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Point defects play a central role in driving the properties of materials. First-principles methods are widely used to compute defect energetics and structures, including at scale for high-throughput defect databases. However, these methods…

Machine Learning · Computer Science 2025-09-30 Evan Dramko , Yihuang Xiong , Yizhi Zhu , Geoffroy Hautier , Thomas Reps , Christopher Jermaine , Anastasios Kyrillidis

Generalized gradient approximated (GGA) density functional theory (DFT) typically overestimates polarizability and bond-lengths, and underestimates force constants of covalent bonds. To overcome this problem we show that one can use…

Chemical Physics · Physics 2016-06-29 O. Anatole von Lilienfeld

The recent progress of using graph based encoding of crystal structures for high throughput material property prediction has been quite successful. However, using a single modality model prevents us from exploiting the advantages of an…

Machine Learning · Computer Science 2025-05-09 Abhiroop Bhattacharya , Sylvain G. Cloutier

Discovery of novel and promising materials is a critical challenge in the field of chemistry and material science, traditionally approached through methodologies ranging from trial-and-error to machine learning-driven inverse design. Recent…

Machine Learning · Computer Science 2024-12-13 Dong Hyeon Mok , Seoin Back

Deep learning has revolutionized the computer vision and image classification domains. In this context Convolutional Neural Networks (CNNs) based architectures are the most widely applied models. In this article, we introduced two…

Computer Vision and Pattern Recognition · Computer Science 2023-05-24 Seyedsaman Emami , Gonzalo Martínez-Muñoz

Pretrained foundation models learn embeddings that can be used for a wide range of downstream tasks. These embeddings optimise general performance, and if insufficiently accurate at a specific task the model can be fine-tuned to improve…

Machine Learning · Computer Science 2025-02-20 Matthew P. Wilson , Edward O. Pyzer-Knapp , Nicolas Galichet , Luke Dicks

The advent of neural-network-based deep learning techniques has led to the emergence of increasingly sophisticated numerical interatomic potentials, including graph neural networks and large language-motivated foundation models.…

Chemical Physics · Physics 2026-03-09 Susan R. Atlas

Large-scale atomistic simulations rely on interatomic potentials providing an efficient representation of atomic energies and forces. Modern machine-learning (ML) potentials provide the most precise representation compared to electronic…

Computational Physics · Physics 2025-04-23 David Immel , Ralf Drautz , Godehard Sutmann

A data-driven model augmentation framework, referred to as Weakly-coupled Integrated Inference and Machine Learning (IIML), is presented to improve the predictive accuracy of physical models. In contrast to parameter calibration, this work…

Computational Engineering, Finance, and Science · Computer Science 2022-07-25 Vishal Srivastava , Valentin Sulzer , Peyman Mohtat , Jason B. Siegel , Karthik Duraisamy

Overcoming the challenge of limited data availability within materials science is crucial for the broad-based applicability of machine learning within materials science. One pathway to overcome this limited data availability is to use the…

Materials Science · Physics 2024-12-24 Reshma Devi , Keith T. Butler , Gopalakrishnan Sai Gautam

We examine how the universality of two-nucleon interactions evolved using similarity renormalization group (SRG) transformations correlates with T-matrix equivalence, with the ultimate goal of gaining insight into universality for…

Nuclear Theory · Physics 2014-01-29 B. Dainton , R. J. Furnstahl , R. J. Perry

Given two or more Deep Neural Networks (DNNs) with the same or similar architectures, and trained on the same dataset, but trained with different solvers, parameters, hyper-parameters, regularization, etc., can we predict which DNN will…

Machine Learning · Computer Science 2020-01-28 Charles H. Martin , Michael W. Mahoney

Molecular representation learning is crucial for the problem of molecular property prediction, where graph neural networks (GNNs) serve as an effective solution due to their structure modeling capabilities. Since labeled data is often…

Machine Learning · Computer Science 2023-09-26 Cameron Diao , Kaixiong Zhou , Zirui Liu , Xiao Huang , Xia Hu

Invariance (defined in a general sense) has been one of the most effective priors for representation learning. Direct factorization of parametric models is feasible only for a small range of invariances, while regularization approaches,…

Machine Learning · Computer Science 2020-07-28 Yingyi Ma , Vignesh Ganapathiraman , Yaoliang Yu , Xinhua Zhang

Despite recent advances in representation learning in hypercomplex (HC) space, this subject is still vastly unexplored in the context of graphs. Motivated by the complex and quaternion algebras, which have been found in several contexts to…

Machine Learning · Computer Science 2022-02-22 Tuan Le , Marco Bertolini , Frank Noé , Djork-Arné Clevert

Efficient catalyst screening necessitates predictive models for adsorption energy, a key property of reactivity. However, prevailing methods, notably graph neural networks (GNNs), demand precise atomic coordinates for constructing graph…

Computational Engineering, Finance, and Science · Computer Science 2023-09-04 Janghoon Ock , Chakradhar Guntuboina , Amir Barati Farimani

The generalization accuracy of machine learning models of potential energy surfaces (PES) and force fields (FF) for large polyatomic molecules can be generally improved either by increasing the number of training points or by improving the…

Chemical Physics · Physics 2023-03-20 K. Asnaashari , R. V. Krems

Universal Machine Learning Interactomic Potentials (MLIPs) enable accelerated simulations for materials discovery. However, current research efforts fail to impactfully utilize MLIPs due to: 1. Overreliance on Density Functional Theory…

Materials Science · Physics 2025-02-07 Santiago Miret , Kin Long Kelvin Lee , Carmelo Gonzales , Sajid Mannan , N. M. Anoop Krishnan

Many modern neural network architectures are trained in an overparameterized regime where the parameters of the model exceed the size of the training dataset. Sufficiently overparameterized neural network architectures in principle have the…

Machine Learning · Computer Science 2019-02-14 Samet Oymak , Mahdi Soltanolkotabi

Many learning-based approaches have difficulty scaling to unseen data, as the generality of its learned prior is limited to the scale and variations of the training samples. This holds particularly true with 3D learning tasks, given the…

Computer Vision and Pattern Recognition · Computer Science 2020-12-15 Mingyue Yang , Yuxin Wen , Weikai Chen , Yongwei Chen , Kui Jia