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Plasmonic dimer cavities can induce extreme electric-field hot spots that allow one to access ultrastrong coupling regimes using Raman-type spectroscopy on single vibrating molecules. Using a generalized master equation, we study resonant…

Quantum Physics · Physics 2021-07-29 Stephen Hughes , Alessio Settineri , Salvatore Savasta , Franco Nori

Parametric amplification is a key ingredient of a wide range of phenomena, from the classical to the quantum domain. Although such phenomena have been demonstrated in non-equilibrium settings, their use for fluctuation engineering has been…

Quantum Physics · Physics 2025-11-12 H. P. Ojeda Collado , Ludwig Mathey

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

Resonance Raman scattering, which probes electrons, phonons and their interplay in crystals, is extensively used in two-dimensional materials. Here we investigate Raman modes in MoSe$_2$ at different laser excitation energies from 2.33 eV…

We investigated interlayer phonon modes of mechanically exfoliated few-layer 2H-SnS2 samples by using room temperature low-frequency micro-Raman spectroscopy. Raman measurements were performed using laser wavelength of 441.6, 514.4, 532 and…

Materials Science · Physics 2018-07-16 Tharith Sriv , Kangwon Kim , Hyeonsik Cheong

A consistent semiquantitative theoretical analysis of electronic Raman scattering from many-electron quantum dots under resonance excitation conditions has been performed. The theory is based on random-phase-approximation-like wave…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Alain Delgado , Augusto Gonzalez , D. J. Lockwood

Phonon polaritons are hybrid states of light and matter that are typically realised when optically active phonons couple strongly to photons. We suggest a new approach to realising phonon polaritons, by employing a transverse-pumping Raman…

Mesoscale and Nanoscale Physics · Physics 2024-10-22 Alexander N. Bourzutschky , Benjamin L. Lev , Jonathan Keeling

The line shape of the double-resonant $2D$ Raman mode in bilayer graphene is often considered to be characteristic for a certain laser excitation energy. Here, in a joint experimental and theoretical study, we analyze the dependence of the…

Mesoscale and Nanoscale Physics · Physics 2018-12-19 Felix Herziger , Christoph Tyborski , Oliver Ochedowski , Marika Schleberger , Janina Maultzsch

Stimulated low frequency Raman scattering (SLFRS) in single-crystal diamond films (SCD) with a graphitized layer built-in is investigated. SLFRS process in all studied structures has frequency shift in gigahertz range (5.1-13.2 GHz).…

Optics · Physics 2018-01-11 M. V. Tareeva , V. A. Dravin , R. A. Khmelnitsky , K. A. Tsarik

We report on the observation of both stable dissipative solitons and noise-like pulses with the presence of strong Raman scattering in a relatively short all-normal-dispersion Yb-doped fiber laser. We show that Raman scattering can be…

Optics · Physics 2015-10-28 Daojing Li , Deyuan Shen , Lei Li , Hao Chen , Dingyuan Tang , Luming Zhao

A theoretical study describing the coherence properties of near-field Raman scattering in two- and one-dimensional systems is presented. The model is applied to the Raman modes of pristine graphene and graphene edges. Our analysis is based…

Mesoscale and Nanoscale Physics · Physics 2014-03-31 Luiz Gustavo Cançado , Ryan Beams , Ado Jorio , Lukas Novotny

Raman spectra from silicon nanostructures, recorded using excitation laser power density of 1.0 kW/cm^2, is employed here to reveal the dominance of thermal effects at temperatures higher than the room temperature. Room temperature Raman…

Mesoscale and Nanoscale Physics · Physics 2012-01-25 Rajesh Kumar , Vivek Kumar , A. K. Shukla

Inelastic light (Raman) scattering has been used to study electronic excitations and phonon anomalies in detwinned, slightly overdoped YBa$_2$Cu$_3$O$_{6.95}$ and moderately overdoped Y$_{0.85}$Ca$_{0.15}$Ba$_2$Cu$_3$O$_{6.95}$ single…

Superconductivity · Physics 2015-05-13 M. Bakr , A. P. Schnyder , L. Klam , D. Manske , C. T. Lin , B. Keimer , M. Cardona , C. Ulrich

Time-resolved spontaneous Raman spectroscopy serves as a probe for incoherent quasiparticle and collective excitation dynamics, and allows to distinguish symmetry changes across a photoinduced phase transition through the inelastic light…

Materials Science · Physics 2019-03-27 J. Zhu , R. B. Versteeg , P. Padmanabhan , P. H. M. van Loosdrecht

We study the variations of electron-phonon coupling and their spectroscopic consequences in response to sliding of two layers in bilayer graphene using first-principles calculations and a model Hamiltonian. Our study shows that the long…

Mesoscale and Nanoscale Physics · Physics 2013-07-25 Seon-Myeong Choi , Seung-Hoon Jhi , Young-Woo Son

We investigate the modulation of optical phonons in semiconductor crystal by surface acoustic wave (SAW) propagating on the crystal surface. The SAW fields induce changes on the order of 10\textsuperscript{-3} in the average Raman…

Mesoscale and Nanoscale Physics · Physics 2016-06-08 F. Iikawa , A. Hernández-Mínguez , M. Ramsteiner , P. V. Santos

Raman spectroscopy is a powerful technique to characterize materials. It probes non-destructively chemical composition, crystallinity, defects, strain and coupling phenomena. However, the Raman response of surfaces or thin films is often…

In a recent report sum-frequency excitation of a Raman-active phonon was experimentally demonstrated for the first time. This mechanism is the sibling of impulsive stimulated Raman scattering, in which difference-frequency components of a…

Materials Science · Physics 2018-05-23 Dominik M. Juraschek , Sebastian F. Maehrlein

Phonon polaritons (PhPs) are hybrid photon-phonon waves which enable strong light-matter interactions and subdiffractional confinement, potentially empowering applications in sensing, nonlinear optics and nanoscale energy manipulation. In…

A comparison of experimentally observed Raman scattering data with Raman line-shapes, generated theoretically using phonon confinement model, has been carried out to understand the sensitivity of different Raman spectral parameters on…

Mesoscale and Nanoscale Physics · Physics 2020-03-20 Neeshu K. M. , Chanchal Rani , Ritika Kaushik , Manushree Tanwar , Ashisha Kumar , Rajesh Kumar