Related papers: Extracting RABBITT-like phase information from tim…
We reveal for the first time that ultraviolet (UV) observables can diagnose quantum phase transitions (QPTs). In a class of holographic models exhibiting metal-insulator transitions, we study two types of UV observables -- high-frequency…
We study effects of nonadiabatic couplings in a model of a diatomic molecule in the context of attosecond transient absorption spectroscopy. By using a model system consisting of four diabatic electronic states and with a variable strength…
The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) can become resonant with a discrete atomic level either in the intermediate or the final continuous states. Experimental observations of…
The electronic excitation occurring on adsorbates at ultrafast time scales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of X-ray absorption…
We employ the Dirac-Frenkel variational principle and multiple Davydov ansatz to study time-dependent fluorescence spectra of a driven qubit in the weak- to strong qubit-reservoir coupling regimes, where both the Rabi frequency and…
Hanbury-Brown Twiss (HBT) correlation measurements provide valuable information about the phase space distribution of matter in ultrarelativistic heavy-ion collisions. The rapidity dependence of HBT radii arises from a nontrivial interplay…
Non-collinear four-wave mixing (FWM) techniques at near-infrared (NIR), visible, and ultraviolet frequencies have been widely used to map vibrational and electronic couplings, typically in complex molecules. However, correlations between…
Ultrafast optical pulses are an increasingly important tool for controlling quantum materials and triggering novel photo-induced phase transitions. Understanding these dynamic phenomena requires a probe sensitive to spin, charge, and…
We investigate the ultrafast electron dynamics of a model of a wide-bandgap material with inner, valence, and conduction bands excited by an intense few-femtosecond pump and monitored by a delayed attosecond extreme-ultraviolet probe pulse.…
We theoretically study the effects of Rabi oscillations on resonant x-ray scattering in Ne$^+$ using intense attosecond and few-femtosecond pulses. The total photon yield strongly depends on the pulse area and has an upper bound at high…
A new approach for few-femtosecond time-resolved photoelectron spectroscopy in condensed matter that balances the combined needs for both temporal and energy resolution is demonstrated. Here, the method is designed to investigate a…
Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…
Using resonant light absorption, random walk motions of rubidium atoms in nitrogen buffer gas are observed directly. The transmitted light intensity through atomic vapor is measured and its spectrum is obtained, down to orders of magnitude…
We generalize the one electron attosecond streaking camera to time-resolve the correlated two-electron escape dynamics during a collision process involving a deep core electron. The collision process is triggered by an XUV attosecond pulse…
Recent seminal experiments have utilized time-resolved X-ray absorption spectroscopy (XAS) to investigate the ultrafast photo-induced renormalization of the electron interaction (''Hubbard $U$'') in Mott and charge transfer insulators. In…
This proceeding discusses nonequilibrium effects in matter exposed to XUV/X-ray irradiation. When ultrashort, intense XUV/X-ray pulses interact with materials, they trigger a complex sequence of processes, including electronic excitation,…
RMT is a program which solves the time-dependent Schrodinger equation for general, multielectron atoms, ions and molecules interacting with laser light. As such it can be used to model ionization (single-photon, multi-photon and…
The time-of-flight method is a fundamental approach for characterizing the transport properties of semiconductors. Recently, the transient photocurrent and optical absorption kinetics have been simultaneously measured for thin films;…
Phase retrieval is at the heart of adaptive optics and modern high-resolution imaging. Without phase information, optical systems are limited to intensity-only measurements, hindering full reconstruction of object structures and wavefront…
Ultrafast laser excitation can trigger multiplex coherent dynamics in molecules. Here, we report attosecond transient absorption experiments addressing simultaneous probing of electronic and vibrational dynamics in a prototype molecule,…