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Variational quantum algorithms constitute one of the most widespread methods for using current noisy quantum computers. However, it is unknown if these heuristic algorithms provide any quantum-computational speedup, although we cannot…

The quantum approximate optimization algorithm (QAOA) has become a cornerstone of contemporary quantum applications development. In QAOA, a quantum circuit is trained -- by repeatedly adjusting circuit parameters -- to solve a problem.…

Quantum Physics · Physics 2021-08-17 V. Akshay , D. Rabinovich , E. Campos , J. Biamonte

We propose a technique for optimizing parameterized circuits in variational quantum algorithms based on the probabilistic tensor sampling optimization. This method allows one to relax random initialization issues or heuristics for…

Quantum Physics · Physics 2024-02-01 G. V. Paradezhenko , A. A. Pervishko , D. Yudin

The Quantum approximate optimization algorithm (QAOA) is a quantum-classical hybrid algorithm aiming to produce approximate solutions for combinatorial optimization problems. In the QAOA, the quantum part prepares a quantum parameterized…

Quantum Physics · Physics 2024-04-23 Ningyi Xie , Xinwei Lee , Dongsheng Cai , Yoshiyuki Saito , Nobuyoshi Asai

Quantum computers have the potential to advance material design and drug discovery by performing costly electronic structure calculations. A critical aspect of this application requires optimizing the limited resources of the quantum…

Variational quantum eigensolvers (VQE) are among the most promising approaches for solving electronic structure problems on near-term quantum computers. A critical challenge for VQE in practice is that one needs to strike a balance between…

We propose a machine learning based approach to accelerate quantum approximate optimization algorithm (QAOA) implementation which is a promising quantum-classical hybrid algorithm to prove the so-called quantum supremacy. In QAOA, a…

Emerging Technologies · Computer Science 2020-04-07 Mahabubul Alam , Abdullah Ash-Saki , Swaroop Ghosh

To enable the accelerated discovery of materials with desirable properties, it is critical to develop accurate and efficient search algorithms. Quantum annealers and similar quantum-inspired optimizers have the potential to provide…

Machine learning-based inverse materials discovery has attracted enormous attention recently due to its flexibility in dealing with black box models. Yet, many metaheuristic algorithms are not as widely applied to materials discovery…

Materials Science · Physics 2023-12-15 Hanfeng Zhai , Hongxia Hao , Jingjie Yeo

For a very long time, computational approaches to the design of new materials have relied on an iterative process of finding a candidate material and modeling its properties. AI has played a crucial role in this regard, helping to…

We propose a framework for optimization of the chemical composition of multinary compounds with the aid of machine learning. The scheme is based on first-principles calculation using the Korringa-Kohn-Rostoker method and the coherent…

Materials Science · Physics 2019-06-05 Taro Fukazawa , Yosuke Harashima , Zhufeng Hou , Takashi Miyake

We present a novel formulation of structural design optimization problems specifically tailored to be solved by quantum annealing (QA). Structural design optimization aims to find the best, i.e., material-efficient yet high-performance,…

Computational Engineering, Finance, and Science · Computer Science 2024-04-17 Fabian Key , Lukas Freinberger

Finding low-energy molecular conformers is challenging due to the high dimensionality of the search space and the computational cost of accurate quantum chemical methods for determining conformer structures and energies. Here, we combine…

Computational Physics · Physics 2020-06-29 Lincan Fang , Esko Makkonen , Milica Todorovic , Patrick Rinke , Xi Chen

There is a pressing need to develop new rechargeable battery technologies that can offer higher energy storage, faster charging, and lower costs. Despite the success of existing methods for the simulation of battery materials, they can…

Quantum chemistry calculations for small molecules on quantum hardware have been demonstrated to date only on universal-gate quantum computers, not quantum annealers. The latter devices are limited to finding the lowest eigenstate of the…

Chemical Physics · Physics 2019-01-16 Scott N. Genin , Ilya G. Ryabinkin , Artur F. Izmaylov

This study investigates the application of Factorization Machines with Quantum Annealing (FMQA) to address the crystal structure problem (CSP) in materials science. FMQA is a black-box optimization algorithm that combines machine learning…

Crystal structure prediction is now playing an increasingly important role in discovery of new materials. Global optimization methods such as genetic algorithms (GA) and particle swarm optimization (PSO) have been combined with first…

Materials Science · Physics 2021-02-09 Jianjun Hu , Wenhui Yang , Rongzhi Dong , Yuxin Li , Xiang Li , Shaobo Li

The Quantum Approximate Optimization Algorithm (QAOA) has shown promise in solving combinatorial optimization problems by leveraging quantum computational power. We propose a simple approach, the Two-Step QAOA, which aims to improve the…

Quantum Physics · Physics 2025-02-25 Yuichiro Minato

An essential component of many sophisticated metaheuristics for solving combinatorial optimization problems is some variation of a local search routine that iteratively searches for a better solution within a chosen set of immediate…

Quantum Physics · Physics 2025-02-05 M. Podobrii , V. Kuzmin , V. Voloshinov , M. Veshchezerova , M. R. Perelshtein

Quantum Approximate Optimization Algorithm (QAOA) is one of the most promising quantum heuristics for combinatorial optimization. While QAOA has been shown to perform well on small-scale instances and to provide an asymptotic speedup over…

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