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The structural features of polystyrene brushes grafted on spherical silica nanoparticles immersed in polystyrene are investigated by means of a Monte Carlo methodology based on polymer mean field theory. The nanoparticle radii (either 8 nm…

Soft Condensed Matter · Physics 2014-01-17 Georgios G. Vogiatzis , Doros N. Theodorou

A large body of experimental work on the microstructure and dynamics of simplifiedindustrial nanocomposites made of disordered silica filler in a styrene-butadiene matrixby solid-phase mixing is regrouped and critically discussed in this…

Soft Condensed Matter · Physics 2018-11-21 Anne-Caroline Genix , Guilhem P. Baeza , Julian Oberdisse

The present communication reports the first direct measurement of the conformation of a polymer corona grafted around silica nano-particles dispersed inside a nanocomposite, a matrix of the same polymer. This measurement constitutes an…

It has recently been proposed that the miscibility of nanoparticles with a polymer matrix can be controlled by grafting polymer chains to the nanoparticle surface. As a first step to study this situation, we have used molecular dynamics…

Soft Condensed Matter · Physics 2010-08-06 Joshua Kalb , Douglas Dukes , Sanat K. Kumar , Robert S. Hoy , Gary S. Grest

The self-assembly of copolymeric vesicles and micelles in micromixers is studied by External Potential Dynamics (EPD) simulations -- a dynamic density functional approach that explicitly accounts for the polymer architecture both at the…

Soft Condensed Matter · Physics 2018-04-10 Simon Kessler , Klaus Drese , Friederike Schmid

We examine the dynamics of silica particles grafted with high molecular weight polystyrene suspended in semidilute solutions of chemically similar linear polymer using x-ray photon correlation spectroscopy. The particle dynamics decouple…

Soft Condensed Matter · Physics 2019-08-27 Ryan Poling-Skutvik , Ali H. Slim , Suresh Narayanan , Jacinta C. Conrad , Ramanan Krishnamoorti

This paper presents a study of the polymer-filler interfacial effects on filler dispersion and mechanical reinforcement in Polystyrene (PS) / silica nanocomposites by direct comparison of two model systems: un-grafted and PS-grafted silica…

Soft Condensed Matter · Physics 2011-07-12 Chloé Chevigny , Nicolas Jouault , Florent Dalmas , François Boué , Jacques Jestin

Inhaled nanoparticles (< 100 nm) reaching the deep lung region first interact with the pulmonary surfactant, a thin lipid film lining the alveolar epithelium. To date, most biophysical studies have focused on particle induced modifications…

Soft Condensed Matter · Physics 2021-09-21 L. P. A. Thai , F. Mousseau , E. K. Oikonomou , M. Radiom , J. -F. Berret

To prevent the flocculation and phase separation of nanoparticles in solution, nanoparticles are often functionalized with short chain surfactants. Here we present fully-atomistic molecular dynamics simulations which characterize how these…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 J. Matthew D. Lane , Ahmed E. Ismail , Michael Chandross , Christian D. Lorenz , Gary S. Grest

Mixtures of nanoparticles and polymer-like objects are encountered in many nanotechnological applications and biological systems. We study the behavior of grafted polymer layers decorated by nanoparticles that are attracted to the polymers…

Soft Condensed Matter · Physics 2011-10-31 Michael G. Opferman , Rob D. Coalson , David Jasnow , Anton Zilman

Cells offer numerous inspiring examples where proteins and membranes combine to form complex structures that are key to intracellular compartmentalization, cargo transport, and specialization of cell morphology. Despite this wealth of…

We investigate the flow of spherical, bulk granular particles down an inclined plane mixed with small-sized spherical lubricant particles using discrete element method simulations. Predefined cohesive interaction is implemented between…

Soft Condensed Matter · Physics 2026-04-27 Sayali V. Chaudhary , Ashish V. Orpe

An aqueous suspension of silica nanoparticles or nanofluid can alter the wettability of surfaces, specifically by making them hydrophilic and oil-repellent under water. Wettability alteration by nanofluids have important technological…

Applied Physics · Physics 2021-08-13 Shidong Li , Anqi Sng , Dan Daniel , Hon Chung Lau , Ole Torsæter , Ludger P. Stubbs

Hypothesis: Slippery Omniphobic Covalently Attached Liquids (SOCAL) have been proposed for making omnirepellent thin films of self-assembled dimethylsiloxane polymer brushes grafted from silica surfaces. Smooth and flat at very small scale,…

Soft Condensed Matter · Physics 2023-11-21 M. Callau , C. Fajolles , J. Leroy , E. Verneuil , Patrick Guenoun

The ordering of nanoparticles into predetermined configurations is of importance to the design of advanced technologies. In this work, we moderate the surface anchoring against the bulk elasticity of liquid crystals to dynamically shape…

Soft Condensed Matter · Physics 2023-12-01 Lisa Tran , Hye-Na Kim , Ningwei Li , Shu Yang , Kathleen J. Stebe , Randall D. Kamien , Martin F. Haase

Ordering nanoparticles into a desired super-structure is often crucial for their technological applications. We use molecular dynamics simulations to study the assembly of nanoparticles in a polymer brush randomly grafted to a planar…

Soft Condensed Matter · Physics 2017-12-11 Shengfeng Cheng , Mark J. Stevens , Gary S. Grest

We performed molecular dynamics simulations to study equilibrium and flow properties of a liquid in a nano-channel with confining surfaces coated with a layer of grafted semiflexible polymers. The coverage spans a wide range of grafting…

Computational Physics · Physics 2015-09-30 Kevin Speyer , Claudio Pastorino

The presence of nanoparticles in a diblock copolymer leads to changes in the morphology and properties of the matrix and can produce highly organized hybrid materials. The resulting material properties depend not only on the polymer…

Soft Condensed Matter · Physics 2018-05-30 Javier Diaz , Marco Pinna , Andrei Zvelindovsky , Adelchi Asta , Ignacio Pagonabarraga

Surfactants are often used to stabilise two-dimensional (2D) materials in environmentally friendly solvents such as water. Aqueous-surfactant solutions prevent agglomeration of nanosheets through steric and electrostatic repulsion,…

Materials Science · Physics 2021-11-05 Diego Tomohisa Pérez-Álvarez , Philip Davies , Jason Stafford

Liquids in contact with solids are submitted to intermolecular forces making liquids heterogeneous and stress tensors are not any more spherical as in homogeneous bulks. The aim of this article is to show that a square-gradient functional…

Classical Physics · Physics 2017-08-23 Henri Gouin
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