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Crystallization of supersaturated liquids usually starts by heterogeneous nucleation. Mounting evidence shows that even homogeneous nucleation in simple liquids takes place in two steps; first a dense amorphous precursor forms, and the…

Materials Science · Physics 2014-07-15 László Gránásy , Frigyes Podmaniczky , Gyula I. Tóth , György Tegze , Tamás Pusztai

We study the nucleation of crystalline cluster phases in the generalized exponential model with exponent n=4. Due to the finite value of this pair potential for zero separation, at high densities the system forms cluster crystals with…

Soft Condensed Matter · Physics 2016-09-01 Christian Leitold , Christoph Dellago

We consider the problem of gelation in the cluster coagulation model introduced by Norris [\textit{Comm. Math. Phys.}, 209(2):407-435 (2000)], where pairs of clusters of types $(x,y)$ taking values in a measure space $E$, merge to form a…

Probability · Mathematics 2025-08-08 Luisa Andreis , Tejas Iyer , Elena Magnanini

Understanding the pathways to crystallization during the deposition of a vapor phase on a cold solid substrate is of great interest in industry, e.g., for the realization of electronic devices made of crystallites-free glassy materials, as…

Soft Condensed Matter · Physics 2023-10-03 Fabio Leoni , Hajime Tanaka , John Russo

Quantum corrections can be important for diffusion and the melting temperature of dense plasmas in compact astrophysical objects, particulary white dwarfs and neutron stars. Typically ions in these systems are modeled classically, but…

Solar and Stellar Astrophysics · Physics 2015-03-19 Justin Mason

Hard-sphere model systems are well-suited in both experiment and simulations to investigate fundamental aspects of the crystallization of fluids. In experiments on colloidal models of hard-sphere fluids, the uid is unavoidably at contact…

Soft Condensed Matter · Physics 2021-04-28 Jorge R. Espinosa , Carlos Vega , Chantal Valeriani , Daan Frenkel , Eduardo Sanz

We used molecular dynamics simulations and the path sampling technique known as forward flux sampling to study homogeneous nucleation of NaCl crystals from supersaturated aqueous solutions at 298 K and 1 bar. Nucleation rates were obtained…

Chemical Physics · Physics 2018-02-14 Hao Jiang , Amir Haji-Akbari , Pablo G. Debenedetti , Athanassios Z. Panagiotopoulos

Homogeneous melting of superheated crystals at constant energy is a dynamical process, believed to be triggered by the accumulation of thermal vacancies and their self-diffusion. From microcanonical simulations we know that if an ideal…

Statistical Mechanics · Physics 2019-02-27 Sergio Davis , Claudia Loyola , Joaquín Peralta

Although numerous white dwarf stars host dusty debris disks, the temperature distribution of these stars differs significantly from the white dwarf population as a whole. Dusty debris disks exist exclusively around white dwarfs cooler than…

Earth and Planetary Astrophysics · Physics 2021-06-09 Jordan K. Steckloff , John Debes , Amy Steele , Brandon Johnson , Elisabeth R. Adams , Seth A. Jacobson , Alessondra Springmann

To predict the radiative forcing of clouds it is necessary to know the rate with which ice homogeneously nucleates in supercooled water. Such rate is often measured in drops to avoid the presence of impurities. At large supercooling small…

Soft Condensed Matter · Physics 2020-03-06 Jorge R. Espinosa , Carlos Vega , Eduardo Sanz

We perform direct large molecular dynamics simulations of homogeneous SPC/E water nucleation, using up to $\sim 4\cdot 10^6$ molecules. Our large system sizes allow us to measure extremely low and accurate nucleation rates, down to $\sim…

Atomic and Molecular Clusters · Physics 2015-09-02 R. Angelil , J. Diemand , K. Tanaka , H. Tanaka

We use molecular simulation to calculate the nucleation free energy barrier for the freezing of a 456 atom gold cluster over a range of temperatures. The results show that the embryo of the solid cluster grows at the vapor-surface interface…

Soft Condensed Matter · Physics 2007-05-23 Eduardo Mendez-Villuendas Richard K. Bowles

We determined bulk crystal nucleation rates in aqueous suspensions of charged spheres at low metastability. Experiments were performed in dependence on electrolyte concen-tration and for two different particle number densities. The…

Soft Condensed Matter · Physics 2021-11-04 Jürgen Schwarz , Paul Leiderer , Thomas Palberg

We study the homogeneous nucleation process in Stillinger-Weber silicon in the NVT ensemble. A clear first-order transition from the liquid to crystal phase is observed thermodynamically with kinetic and structural evidence of the…

Materials Science · Physics 2009-11-10 Philippe Beaucage , Normand Mousseau

The layered crystal formation in dusty plasma medium depicted by the Yukawa interaction amidst dust has been investigated using Molecular Dynamics simulations. The multilayer structures are shown to form in the presence of a combined…

Plasma Physics · Physics 2018-12-14 Srimanta Maity , Amita Das

Gamma ray heating and neutrino cooling rates, due to weak interaction processes, on $sd$-shell nuclei in stellar core are calculated using the proton neutron quasiparticle random phase approximation theory. The recent extensive experimental…

Nuclear Theory · Physics 2025-05-05 Muhammad Fayaz , Jameel-Un Nabi , Muhammad Majid

White dwarfs are stellar embers depleted of nuclear energy sources that cool over billions of years. These stars, which are supported by electron degeneracy pressure, reach densities of 1e7 grams per cubic centimetre in their cores. It has…

Nuclear weak rates in stellar environments are obtained by shell-model calculations including Gamow-Teller (GT) and spin-dipole transitions, and applied to nuclear weak processes in stars. The important roles of accurate weak rates for the…

Nuclear Theory · Physics 2022-06-24 Toshio Suzuki

Accurate estimate of nucleation rate is crucial for the study of ice nucleation and ice-promoting/anti-freeze strategies. Within the framework of Classical Nucleation Theory (CNT), the estimate of ice nucleation rate is very sensitive to…

Soft Condensed Matter · Physics 2021-07-07 Chaohong Wang , Hao Wang , Jianyang Wu , Zhisen Zhang

We investigate vapor homogeneous nucleation in a superheated Lennard Jones liquid with computer simulations. Special simulation techniques are required to address this study since the nucleation of a critical vapor bubble --one that has…

Soft Condensed Matter · Physics 2020-03-06 Pablo Rosales-Pelaez , Marta Irene Garcia-Cid , Chantal Valeriani , Carlos Vega , Eduardo Sanz