Related papers: Chiral broadband High Harmonic Generation Source b…
By experimentally studying high-order harmonic beams generated in gases, we show how the spatial characteristics of these ultrashort XUV beams can be finely controlled under standard generation conditions. For the first time, we demonstrate…
High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…
Coherent supercontinuum radiation in the extreme-ultraviolet (XUV) range is indispensable for synthesizing attosecond light pulses and for exploring transient atomic structures. Here, we report the striking observations of coherent XUV…
Topological materials are of interest to both fundamental science and advanced technologies, because topological states are robust with respect to perturbations and dissipation. Experimental detection of topological invariants is thus in…
Ever since the advent of high-order harmonic generation, one of the main goals has been to maximize the high harmonic yield. This is due to the wide range of applications in multidisciplinary research fields, including nonlinear XUV optics…
In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…
Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave…
The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…
High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…
We describe an approach based on topology optimization that enables automatic discovery of wavelength-scale photonic structures for achieving high-efficiency second-harmonic generation (SHG). A key distinction from previous formulation and…
Understanding the mechanisms and spatial correlations of crystallographic symmetry breaking in ferroelectric materials is essential to tuning their functional properties. While optical second harmonic generation (SHG) has long been utilized…
With its direct correspondence to electronic structure, angle-resolved photoemission spectroscopy (ARPES) is a ubiquitous tool for the study of solids. When extended to the temporal domain, time-resolved (TR)-ARPES offers the potential to…
Unraveling and controlling chemical dynamics requires techniques to image structural changes of molecules with femtosecond temporal and picometer spatial resolution. Ultrashort-pulse x-ray free-electron lasers have significantly advanced…
Second harmonic generation microscopy (SHG) is a powerful imaging modality which has found applications in investigating both biological and synthetic nanostructures. Like all optical microscopy techniques, the resolution of SHG is limited…
The ability to control absorption by modifying the polarization of light presents an exciting opportunity to experimentally determine the orbital alignment of absorption features. Here, attosecond extreme ultraviolet (XUV) transient…
We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…
X-ray devices are far superior to optical ones for providing nanometre spatial and attosecond temporal resolutions. Such resolution is indispensable in biology, medicine, physics, material sciences, and their applications. A bright…
Many atomic and molecular systems of fundamental interest possess resonance frequencies in the extreme ultraviolet (XUV) where laser technology is limited and radiation sources have traditionally lacked long-term phase coherence. Recent…
A step towards a successful implementation of timeresolved digital in-line holography with extreme ultraviolet radiation is presented. Ultrashort XUV pulses are produced as high-order harmonics of a femtosecond laser and a Schwarzschild…
High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…