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We use X-Ray Photon Correlation Spectroscopy to investigate the structural relaxation process in a metallic glass on the atomic length scale. We report evidence for a dynamical crossover between the supercooled liquid phase and the…

Soft Condensed Matter · Physics 2015-06-11 B. Ruta , Y. Chushkin , G. Monaco , L. Cipelletti , E. Pineda , P. Bruna , V. M. Giordano , M. Gonzalez-Silveira

Relaxation processes significantly influence the properties of glass materials. However, understanding their specific origins is difficult, even more challenging is to forecast them theoretically. In this study, using microseconds molecular…

Materials Science · Physics 2019-09-09 Yang Sun , Si-Xu Peng , Qun Yang , Feng Zhang , Meng-Hao Yang , Cai-Zhuang Wang , Kai-Ming Ho , Hai-Bin Yu

We solve exactly and describe in detail a simplified scalar model for the low frequency shear rheology of foams, emulsions, slurries, etc. [P. Sollich, F. Lequeux, P. Hebraud, M.E. Cates, Phys. Rev. Lett. 78, 2020 (1997)]. The model…

Soft Condensed Matter · Physics 2007-05-23 Peter Sollich

Dilute oil dispersions of fractal carbon black particles with attractive Van der Waals interactions display continuous shear thickening followed by shear thinning at high shear rates. The shear thickening transition occurs at…

Soft Condensed Matter · Physics 2009-11-13 Chinedum O. Osuji , Chanjoong Kim , David A. Weitz

An analytical framework is proposed to describe the elasticity, viscosity and fragility of metallic glasses in relation to their atomic-level structure and the effective interatomic interaction. The bottom-up approach starts with forming an…

Soft Condensed Matter · Physics 2016-08-15 Alexandra E. Lagogianni , Johannes Krausser , Zach Evenson , Konrad Samwer , A Zaccone

Using density-functional molecular dynamics simulations we analyzed the cooling-rate effects on the physical properties of GeS$_2$ chalcogenide glasses. Liquid samples were cooled linearly in time according to $T(t) = T_0 - \gamma t$ where…

Disordered Systems and Neural Networks · Physics 2007-05-23 Sebastien Le Roux , Philippe Jund

The dependence of mechanical properties on microscopic interactions remains a central problem in the physics of disordered solids near the jamming transition. We numerically and theoretically investigate the mechanical response of jammed…

Soft Condensed Matter · Physics 2026-04-07 Michio Otsuki , Kiwamu Yoshii , Hideyuki Mizuno

Metallic glasses response to the mechanical stress in a complex and inhomogeneous manner with plastic strain highly localized into nanoscale shear bands. Contrary to the well-defined deformation mechanism in crystalline solids,…

Materials Science · Physics 2020-07-01 Baoan Sun , Liping Yu , Gang Wang , Xing Tong , Chuan Geng , Jingtao Wang , Jingli Ren , Weihua Wang

The structure, thermodynamics and slow activated dynamics of the equilibrated metastable regime of glass-forming fluids remains a poorly understood problem of high theoretical and experimental interest. We apply a highly accurate…

Soft Condensed Matter · Physics 2024-08-21 Subhashish Chaki , Baicheng Mei , Kenneth S. Schweizer

Rheological measurements of model colloidal gels reveal that large variations in the shear moduli as colloidal volume-fraction changes are not reflected by simple structural parameters such as the coordination number, which remains almost a…

Soft Condensed Matter · Physics 2018-08-07 D. Zeb Rocklin , Lilian C. Hsiao , Megan Szakasits , Michael J. Solomon , Xiaoming Mao

Molecular dynamics simulations are carried out to investigate mechanical properties and porous structure of binary glasses subjected to steady shear. The model vitreous systems were prepared via thermal quench at constant volume to a…

Soft Condensed Matter · Physics 2017-11-29 Nikolai V. Priezjev , Maxim A. Makeev

We have established a comprehensive study of the molecular dynamics of the menthol-thymol mixture, the prototype of the new class of type V deep eutectic solvents. Dielectric spectroscopy and differential scanning calorimetry were combined…

Soft Condensed Matter · Physics 2022-08-23 Claire D'Hondt , Denis Morineau

Theoretical approaches are formulated to investigate the molecular mobility under various cooling rates of amorphous drugs. We describe the structural relaxation of a tagged molecule as a coupled process of cage-scale dynamics and…

Soft Condensed Matter · Physics 2019-12-10 Anh D. Phan , Katsunori Wakabayashi , Marian Paluch , Vu D. Lam

We construct a linear response theory of applying shear deformations from boundary walls in the film geometry in Kubo's theoretical scheme. Our method is applicable to any solids and fluids. For glasses, we assume quasi-equilibrium around a…

Soft Condensed Matter · Physics 2018-12-27 Akira Onuki , Takeshi Kawasaki

Shear localization in slowly-driven bulk metallic glasses (BMGs) is typically accompanied by a sharp drop in the bulk stress response as a signature of the plastic yielding transition. It is also observed that the sharpness of this…

Soft Condensed Matter · Physics 2023-09-22 Kamran Karimi , Stefanos Papanikolaou

We study the shear induced fluidization of amorphous solids subjected to external loading by investigating the relaxation dynamics of the deformed states using computer simulation. A simple shear deformation is employed at constant rate to…

Soft Condensed Matter · Physics 2021-12-07 Santhosh Kumar R , Bhaskar Sen Gupta

Cycling of a metallic glass between ambient and cryogenic temperatures can induce higher-energy states characteristic of glass formation on faster cooling. This rejuvenation, unexpected because it occurs at small macroscopic strains and…

Disordered Systems and Neural Networks · Physics 2022-09-22 Baoshuang Shang , Weihua Wang , Alan Lindsay Greer , Pengfei Guan

The internal states or local structures of bulk metallic glass (BMGs) can be well reflected from the changes of density, structural relaxation as well as the elastic constants. With the increasing free volume (FV) content, more local atomic…

Materials Science · Physics 2013-10-11 J. Tan , C. J. Li , Y. H. Jiang , R. Zhou , J. Eckert

This investigation extends earlier studies of a shear-transformation-zone (STZ) theory of plastic deformation in amorphous solids. My main purpose here is to explore the possibility that the configurational degrees of freedom of such…

Materials Science · Physics 2009-11-10 J. S. Langer

We report surface shear rheological measurements on dense insoluble monolayers of micron sized colloidal spheres at the oil/water interface and of the protein $\beta$-lactoglobulin at the air/water surface. As expected, the elastic modulus…

Soft Condensed Matter · Physics 2009-11-10 Pietro Cicuta , Edward J. Stancik , Gerald G. Fuller
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