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In this paper we combine two powerful computational techniques, well-tempered metadynamics and time lagged independent component analysis. The aim is to develop a new tool for studying rare events and exploring complex free energy…

Statistical Mechanics · Physics 2017-12-08 James McCarty , Michele Parrinello

In living systems, collective molecular behavior is driven by thermodynamic forces in the form of chemical gradients. Leveraging recent advances in the field of nonequilibrium physics, I show that increasing the thermodynamic force alone…

Subcellular Processes · Quantitative Biology 2022-09-21 Milo M. Lin

We present numerical results for a chemical reaction of colloidal particles which are transported by a laminar fluid and are focused by periodic obstacles in such a way that the two components are well mixed and consequently the chemical…

Chemical Physics · Physics 2015-06-12 A. M. Lacasta , L. Ramirez-Piscina , J. M. Sancho , K. Lindenberg

We discuss recent progress in the theoretical description of chemotaxis by coupling the diffusion equation of a chemical species to equations describing the motion of sensing microorganisms. In particular, we discuss models for…

Soft Condensed Matter · Physics 2019-02-05 B. Liebchen , H. Löwen

We develop a novel method to analyze the dynamics of stochastic rewriting systems evolving over finitary adhesive, extensive categories. Our formalism is based on the so-called rule algebra framework and exhibits an intimate relationship…

Logic in Computer Science · Computer Science 2023-06-22 Nicolas Behr , Vincent Danos , Ilias Garnier

We investigate the plasma enhancement of nuclear reactions in the intermediate coupling regime using orbital free molecular dynamics (OFMD) simulations. Mixtures of H-Cu and H-Ag serve as prototypes of simultaneous weak and strong couplings…

Mixtures of particles that interact through phoretic effects are known to aggregate if they belong to species that exhibit attractive self-interactions. We study self-organization in a model metabolic cycle composed of three species of…

Soft Condensed Matter · Physics 2023-09-29 Vincent Ouazan-Reboul , Ramin Golestanian , Jaime Agudo-Canalejo

The energy for protein folding arises from multiple sources and is not large in total. In spite of the many specific successes of energy landscape and other approaches, there still seems to be some missing guiding factor that explains how…

Mathematical Physics · Physics 2011-08-22 Walter Simmons , Joel L. Weiner

Particles moving in oscillating potential with broken mirror symmetry are considered. We calculate their energetic efficiency, when acting as molecular motors carrying a load against external force. It is shown that interaction between…

Statistical Mechanics · Physics 2010-09-03 Frantisek Slanina

Motivated by the possibility of electrochemical control of phase separation, a variational theory of thermodynamic stability is developed for driven reactive mixtures, based on a nonlinear generalization of the Cahn-Hilliard and Allen-Cahn…

Chemical Physics · Physics 2017-11-01 Martin Z. Bazant

Collective transport through channels shows surprising properties under one-dimensional confinement: particles in a single file exhibit sub-diffusive behavior, while liquid confinement causes distance-independent correlations between the…

Soft Condensed Matter · Physics 2019-06-05 Karolis Misiunas , Ulrich F. Keyser

We study the spontaneous excitation of an accelerated multilevel atom in dipole coupling to the derivative of a massless quantum scalar field and separately calculate the contributions of the vacuum fluctuation and radiation reaction to the…

General Relativity and Quantum Cosmology · Physics 2009-11-13 Yunfeng Zhu , Hongwei Yu

The physics of activated escape of objects out of a metastable state plays a key role in diverse scientific areas involving chemical kinetics, diffusion and dislocation motion in solids, nucleation, electrical transport, motion of flux…

Adaptation and Self-Organizing Systems · Physics 2016-08-08 D. Hennig , C. Mulhern , L. Schimansky-Geier , G. P. Tsironis , P. Hänggi

The propulsion of active particles by self-diffusiophoresis is driven by asymmetric catalytic reactions on the particle surface that generate a mechanochemical coupling between the fluid velocity and the concentration fields of fuel and…

Statistical Mechanics · Physics 2018-12-24 Pierre Gaspard , Raymond Kapral

The dynamic behavior of microtubules in solution can be strongly modified by interactions with walls or other structures. We examine here a microtubule growth model where the increase in size of the plus-end is perturbed by collisions with…

Soft Condensed Matter · Physics 2010-09-29 Vladimir A. Baulin , Carlos M. Marques , Fabrice Thalmann

A system formed by a crowded environment of catalytic obstacles and complex oscillatory chemical reactions is inquired. The obstacles are static spheres of equal radius, which are placed in a random way. The chemical reactions are carried…

Chemical Physics · Physics 2018-12-05 Carlos Echeverria , José L. Herrera , Kay Tucci , Orlando Alvarez-Llamoza , Miguel Morales

We study the dynamics of active Janus particles that self-propel in solution by light-activated catalytic decomposition of chemical "fuel." We develop an analytical model of a photo-active self-phoretic particle that accounts for…

Soft Condensed Matter · Physics 2019-05-23 W. E. Uspal

Autocatalytic reaction fronts between reacted and unreacted species may propagate as solitary waves, namely at a constant front velocity and with a stationary concentration profile, resulting from a balance between molecular diffusion and…

Fluid Dynamics · Physics 2007-05-23 M. Leconte , J. Martin , N. Rakotomalala , D. Salin

In this review article, we focus on collective motion in externally driven colloidal suspensions, as well as how these collective effects can be harnessed for use in microfluidic applications. We highlight the leading role of hydrodynamic…

Soft Condensed Matter · Physics 2018-11-01 Michelle Driscoll , Blaise Delmotte

Random non-reciprocal interactions between a large number of conserved densities are shown to enhance the stability of the system towards pattern formation. The enhanced stability is an exact result when the number of species approaches…

Soft Condensed Matter · Physics 2025-10-08 Laya Parkavousi , Navdeep Rana , Ramin Golestanian , Suropriya Saha