Related papers: Femtosecond Temporal Phase-Resolved Nonlinear Opti…
As optical two-dimensional coherent spectroscopy (2DCS) is extended to a broader range of applications, it is critical to improve the detection sensitivity of optical 2DCS. We developed a fast phase-cycling scheme in a non-collinear optical…
Ultrafast science and technology have brought in burgeoning opportunities to optical metrology, strong-field physics, non-equilibrium physics, etc., through light-matter interaction due to ever-advancing temporal resolution and peak power…
The time-dependent optical properties of molecular systems are investigated by step-scan Fourier-transform spectroscopy in order to explore the dynamics at phase transitions and molecular orientation in the milli- and microsecond range. The…
Interferometry has underpinned a century of discoveries, ranging from the disproval of the ether theory to the detection of gravitational waves, offering insights into wave dynamics with unrivalled precision through the measurement of phase…
We realize and model a Rydberg-state atom interferometer for measurement of phase and intensity of radio-frequency (RF) electromagnetic waves. A phase reference is supplied to the atoms via a modulated laser beam, enabling atomic…
We present an optical method to measure radio-frequency electro-optic phase modulation profiles by employing spectrum-to-time mapping realized by highly chirped optical pulses. We directly characterize temporal phase modulation profiles of…
In the last two decades, non-equilibrium spectroscopies have evolved from avant-garde studies to crucial tools for expanding our understanding of the physics of strongly correlated materials. The possibility of obtaining simultaneously…
Fluorescence-detected Fourier transform (FT) spectroscopy is a technique in which the relative paths of an optical interferometer are controlled to excite a material sample, and the ensuing fluorescence is detected as a function of the…
Soliton molecules are the manifestation of attractive and repulsive interaction between optical pulses mediated by a nonlinear medium. However, the formation and breakup of soliton molecules are difficult to observe due to the transient…
Nonlinear spectroscopy is widely used to study the transient dynamics of molecules under strong light-matter coupling, though it remains unclear to what extent uncoupled intracavity molecules obscure signals from the strongly-coupled…
Photomixing of two near-infrared lasers is well established for continuous-wave terahertz spectroscopy. Photomixing of three lasers allows us to measure at three terahertz frequencies simultaneously. Similar to Fourier spectroscopy, the…
Nonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors…
Temperature drift, stress birefringence and low frequency vibration lead to the randomness and fluctuation of the output of optical voltage sensor(OVS). In order to solve the problem, this study adopts the lock-in amplifier technology with…
We study a nonlinear interferometer consisting of two consecutive parametric amplifiers, where all three optical fields (pump, signal and idler) are treated quantum mechanically, allowing for pump depletion and other quantum phenomena. The…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
We perform high-resolution real-time read-out of the motion of a single trapped and laser-cooled Ba ion. By using an interferometric setup we demonstrate shot-noise limited measurement of thermal oscillations with resolution of 4 times the…
The development of a multiple-channel lock-in optical spectrometer (LIOS) is presented, which enables parallel phase-sensitive detection at the output of an optical spectrometer. The light intensity from a spectrally broad source is…
Although Rydberg atom-based electric field sensing provides key advantages over traditional antenna-based detection, it remains limited by the need for a local oscillator (LO) for low-field and phase resolved detection. In this work, we…
Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…
Attosecond time-resolution experiments using noncollinear interferometers require precise and active control of the optical delay to prevent instabilities - including both slow drifts and rapid vibrations - that can obscure the time…