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Heterogeneous catalysts consisting of supported metallic nanoparticles typically derive exceptional catalytic activity from their large proportion of under-coordinated surface sites which promote adsorption of reactant molecules.…

Materials Science · Physics 2022-10-03 James P. Horwath , Colin Lehman-Chong , Aleksandra Vojvodic , Eric A. Stach

The simulation of quantum transport in a realistic, many-particle system is a nontrivial problem with no quantitatively satisfactory solution. While real-time propagation has the potential to overcome the shortcomings of conventional…

Mesoscale and Nanoscale Physics · Physics 2015-10-16 Justin E. Elenewski , Yanxiang Zhao , Hanning Chen

Quantum coherence is a fundamental characteristic to distinguish quantum systems from their classical counterparts. Though quantum coherence persists in isolated non-interacting systems, interactions inevitably lead to decoherence, which is…

Quantum Gases · Physics 2017-11-15 Ke-Ji Chen , Ho Kwan Lau , Hon Ming Chan , Dajun Wang , Qi Zhou

We use state- and time-resolved coherent Raman spectroscopy to study the rotational dynamics of oxygen molecules in ultra-high rotational states. While it is possible to reach rotational quantum numbers up to $N \approx 50$ by increasing…

Chemical Physics · Physics 2015-06-19 Alexander A. Milner , Aleksey Korobenko , Valery Milner

We summarize our results on decoherence for short- to intermediate-time dynamics of an externally controlled two-state quantum system - a qubit - interacting with thermal bosonic environment. The developed approximation schemes are…

Quantum Physics · Physics 2010-09-22 Vladimir Privman , Dmitry Solenov

The role of quantum coherence loss in mixed quantum-classical dynamical systems is explored in the context of the theory of quantum decoherence introduced recently by Bittner and Rossky. (J. Chem. Phys. {\bf 103}, 8130 (1995)). This theory,…

Chemical Physics · Physics 2009-10-30 Eric R. Bittner , Peter J. Rossky

The fact that gravitational environments cannot be shielded (since gravity is universal) makes them of great theoretical interest to decoherence mechanisms and to the quantum-to-classical transition. While past results seemed to indicate…

Quantum Physics · Physics 2026-02-27 Thiago H. Moreira , Lucas Chibebe Céleri

We analyze quantum interference and decoherence effects in single-molecule junctions both experimentally and theoretically by means of the mechanically controlled break junction technique and density-functional theory. We consider the case…

Mesoscale and Nanoscale Physics · Physics 2012-09-26 Stefan Ballmann , Rainer Härtle , Pedro B. Coto , Marcel Mayor , Mark Elbing , Martin R. Bryce , Michael Thoss , Heiko B. Weber

Neutrino interactions with an external environment can in influence the neutrino oscillation pattern and the oscillations can be damped as a result of the neutrino quantum decoherence. In particular, the quantum decoherence of neutrino…

High Energy Physics - Phenomenology · Physics 2020-05-20 Konstantin Stankevich , Alexander Studenikin

The adsorption phenomenon of neutral particles from the limiting surfaces of the sample in the Langmuir approximation is investigated. The diffusion equation regulating the redistribution of particles in the bulk is assumed to be of…

Mathematical Physics · Physics 2014-02-13 A Sapora , M Codegone , G Barbero , LR Evangelista

The quantum dynamics of a subset of interacting bosons in a subspace of fixed particle number is described in terms of symmetrized many-particle states. A suitable partial trace operation over the von Neumann equation of an $N$-particle…

Quantum Physics · Physics 2018-02-21 Manuel Gessner , Andreas Buchleitner

We consider electronic transport through a single-molecule junction where the molecule has a degenerate spectrum. Unlike previous transport models, and theories a rate-equations description is no longer possible, and the quantum coherences…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Maximilian G. Schultz

The dynamics of many open quantum systems are described by stochastic master equations. In the discrete-time case, we recall the structure of the derived quantum filter governing the evolution of the density operator conditioned to the…

Optimization and Control · Mathematics 2015-03-23 Pierre Six , Philippe Campagne-Ibarcq , Landry Bretheau , Benjamin Huard , Pierre Rouchon

Physical systems in real life are inextricably linked to their surroundings and never completely separated from them. Truly closed systems do not exist. The phenomenon of decoherence, which is brought about by the interaction with the…

High Energy Physics - Phenomenology · Physics 2024-07-11 Gabriela Barenboim , Alberto M. Gago

On this work, we consider a particle moving in front of a dielectric plate, and study two of the most relevant effects of the vacuum field fluctuations: the dissipation, and the decoherence of the particle's internal degrees of freedom. We…

Quantum Physics · Physics 2016-04-19 M. Belén Farias , Fernando C. Lombardo

Noneqiuilibrium dynamics of rotating droplets are studied by molecular dynamics simulations. Small deviations from the theoretical prediction are observed when the size of a droplet is small, and the deviations become smaller as the size of…

Computational Physics · Physics 2011-06-02 Hiroshi Watanabe , Naoki Mitsuda , Tomoaki Nogawa , Nobuyasu Ito

Our ability to numerically model and understand the complex flow behavior of solid-bearing suspensions has increased significantly over the last couple of years, partly due to direct numerical simulations that compute flow around individual…

Computational Physics · Physics 2019-03-21 Zhipeng Qin , Kali Alison , Jenny Suckale

Complex molecules are intriguing objects at the interface between quantum and classical phenomena. Compared to the electrons, neutrons, or atoms studied in earlier matter-wave experiments, they feature a much more complicated internal…

Quantum Physics · Physics 2022-04-27 Markus Arndt , Stefan Gerlich , Klaus Hornberger

We investigate the dynamics of nanoparticles in semidilute polymer solutions when the nanoparticles are comparably sized to the polymer coils using explicit- and implicit-solvent simulation methods. The nanoparticle dynamics are…

There has been considerable interest over the past years in investigating the role of gravity in quantum phenomenon such as entanglement and decoherence. In particular, gravitational time dilation is believed to decohere superpositions of…

General Relativity and Quantum Cosmology · Physics 2023-04-03 Raghvendra Singh , Kabir Khanna , Dawood Kothawala