TlMnO3 have been studied by neutron powder diffraction. The crystal structure involves two types of primary structural distortions: a+b-b-octahedral tilting…

Strongly Correlated Electrons · Physics 2019-03-07 Dmitry D. Khalyavin , Pascal Manuel , Wei Yi , Alexei A. Belik

We provide a theoretical demonstration of controllable non-relativistic spin splitting in both electronic and magnonic bands via targeted structural distortions tied to specific phonon modes. Using MnF$_2$ as a model system, we identify a…

Materials Science · Physics 2025-09-11 Subhadeep Bandyopadhyay , Anoop Raj , Philippe Ghosez , Sumiran Pujari , Sayantika Bhowal

Spin splitting, or removal of spin degeneracy in the electronic energy band/level is often a measure of spin-orbit coupling strength and a way to manipulate spin degrees of freedom. We use first-principles simulations to predict giant spin…

Materials Science · Physics 2024-03-18 Nikhilesh Maity , Ravi Kashikar , S. Lisenkov , I. Ponomareva

Spin-polarized currents play a key role in spintronics. Recently, it has been found that antiferromagnets with a non-spin-degenerate band structure can efficiently spin-polarize electric currents, even though their net magnetization is…

Materials Science · Physics 2021-12-20 Gautam Gurung , Ding-Fu Shao , Evgeny Y. Tsymbal

Magnetoelectric phase diagrams of the rare-earth (R) Mn perovskites RMnO3 are theoretically studied by focusing on crucial roles of the symmetric magnetostriction or the Peierls-type spin-phonon coupling through extending our previous work…

Strongly Correlated Electrons · Physics 2011-10-07 Masahito Mochizuki , Nobuo Furukawa , Naoto Nagaosa

We report the observation of a persistent spin texture (PST) in pseudo-2D hybrid perovskite, characterized by significant spin splitting strength on the order of \(3 \, \text{eV} \cdot \text{\AA}\). Using first-principles density functional…

Materials Science · Physics 2025-11-25 Shantanu Pathak , Saswata Bhattacharya

Recent studies have shown that the non-relativistic antiferromagnetic ordering could generate momentum-dependent spin splitting analogous to the Rashba effect, but free from the requirement of relativistic spin-orbit coupling. Whereas the…

Materials Science · Physics 2021-06-16 Lin-Ding Yuan , Zhi Wang , Jun-Wie Luo , Alex Zunger

Spatial, momentum and energy separation of electronic spins in condensed matter systems guides the development of novel devices where spin-polarized current is generated and manipulated. Recent attention on a set of previously overlooked…

Muon spin relaxation measurements are reported on samples of dimethylammonium metal formates containing magnetic divalent nickel, cobalt, manganese, and copper ions. These hybrid organic-inorganic perovskites exhibit weak ferromagnetism and…

Strongly Correlated Electrons · Physics 2015-05-19 P. J. Baker , T. Lancaster , I. Franke , W. Hayes , S. J. Blundell , F. L. Pratt , P. Jain , Z. -M. Wang , M. Kurmoo

By means of neutron powder diffraction, we investigated the effect of the polar Bi$^{3+}$ ion on the magnetic ordering of the Mn$^{3+}$ ions in BiMn$_3$Mn$_4$O$_{12}$, the counterpart with \textit{quadruple} perovskite structure of the…

Strongly Correlated Electrons · Physics 2019-06-05 A. Gauzzi , G. Rousse , F. Mezzadri , G. Calestani , G. André , F. Bourée , M. Calicchio , E. Gilioli , R. Cabassi , F. Bolzoni , A. Prodi , P. Bordet , M. Marezio

Spin splitting and the resulting spin texture are central to emerging spintronic applications. In non-centrosymmetric non-magnetic materials containing heavy elements, spin textures are typically governed by low-order, momentum-dependent…

Materials Science · Physics 2025-07-31 Jiaxuan Wu , Boyun Zeng , Hanghui Chen

The non-relativistic spin-splitting (NRSS) of electronic bands in "altermagnets" has sparked renewed interest in antiferromagnets (AFMs) that have no net magnetization. However, altermagnets with collinear and compensated magnetism are not…

Materials Science · Physics 2024-12-31 Lin-Ding Yuan , Alexandru B. Georgescu , James M. Rondinelli

We identify a nonequilibrium route for generating altermagnetic spin splitting in antiferromagnet by ultrafast light. Unlike existing strategies, this route does not require relativistic angular-momentum transfer, static symmetry breaking,…

Materials Science · Physics 2026-04-13 Huang-Zhao-Xiang Chen , Lin-Ding Yuan , Wen-Hao Liu , Lin-Wang Wang , Jun-Wei Luo , Zhi Wang
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