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The development of compact and bright XUV and soft X-ray sources based on high-order harmonic generation is boosting advances towards understanding the behavior of matter with extreme temporal and spatial resolutions. Here, we report…

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

Strongly Correlated Electrons · Physics 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki

High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG…

Optics · Physics 2023-04-26 Liang Li , Pengfei Lan , Xiaosong Zhu , Peixiang Lu

The high-order harmonic generation (HHG), if phase matched, opens a unique way to produce coherent ultrafast extreme-UV (XUV) or soft x-ray light sources. Here we describe a robust and tunable method for scaling and narrowing the bandwidth…

Optics · Physics 2017-10-03 L. Mashhadi , G. Shayeganrad

High-harmonic generation (HHG) in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. Here we argue that the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Joel D. Cox , Andrea Marini , F. Javier García de Abajo

Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we…

Optics · Physics 2024-10-16 Thomas K. Allison , Alice Kunin , Gerd Schönhense

High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic…

Ultrafast light sources have become an indispensable tool to access and understand transient phenomenon in material science. However, a simple and easy-to-implement method for harmonic selection, with high transmission efficiency and pulse…

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

We demonstrate the highest flux tabletop source of coherent soft X-rays to date, driven by a single-stage 10 mJ Ti:sapphire regenerative amplifier at 1 kHz. We first down-convert the laser to 1.3 um using a parametric amplifier, before…

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

High harmonic generation (HHG) in solids has emerged as a powerful spectroscopic method for resolving ultrafast electron dynamics and band structure properties across a wide range of materials. However, quantitative HHG studies require…

Optics · Physics 2025-12-16 S. Mandal , P. Kumar , Z. Pi , H. Y. Kim , M. Zhan , E. Goulielmakis

High harmonic generation (HHG) has become a multipurpose source of coherent XUV radiation used in various applications. One of the notable aspects of HHG is its wide spectrum consisting of many harmonic orders. This might represent a…

Coherent extreme ultraviolet (XUV) radiation produced by table-top high-harmonic generation (HHG) sources provides a wealth of possibilities in research areas ranging from attosecond physics to high resolution coherent imaging. However, it…

Optics · Physics 2016-10-28 G. S. M. Jansen , D. Rudolf , L. Freisem , K. S. E. Eikema , S. Witte

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

We have successfully developed and implemented an entire and compact table-top high-order harmonics generation (HHG) setup from monochromatic and intense femtosecond ($10^{-15}$ s) laser pulses launched in a target composed of a high-purity…

Each successive generation of x-ray machines has opened up new frontiers in science, such as the first radiographs and the determination of the structure of DNA. State-of-the-art x-ray sources can now produce coherent high brightness keV…

Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for…

Phase-matched harmonic conversion of visible laser light into soft x-rays was demonstrated. The recently developed technique of guided-wave frequency conversion was used to upshift light from 800 nanometers to the range from 17 to 32…

Electromagnetic radiation in the soft x-ray spectral range ($1-100~\rm{nm}$ wavelengths or $0.01-1~\rm{keV}$ photon energies) is rapidly gaining importance in both fundamental research and industrial applications. At present the degree of…